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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Stimulated Raman Scattering And Four-Wave Mixing: Steady-State Plane-Wave Analytic Solutions

Jay R. Ackerhalt

Published Dec 30, 1981• 1 citation
Publisher

Abstract

The equations for plane-wave steady-state propagation of n fields interacting via four wave processes in a Raman medium have been known since at least 1962. Complete analytic solutions have only been found for the process of harmonic generation. However, solutions have been obtained in the gain regime assuming zero pump depletion. Assuming all fields satisfy the phase matching condition we have found general analytic solutions to these equations. The solutions are complete in that they describe both pump deletion and saturation. Some example problems will be studied.

DOI
10.1117/12.932058

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The equations for plane-wave steady-state propagation of n fields interacting via four wave processes in a Raman medium have been known since at least 1962. Complete analytic solutions have only been found for the process of harmonic generation. However, solutions have been obtained in the gain regime assuming zero pump depletion. Assuming all fields satisfy the phase matching condition we have found general analytic solutions to these equations. The solutions are complete in that they describe both pump deletion and saturation. Some example problems will be studied.
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Parametric instability induced by the medium saturation in stimulated Raman scattering is investigated theoretically via a generalized detuning (1) where ω p,s,o are the frequency of the pump, Stokes, and phonon, ϕ ˙ p s is the phase modulation, and the last term is the nonlinear correction of the highly excited anharmonic molecule with an amplitude Q.The steady-state gain and hence the Stokes efficiency, in the presence of the anharmonic term, are governed by a cubic equation of |Q|2which is to be solved from the Bloch and Maxwell equations including the pump depletion. Numerical results are shown for the transition diagram of Stokes efficiency vs input pump intensity at various system conditions at the steady-state. For the transient regime, with pulse duration shorter than the dephasing time, we analyze the temporal profiles of the Stokes and the depleted pump based on a transformed equation which combines Bloch and Maxwell equation as follows: (2) where Tis a nonlinear time, G s is the steady-state gain, l0is the input pump intensity, and Uis the real part of the phonon amplitude Q.For an input pulse intensity given by sech2(t/t p ), Eq. (2) is solved numerically to study the transient pulse profiles in the presence of pump depletion and medium saturation.
We treat theoretically the two-pulse plane-wave propagation problem associated with the stimulated Raman process. A strong pump pulse and a weak probe pulse interact self-consistently during mutual propagation through a medium in the three-level lambda configuration. We treat the pulse interaction fully coherently, but take initially incoherent mixed ground states to describe the medium. We present analytic pulse envelope solutions to the nonlinear evolution equations, and then test them numerically. We show that the entire process can be interpreted consistently as a three-regime evolution, in which the first and last regimes display behavior quantitatively the same as self-induced transparency. They are connected through a Raman transfer process in the intermediate regime.
The problem with generating of new frequencies (signal and idler waves) in parametric four-photon processes without including the Raman scatter was solved only in approximation for a constant electric field or a constant intensity of the pump wave. The overall task which includes the change in intensity and the phase of the pump wave has not been studied in detail in the literature up to now. The main idea of present work is to solve the more general problem in which we have energy exchange between pump wave, signal and idler waves.