Vortices are usually associated with systems containing large numbers of particles. Of particular topical interest though are those formed within atomic-scale wave functions and observed in macroscopic systems such as superfluids and quantum condensates. We uncover them here in one of the most fundamental quantum systems consisting of just one electron and two protons. Moreover, the results of novel simulations of the dynamics of this system reveal previously unknown mechanisms of angular momentum transfer and new ways to image atomic-scale quantized vortices at macroscopic distances. Probing of vortices and vortex-driven dynamics in quantum systems is thereby illustrated.
Vortices are usually associated with systems containing large numbers of particles. Of particular topical interest though are those formed within atomic-scale wave functions and observed in macroscopic systems such as superfluids and quantum condensates. We uncover them here in one of the most fundamental quantum systems consisting of just one electron and two protons. Moreover, the results of novel simulations of the dynamics of this system reveal previously unknown mechanisms of angular momentum transfer and new ways to image atomic-scale quantized vortices at macroscopic distances. Probing of vortices and vortex-driven dynamics in quantum systems is thereby illustrated.
Calculations of the time‐dependent wave function for proton impact on atomic hydrogen using the Lattice‐Time‐Dependent‐Schrödinger‐Equation (LTDSE) method [1] follow the wave function from microscopic to macroscopic times. Isolated zeros, now identified as vortices, appear when the target and projectile nuclei are separated by a few atomic units [2]. Such structure has apparently been observed frequently in ab. initio. calculations. Our work shows that such structures persist to macroscopic distances and appear as “holes” in electron momentum distributions. They can, in principle, be observed in reaction microscope studies. Such observation is formally justified by the “imaging theorem”, which can be derived from first principles. Similarly, two‐electron momentum distributions as observed, e.g., in (e,2e) coincidence measurements may show isolated zeros [3]. Calculations using correlated wave functions support the interpretation that a minima in (e,2e) for helium targets corresponds to a vortex. In this case the “imaging theorem” can be applied to argue that there must be vortices in the two‐electron wave function[4]. A general discussion of vortices in quantum mechanics will be illustrated using exact LTDSE calculations, and, for interpretive purposes, the time‐dependent first Born approximation. These calculations show that the plane wave B1 amplitudes have no vortices, but the time‐dependent B1 amplitudes do. It will be further shown that angular momentum transfer is the key to forming vortices in the time‐dependent theory.
The extension of quantum phenomena into macroscopic scales is responsible for a whole class of effects such as superconductivity, superfluidity, and Bose-Einstein condensation, which played central roles in physics throughout the last century.The production of the first Bose-Einstein condensates made possible the realization of experiments involving macroscopic quantum phenomena with an unprecedented level of control of the external parameters.The persistent currents in condensates are intimately related to the nucleation of quantized vortices, which are topological defects as response to transference of quanta of angular momentum.A conventional method for generation of such defects consists in confining the condensed atomic cloud into a rotating trap.It turns out that, for angular velocities higher than a critical value, vortex states become energetically favorable, thus inducing the creation of quantized vortices.Experimental realizations of condensed alkali-metal atoms confined by more general time-dependent potentials allowed the observation not only of vortex lattices but also of quantum turbulence.Since quantum turbulence is characterized by the presence of a self-interacting tangle of quantized vortices, the correct understanding of dynamics, formation, and stability of vortices has shown to be of paramount importance being the subject of many theoretical works.In particular, the role of acoustic excitations generated by decaying multi-charged vortices in the development of turbulence is still an open question.This work aims to provide a set of tools that helps to identify the presence as well as the charge of vortices in non-turbulent clouds observed using time-of-flight pictures.We have done a detailed study of condensates containing multi-charged vortices placed at its center where time-of-flight dynamics is only one point of our interest.Due to the control that this system provides experimentally, the collective modes become an important description since they can be excited using well stablished experimental methods as such as modulation of the s-wave scattering length, and they can also be responsible to vortex decaying.For such purposes we have used the semi-analytical variational method, and the fully numerical calculation of Gross-Pitaevskii equation.Thus we have describes the collective modes that couples dynamics of vortex with the oscillation of external components of condensed atomic cloud as well as the effects in time-of-flight.The angular momentum acts increasing the kinetic energy around the vortex core, which results in a faster expansion of perpendicular direction to it.This situation shifts the frequencies of collective oscillations of a vortex-free state, and generates richer collective modes due the coupling.Now there are four possible modes, being two types of monopole mode and two types of quadrupole modes.The difference among these types is the phase of vortex oscillation.When one considers fluctuations without polar symmetry, their collective modes result in the vortex decaying.In order to control and prevent these processes we have proposed three dynamical mechanisms such as modulation of s-wave scattering length, modulation of frequencies of harmonic trap, and modulation of the amplitude of Laguerre-Gauss potential.The last one has proven to be more effective.
The condensation of weakly interacting alkali atom gases observed in 1995 is a manifestation of the macroscopic quantum phenomenon called Bose-Einstein condensation. In contrast to superconductivity and Helium superfluids, the dilute alkali atom condensates are directly observable using optical imaging techniques and they constitute highly controllable quantum systems. Hence, they offer an ideal test bench to investigate the applicability of quantum field theories and to predict the properties of the condensates starting from the first principles.\n\nSince the first experimental realizations of dilute Bose-Einstein condensates, a great interest has been focused on this field, resulting in numerous experimental studies concerning, for example, nonlinear dynamics and the elementary excitations of these many-particle quantum systems. The existence of topological phase singularities, quantized vortices, first predicted theoretically and finally observed experimentally in 1999, led to another series of pioneering theoretical and experimental studies.\n\nSeveral methods to create single-quantum vortices were realized already in 2001 but, however, the puzzle of creating multiply quantized vortices still remained. In this thesis, the so-called topological method to create two and four times quantized vortices is studied in detail. Since the instrumentation required for the experimental realization of the topological method had already been installed in many laboratories, the theoretical predictions of this thesis were experimentally verified shortly after their publication. Multiply quantized vortices are energetically unstable and tend to split into singly quantized vortices. However, the dissipation of energy in the condensates is minimal at low temperatures and, consequently, can lead to long lifetimes for the multiquantum vortices. Nevertheless, one prediction of this thesis is that the lifetimes of doubly quantized vortices are relatively short, owing to the known dynamical instability of the state. The splitting of the doubly quantized vortex has recently been observed experimentally.\n\nThe stability of vortices in dilute Bose-Einstein condensates is intimately related to the excitation spectrum of the stationary vortex state. However, developing an accurate, computationally feasible finite-temperature quantum field theory remains an open problem. In this thesis, we study the elementary excitations of an irrotational condensate within a recently developed systematic second order perturbation theory. The collapse and revival of certain elementary excitations is discovered.\n\nThe most recent studies of this thesis are devoted to stationary, but rotationally asymmetric vortex states. In weakly interacting condensates, a novel stationary state, a vortex tripole holding finite angular momentum is presented. Also the lowest elementary excitations of the so-called vortex dipole, tripole, and quadrupole states are studied.
In this review, we give an overview of the experimental and theoretical advances in the physics of quantized vortices in dilute atomic-gas Bose--Einstein condensates in a trapping potential, especially focusing on experimental research activities and their theoretical interpretations. Making good use of the atom optical technique, the experiments have revealed many novel structural and dynamic properties of quantized vortices by directly visualizing vortex cores from an image of the density profiles. These results lead to a deep understanding of superfluid hydrodynamics of such systems. Typically, vortices are stabilized by a rotating potential created by a laser beam, magnetic field, and thermal gas. Finite size effects and inhomogeneity of the system, originating from the confinement by the trapping potential, yield unique vortex dynamics coupled with the collective excitations of the condensate. Measuring the frequencies of the collective modes is an accurate tool for clarifying the character of the vortex state. The topics included in this review are the mechanism of vortex formation, equilibrium properties, and dynamics of a single vortex and those of a vortex lattice in a rapidly rotating condensate.
Angular momentum plays a central role in quantum mechanics, recurring in every length scale from the microscopic interactions of light and matter to the macroscopic behavior of superfluids. Vortex beams, carrying intrinsic orbital angular momentum (OAM), are now regularly generated with elementary particles such as photons and electrons. Thus far, the creation of a vortex beam of a nonelementary particle has never been demonstrated experimentally. We present vortex beams of atoms and molecules, formed by diffracting supersonic beams of helium atoms and dimers off transmission gratings. This method is general and could be applied to most atomic and molecular gases. Our results may open new frontiers in atomic physics, using the additional degree of freedom of OAM to probe collisions and alter fundamental interactions.