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Plasmonics

Intrinsic Quantum Beats of Atomic Populations and Their Nanoscale Realization Through Resonant Plasmonic Antenna

Ying Gu, Luojia Wang, Pan Ren, Junxiang Zhang, Tiancai Zhang, Jingping Xu, Shi‐Yao Zhu, Qihuang Gong

Published Aug 12, 2011• 16 citations
Publisher
DOI
10.1007/s11468-011-9272-x

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Reducing a nonlinear photon pair source to the nanoscale entails drastic reduction in efficiency and thus requires better tools for its evaluation and optimization. In this context, we develop a formalism for the investigation of spontaneous parametric downconversion in hybrid plasmonic structures that combine plasmonic resonances and intrinsic nonlinearity of a nonlinear medium. Combining quantum and numerical approaches, we quantitatively evaluate photon pair correlation for a realistic experimental configuration. We thereby show that hybrid structures embedding a nanocrystal and plasmonic antennas allow for a 10 5 -fold increase in pair production rate in comparison with a single nanocrystal, thus displaying an efficiency close to the best nanoscale sources to date.
Surface plasmons with ultrasmall optical mode volume and strong near field enhancement can be used to realize nanoscale light-matter interaction. Combining surface plasmons with the quantum system provides the possibility of nanoscale realization of important quantum optical phenomena, including the electromagnetically induced transparency (EIT), which has many applications in nonlinear quantum optics and quantum information processing. Here, using a custom-designed resonant plasmon nanocavity, we demonstrate polarized position-dependent linewidth-controllable EIT spectra at the nanoscale. We analytically obtain the double coherent population trapping conditions in a double-Λ quantum system with crossing damping, which give two transparent points in the EIT spectra. The linewidths of the three peaks are extremely sensitive to the level spacing of the excited states, the Rabi frequencies and detunings of pump fields, and the Purcell factors. In particular the linewidth of the central peak is exceptionally narrow. The hybrid system may have potential applications in ultra-compact plasmon-quantum devices.