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Physical Review A

Photon statistics of a bistable absorber

R. Bonifacio, M. Gronchi, L. A. Lugiato

Published Nov 1, 1978• 115 citations
Publisher

Abstract

We discuss the quantum-statistical properties of a system of absorbing atoms in a ring cavity under the action of a resonant classical field. At a semiclassical level, this system exhibits a bistable behavior in the sense that the transmitted light ${E}_{T}$ is a discontinuous function of the incident light ${E}_{I}$ with a hysteresis cycle, which resembles a first-order phase transition. Here we specify this analogy stressing the nonthermodynamic properties of this coherently driven system. The quantized field ${E}_{T}$ is described by a Glauber $P$ function, which obeys to a Fokker-Planck equation. This equation is derived from a very general master equation in the case of a good quality cavity by neglecting derivatives of order higher than second. A remarkable feature of this equation is that the diffusion coefficient is a nonlinear function of the field intensity. The steady-state solution of the Fokker-Planck equation has the following features. The $P$ function can be single or double peaked according to the value of ${E}_{I}$. In fact, our Fokker-Planck equation is like the one of a Brownian particle moving in a potential which presents one minimum or minima separated by a barrier, depending on the value of ${E}_{I}$. The peaks of the $P$ function correspond to the minima of the potential. In the double-peaked case, the peaks have different widths. The maxima of the $p$ function occur at values of ${E}_{T}$, which coincide with the classical stationary solutions that are stable according to the linear stability analysis. These semiclassical solutions give a discontinuous two-valued function of ${E}_{T}$ vs ${E}_{I}$ (hysteresis cycle). On the contrary, the mean value $〈{E}_{T}〉$ is a continuous single-valued function of ${E}_{I}$, which behaves similarly to the Maxwell construction of a first-order phase transition: $〈{E}_{T}〉$ jumps from low to high values in a very sharp transition region of ${E}_{I}$, which lies between the discontinuity points of the hysteresis cycle. However, the Maxwell rule that we obtain is quite different from that of equilibrium thermodynamics. The mean-square fluctuations of ${E}_{T}$ are always very small except in the transition region where they are quite remarkable. We also present an exact expression of the stationary $P$ function, which takes into account all higher-order derivatives, and we show that the Fokker-Planck approximation is very good for calculating mean values and mean-square fluctuations. Finally, we discuss the connections which link bistable absorption to the laser with injected signal and to the laser with a saturable absorber.

DOI
10.1103/physreva.18.2266

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We discuss the quantum-statistical properties of a system of absorbing atoms in a ring cavity under the action of a resonant classical field. At a semiclassical level, this system exhibits a bistable behavior in the sense that the transmitted light ET{E}_{T}ET​ is a discontinuous function of the incident light EI{E}_{I}EI​ with a hysteresis cycle, which resembles a first-order phase transition. Here we specify this analogy stressing the nonthermodynamic properties of this coherently driven system. The quantized field ET{E}_{T}ET​ is described by a Glauber PPP function, which obeys to a Fokker-Planck equation. This equation is derived from a very general master equation in the case of a good quality cavity by neglecting derivatives of order higher than second. A remarkable feature of this equation is that the diffusion coefficient is a nonlinear function of the field intensity. The steady-state solution of the Fokker-Planck equation has the following features. The PPP function can be single or double peaked according to the value of EI{E}_{I}EI​. In fact, our Fokker-Planck equation is like the one of a Brownian particle moving in a potential which presents one minimum or minima separated by a barrier, depending on the value of EI{E}_{I}EI​. The peaks of the PPP function correspond to the minima of the potential. In the double-peaked case, the peaks have different widths. The maxima of the ppp function occur at values of ET{E}_{T}ET​, which coincide with the classical stationary solutions that are stable according to the linear stability analysis. These semiclassical solutions give a discontinuous two-valued function of ET{E}_{T}ET​ vs EI{E}_{I}EI​ (hysteresis cycle). On the contrary, the mean value 〈ET〉〈{E}_{T}〉〈ET​〉 is a continuous single-valued function of EI{E}_{I}EI​, which behaves similarly to the Maxwell construction of a first-order phase transition: 〈ET〉〈{E}_{T}〉〈ET​〉 jumps from low to high values in a very sharp transition region of EI{E}_{I}EI​, which lies between the discontinuity points of the hysteresis cycle. However, the Maxwell rule that we obtain is quite different from that of equilibrium thermodynamics. The mean-square fluctuations of ET{E}_{T}ET​ are always very small except in the transition region where they are quite remarkable. We also present an exact expression of the stationary PPP function, which takes into account all higher-order derivatives, and we show that the Fokker-Planck approximation is very good for calculating mean values and mean-square fluctuations. Finally, we discuss the connections which link bistable absorption to the laser with injected signal and to the laser with a saturable absorber.
We study the properties of the laser field in the case where the cavity contains two cells, one which amplifies and one which absorbs the radiation. We adopt the simplest possible model, in which there is only one running mode in the cavity and all atoms are fixed and homogeneously distributed in space. We first set up a semiclassical description. In the frame of the stationary semiclassical (SC) theory the most striking feature is the occurrence of a domain in which three solutions coexist. A linear-stability analysis shows that two of these solutions are stable. This gives rise to an hysteresis cycle. Most of the results in this section are analytic. In the frame of a purely quantum description, we derive a generalized Fokker-Planck equation which is exactly solved in the stationary case. This yields a stationary quasiprobability distribution function for the field. In the domain where the SC theory predicts three solutions, the field-distribution function has two maxima and one minimum whose positions are precisely given by the SC intensities. With this distribution function we study the intensity and the intensity fluctuations: the intensity shows a rather abrupt increase when crossing the narrow transition region; in this region the intensity fluctuations are extremely high. By means of an approximate method to solve the time-dependent Fokker-Planck equation we study the linewidth and show that it drastically decreases above threshold. Finally we consider the linearized and quasilinearized Fokker-Planck equations which can be solved analytically. We show that the domain in which neither of these equations fits the results of the generalized Fokker-Planck equation is extremely small. The properties of the metastable states are analyzed in terms of the generalized and asymptotic Fokker-Planck equations.
A quantum treatment of a coherently driven dispersive cavity is given based on a cubic nonlinearity in the polarisability of the internal medium. This system displays bistability and hysteresis in the semiclassical solutions. Quantum fluctuations are included via a Fokker-Planck equation in a generalised P representation. The transmitted light shows a transition from a single-peaked spectrum to a double-peaked spectrum above the threshold of the lower branch. Fluctuations in the field are reduced on the upper branch and both photon bunching and photon antibunching are predicted, for different operating points. An exact solution obtained for the steady-state generalised P function shows decidedly non-equilibrium behaviour, e.g. the lack of a Maxwell construction.
The topic of this thesis is a theoretical study of nonequilibrium transitions and quantum statistical properties of nonlinear quantum optical systems driven by an external radiation source. In certain limiting cases, a comparison is made between these transitions and the phase transitions found in equilibrium physical systems. In chapters one and two, the mathematical tools are introduced. In operator terms, the time development is described by a Markovian master equation in the interaction picture. This is equivalent to a corresponding time development equation or Fokker-Planck equation in a vector space of c-numbers. In order to deal with the type of Fokker-Planck equation that results, we introduce a quantum classical correspondence resulting in a distribution function over a complex phase-space, which is a generalisation of the Glauber-Sudarshan P-function. In chapter three this is applied to a model of a coherently driven mode with nonlinear dispersion and absorption. We find in the limit of zero temperature, that the spectrum is symmetric relative to the input frequency, and an exact solution is obtained for the distribution function. For a detuned driving field and nonlinear dispersion, optical bistability can occur. In chapter four a model of sub/second harmonic generation is introduced. This has several non-equilibrium transitions, including dispersive optical bistability, and bistable behaviour with coherent phase-locked input to both modes. Exact solutions occur in the limit of zero temperature and adiabatic elimination of one mode. In both chapters three and four, steady-state photon anti-bunching occurs with an absorptive nonlinearity. In chapter five we include interactions between the radiation mode and a fluorescent atomic system. In this case different behaviour occurs depending on the relative decay rates of the individual atoms and of the radiation mode. In the case of a high-Q interferometer, the atomic variables can be adiabatically eliminated. Both dispersive and absorptive bistability can occur. We show by analytic and numerical calculations (in the case of inhomogeneous broadening) that dispersive operation has advantages in requiring a lower atomic density and input field to observe bistability. When the input field has Gaussian (rather than coherent) photon statistics, there is no bistability, but enhanced photon bunching occurs. Finally, there is a different type of behaviour when the field mode decays rapidly and can be adiabatically eliminated. Within the cooperation lifetime the system can be described by a J²-invariant Hamiltonian, giving the special case of only collective damping. The result is a new type of critical point transition in the thermodynamic limit, with the appearance of a family of solutions like Lotka-Volterra cycles for a coherent driving field above threshold.
We give a microscopic description of the optical bistability, where the transmission coefficient has two different values as a function of input light intensity, and the system exhibits a discontinuous jump with a hysteresis loop. We developed an efficient numerical algorithm to treat the quantum master equation for hybridized systems of many photons and a large number of two-level atoms. By using this method, we characterize the bistability from the viewpoint of eigenmodes and eigenvalues of the time-evolution operator of the quantum master equation. We classify types of optical bistability according to the photon number density in the cavity. In contrast to previous studies of optical bistability in the high-photon-density regime where the photons can be treated as a classical electromagnetic field and the resonance spectrum has a single-peak structure, we study the nature of optical bistability in the low-photon-density regime where the hybridization of photon and atom degrees of freedom occurs and the resonance spectrum has a double-peak structure. Unraveling the nature of the optical bistability in the latter regime may be important for the manipulation of quantum systems. Concretely, we discuss the steady-state properties of the optical bistability: dependencies of the photon number density on the intensity and the double-peak structure of the photon number distribution inside the bistable region. As for the dynamical properties, we find that the relaxation timescale shows an exponential growth with the system size and reveal how the hysteresis loop of the optical bistability depends on the size of the system and the sweeping rate of the driving amplitude. Finally, by investigating the effects of detuning frequency of the input field, we clarify the characteristic properties of the present optical bistability within the low-photon-density regime, which are qualitatively different from the standard optical bistable phenomena.
A bistable absorber in the good-cavity limit and the Fokker-Planck equation describing the time evolution of the quasi-probability distribution for the transmitted field amplitude are considered. It is shown that the system evolves in two stages. The first consists of a local relaxation around the minimum (or minima) of a suitably defined potential. The second stage, which occurs over a much longer time scale, results from tunneling from one minimum to the other across the local maximum of the same potential. In this paper, only the first stage is analyzed. The time evolution of the expectation value of the transmitted field is described analytically. The accuracy of this approach is tested by numerical solutions of the Fokker-Planck equation.
We discuss a mean-field quantum-mechanical model which describes the dynamics of a homogeneously broadened system of two-level atoms contained in a pencil-shaped resonant cavity and driven by a coherent resonant field EI{E}_{I}EI​. The model is treated in the semiclassical approximation. The model is justified on the basis of Maxwell-Bloch equations with two coherently coupled directions of propagation, with boundary conditions for the fields taken into account. Above a suitable critical density of atoms the system exhibits a bistable behavior including both the stationary situation and the transient, both the light transmitted in the forward direction and the fluorescent light. Bistability is shown to be a consequence of atomic cooperation. We give a simple description of optical bistability leading to new predictions for the transient behavior of the transmitted light and for the spectrum of the fluorescent light. The damping constant which characterizes the rate of appraoch to the stationary situation exhibits a hysteresis cycle. In the low-transmission regime the approach is monotonic, whereas in the highly transmitting situation the approach is oscillatory. One finds a critical slowing down in correspondence with the values EI(+){{E}_{I}}^{(+)}EI​(+), ${{E}_{I}}^{(\ensuremath{-})}$ of the incident field where the transmitted field (as well as the total fluorescence intensity, the rate of approach to the stationary state, etc.) changes discontinuously. On the basis of the regression hypothesis we give a qualitative description of the spectrum of the fluorescent light. This is shown to undergo hysteresis and discontinuous changes at the same values EI(+){E}_{I}^{(+)}EI(+)​, ${E}_{I}^{(\ensuremath{-})}$ of the incident field. Below the critical density of atoms one recovers the usual picture of resonance fluorescence, with a continuous transition from a single-line spectrum to a three-peaked structure when the Rabi frequency becomes equal to the natural linewidth. Above the critical density the triplet appears only when the Rabi frequency becomes equal to the cooperative linewidth of pure super-fluorescence (i.e., for EI=EI(+){E}_{I}={E}_{I}^{(+)}EI​=EI(+)​). Moreover, it appears discontinuously: when EI{E}_{I}EI​ crosses the value EI(+){E}_{I}^{(+)}EI(+)​ the spectrum changes from a single narrow line to a triplet with well-separated sidebands.