Theory of coherent, degenerate two-photon absorption and emission

Oded Kafri, Sol Kimel

NILOY KUMAR DUTTA

Vinay Shukla, Ayan Ray

Abstract In this work, we report experimental studies on coherence in a medium exhibiting DROP (Double Resonance Optical Pumping)-FWM (Four Wave Mixing). Here 5S1/2(F) → 5P3/2(F/) → 5D (F//) two photon transition of hot 87Rb atoms is used. The 5S→5P connection is modified by introducing an additional beam phase coupled to the original beam linking F = 2 → F/ transition. The frequency of the additional beam is offset from that of the original beam by ≈ +10Γ (Γ is natural linewidth). Such a two-beam configuration in F→F/ manifold effectively satisfies conditions of Vee (V) linkage or degenerate two-level connection (DTLC), depending on the detuning of the 780nm laser. This transformation profoundly affects the behavior of the ensuing Ladder (Ξ) system. While the (I) Ξ +V condition is favorable for Electromagnetically Induced Transparency (EIT), the (ii) Ξ + DTLC brings in the effect of Electromagnetically Induced Absorption (EIA). The EIT-dominated situation is helpful for FWM to take place, and the EIA effect augments the stronger presence of DROP. This condition is verified by monitoring the blue fluorescence emanating from the 5D→6P3/2→5S1/2 decay route. The DROP effect follows the Amplified Spontaneous Emission (ASE) pattern in the media. The origin of blue photons is also due to FWM under EIT conditions. In the case of EIA, the dominant condition increment in blue fluorescence is due to increased stimulated emission. The blue photons mainly contributed by (i) FWM and (ii) increased participation of stimulated emission are directional in nature and phase coherent.

Qingqing Sun, Ying Gu, Qihuang Gong

We investigate the quantum coherence effects of a closed transition F e = 1 ↔ F g = 0 driven by transverse linearly polarized light field (with [sgrave] ± components) and probed by another transverse, linearly polarized light field. Owing to the competition of two-photon gain and single-photon absorption, the absorption spectrum is shown as a combination of electromagnetically induced transparency (EIT) and Mollow absorption spectrum (MAS). In the degenerate case, the MAS covers the EIT window at the pump-probe detuning centre. In the magnetic field, two single-photon absorption peaks inside the EIT windows appear when the drive Rabi frequency is smaller than the Zeeman splitting while, when the Rabi frequency is larger than the Zeeman splitting, we find four emission peaks due to the two-photon gain. A transition from positive to negative dispersion is obtained, which means a shift between the subluminal and superluminal group velocities.

清 西川, 昭 佐道, Hiroshi Sekiya +3 more

Chana Goren, A. D. Wilson‐Gordon, M. Rosenbluh +1 more

The paper discusses on EIA, or the electromagnetically induced absorption, as a consequence of transfer of coherence (TOC) by spontaneous emission between the excited and ground degenerate states. The paper also explains a different mechanism, the transfer of population (TOP) or optical pumping, which can also lead to EIA peaks in the absorption spectrum of a degenerate two-level system.