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Physical Review A

Scattering of an evanescent light field by a single cesium atom near a nanofiber

Fam Le Kien, V. I. Balykin, K. Hakuta

Published Jan 27, 2006• 67 citations
Publisher

Abstract

We investigate the scattering of an evanescent light field by a single cesium atom outside a nanofiber. We show that the confinement of the field, the presence of the longitudinal field component and the tangential Poynting vector component, the enhancement of spontaneous emission, and the degeneracy of the atomic ground state substantially affect the scattering process. We find that, in the close vicinity of the fiber surface, the transmittance of the field in the stationary regime can be substantially reduced to 48% due to scattering into radiation modes (with the efficiency as high as 44%) and backward guided modes (with the efficiency as high as 8%).

DOI
10.1103/physreva.73.013819

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Physical Review A•Sep 21, 2006•21 citations
We investigate the scattering of an evanescent light field by a single cesium atom outside a nanofiber. We show that the confinement of the field, the presence of the longitudinal field component and the tangential Poynting vector component, the enhancement of spontaneous emission, and the degeneracy of the atomic ground state substantially affect the scattering process. We find that, in the close vicinity of the fiber surface, the transmittance of the field in the stationary regime can be substantially reduced to 48% due to scattering into radiation modes (with the efficiency as high as 44%) and backward guided modes (with the efficiency as high as 8%).
We study the spontaneous emission of a cesium atom in the vicinity of a subwavelength-diameter fiber. We show that the confinement of the guided modes and the degeneracy of the excited and ground states substantially affect the spontaneous emission process. We demonstrate that different magnetic sublevels have different decay rates. When the fiber radius is about 200nm200\phantom{\rule{0.3em}{0ex}}\mathrm{nm}200nm, a significant fraction (up to 28%) of spontaneous emission by the atom can be channeled into guided modes. Our results may find applications for developing nanoprobes for atoms and efficient couplers for subwavelength-diameter fibers.
We study the scattering of guided light from a multilevel cesium atom with the transitions between the hyperfine levels 6S1/2F=46{S}_{1/2}F=46S1/2​F=4 and $6{P}_{3/2}{F}^{\ensuremath{'}}=5$ of the D2{D}_{2}D2​ line into the guided modes of a nanofiber. We show that the rate of scattering of guided light from the atom in the steady-state regime into the guided modes is asymmetric with respect to the forward and backward directions and depends on the polarization of the probe field. The asymmetry between the forward and backward scattering is a result of the complex transition structure of the atom and the existence of a longitudinal component of the guided-mode profile function. In the case of a two-level atom, the rates of spontaneous emission (and consequently the rates of scattering) into the forward and backward guided modes differ from each other when the atomic dipole matrix-element vector is a complex vector in the plane that contains the fiber axis and the atomic position.
In this thesis, I present the realization of a fiber-optical interface using optically trapped cesium atoms, which is an efficient tool for coupling light and atoms. The basic principle of the presented scheme relies on the trapping of neutral cesium atoms in a two-color evanescent field surrounding a nanofiber. The strong confinement of the fiber guided light, which also protrudes outside the nanofiber, provides strong confinement of the atoms as well as efficient coupling to near-resonant light propagating through the fiber. In chapter 1, the necessary physical and mathematical background describing the propagation of light in an optical fiber is presented. The exact solution of Maxwell’s equations allows us to model fiber-guided light fields which give rise to the trapping potentials and the atom-light coupling in the close vicinity of a nanofiber. Chapter 2 gives the theoretical background of light-atom interaction. A quantum mechanical model of the light-induced shifts of the relevant atomic levels is reviewed, which allows us to quantify the perturbation of the atomic states due to the presence of the trapping light-fields. The experimental realization of the fiber-based atom trap is the focus of chapter 3. Here, I analyze the properties of the fiber-based trap in terms of the confinement of the atoms and the impact of several heating mechanisms. Furthermore, I demonstrate the transportation of the trapped atoms, as a first step towards a deterministic delivery of individual atoms. In chapter 4, I present the successful interfacing of the trapped atomic ensemble and fiber-guided light. Three different approaches are discussed, i.e., those involving the measurement of either near-resonant scattering in absorption or the emission into the guided mode of the nanofiber. In the analysis of the spectroscopic properties of the trapped ensemble we find good agreement with the prediction of theoretical model discussed in chapter 2. In addition, I introduce a non-destructive scheme for the interrogation of the atoms states, which is sensitive to phase shifts of far-detuned fiber-guided light interacting with the trapped atoms. The inherent birefringence in our system, induced by the atoms, changes the state of polarization of the probe light and can be thus detected via a Stokes vector measurement.
We study the propagation of nanofiber-guided light through an array of atomic cesium, taking into account the transitions between the hyperfine levels 6S1/2F=46{S}_{1/2}F=46S1/2​F=4 and $6{P}_{3/2}{F}^{\ensuremath{'}}=5$ of the D2{D}_{2}D2​ line. We derive the coupled-mode propagation equation, the input-output equation, the scattering matrix, the transfer matrix, and the reflection and transmission coefficients for the guided field in the linear, quasistationary, weak-excitation regime. We show that, when the initial distribution of populations of atomic ground-state sublevels is independent of the magnetic quantum number, the quasilinear polarizations along the principal axes xxx and yyy, which are parallel and perpendicular, respectively, to the radial direction of the atomic position, are not coupled to each other in the linear coherent scattering process. When the guided probe field is quasilinearly polarized along the major principal axis xxx, forward and backward scattering have different characteristics. We find that, when the array period is far from the Bragg resonance, the backward scattering is weak. Under the Bragg resonance, most of the guided probe light can be reflected back in a broad region of field detunings even though there is an irreversible decay channel into radiation modes. When the atom number is large enough, two different band gaps may be formed, whose properties depend on the polarization of the guided probe field.