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Physical review. B, Condensed matter

Theory of phase conjugation of light in disordered nonlinear media

V. E. Kravtsov, Vladimir I. Yudson, V. M. Agranovich

Published Feb 15, 1990• 37 citations
Publisher

Abstract

In the case of disordered nonlinear media, it is shown that in four-wave mixing a phenomena analogous to phase conjugation may occur. In contrast to the case of transparent media in which two counterpropagating pump waves (with frequency ${\ensuremath{\omega}}_{p}$) are required, phase conjugation may occur in the presence of a single pump wave injected into the disordered nonlinear material. We find that in the angular distribution of radiation of frequency ${\ensuremath{\omega}}_{s}$ (${\ensuremath{\omega}}_{s}$=2${\ensuremath{\omega}}_{p}$-${\ensuremath{\omega}}_{i}$, where ${\ensuremath{\omega}}_{i}$ is the frequency of probe wave) there is a narrow peak in the backscattered direction associated with the probe wave. The intensity of this peak may be some orders of magnitude larger than the diffuse background at the frequency ${\ensuremath{\omega}}_{s}$.

DOI
10.1103/physrevb.41.2794

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In the case of disordered nonlinear media, it is shown that in four-wave mixing a phenomena analogous to phase conjugation may occur. In contrast to the case of transparent media in which two counterpropagating pump waves (with frequency \ensuremathωp{\ensuremath{\omega}}_{p}\ensuremathωp​) are required, phase conjugation may occur in the presence of a single pump wave injected into the disordered nonlinear material. We find that in the angular distribution of radiation of frequency \ensuremathωs{\ensuremath{\omega}}_{s}\ensuremathωs​ (\ensuremathωs{\ensuremath{\omega}}_{s}\ensuremathωs​=2\ensuremathωp{\ensuremath{\omega}}_{p}\ensuremathωp​-\ensuremathωi{\ensuremath{\omega}}_{i}\ensuremathωi​, where \ensuremathωi{\ensuremath{\omega}}_{i}\ensuremathωi​ is the frequency of probe wave) there is a narrow peak in the backscattered direction associated with the probe wave. The intensity of this peak may be some orders of magnitude larger than the diffuse background at the frequency \ensuremathωs{\ensuremath{\omega}}_{s}\ensuremathωs​.
Recently it was shown that in disordered media, nonlinear backscattering of phase-conjugated signal light is possible in the presence of only a single pump wave, in contrast to the case of an ordered medium where two counterpropagating pump waves are necessary. Formally, this disorder-induced nonlinear process corresponds to the cooperon-channel (back)scattering of the signal wave in the presence of diffusion propagation of the pump wave. (The cooperon is the Cooper particle-particle diffusion propagator.) In this contribution, the question is considered whether the disorder-induced backscattering of phase-conjugated light can restore the disturbed signal wave front as it does in the ordered case. Examining correlations of the outgoing waves corresponding to different incoming signal waves, it is shown that the backscattered waves possess a ``phase memory'' even for a large difference of the angles of incidence of incoming waves. This is in contrast to the case of linear backscattering, where such correlations take place only at a very small difference of the angles of incidence (of the order of backscattering peak width). Thus the phase conjugation in disordered media does possess the peculiar coherent properties of that in ordered media.
We have developed a theory for nondegenerate oscillations in optical resonators containing an intracavity phase-conjugate element. The phase-conjugate element consists of a nonlinear transparent medium that is pumped externally by a pair of counterpropagating laser beams of the same frequency and intensity. Phase conjugation of an input beam of slightly different frequency occurs because of nondegenerate four-wave mixing. The theory takes into account linear absorption (or gain) in the medium and is applied to study the threshold behavior of phase-conjugate oscillators. For the special case of no conventional mirrors, the phase-conjugate oscillator reduces to an ordinary phase-conjugate mirror, and our general formulation yields the results of previous studies. Our analysis shows that the parametric gain required for oscillation increases (or decreases) as a result of linear absorption (or gain) in the medium, and oscillation can occur at a frequency different from that of the pump beams in the presence of large linear gain (or loss). The effects of linear absorption (or gain) on the filter operation are also examined.
Nonlinear optics normally involves the change in the susceptibility of a material due to the presence of optical radiation. In many cases, the light-matter interaction produces a change in the refractive index of the medium, as occurs in photorefractive media, as well as in Kerr-like media, Brillouin-active media and absorbing media with thermallyinduced refractive index changes. Such nonlinear refractive index variation corresponds to a change in the real part of the optical susceptibility %. In resonant materials, the optical radiation induces stimulated emission (or absorption) causing transfer of population between different energy states of the medium. This can lead to saturation of the amplification (or absorption) corresponding to changes in the imaginary part of the susceptibility x= i2odk where the amplitude gain coefficient a(I) is a saturable function of the intensity /, and k is the magnitude of the wavevector of the optical radiation. The interference of two (or more) coherent beams I(x) in the laser amplifier can cause a modulation of the population inversion N(x). This modulation of the inversion is commonly known as spatial hole burning in lasers and leads to formation of a gain-grating a(x) = 1/2GN(X) where G is the stimulated emission cross-section. The gain grating can act as a very efficient diffractive optical element exhibiting high diffraction efficiency that may be even greater than unity [16] and also very high phase conjugate reflectivity using four-wave mixing (FWM) geometries [5-7].
Optical phase conjugation by four-wave mixing in a Kerr medium is considered. Two strong counterpropagating lasers pump a nonlinear medium in which they excite the third-order polarization. Mixing with a weak incident field then generates the phase-conjugated image of that field. It is shown how the polarization of the pumps and the tensorial nature of the nonlinear interaction can be accounted for by a geometrical polarization tensor. The electric field is shown to obey two coupled wave equations, which couple a positive- and negative-frequency component of the field. These wave equations allow plane-wave solutions, and we derive the dispersion relation for the wave vectors of these modes. By matching the field of such a mode across the boundaries of the medium to an external incident field, we are able to obtain analytically the Fresnel coefficients for reflection and transmission. Our expressions reduce to earlier results in the appropriate limits.
We have shown previously that two strong laser beams (with the same frequency) counterpropagating in a Kerr nonlinear medium with linear dispersion become un stable when their intensities exceed a certain threshold.1 We demonstrate here that the system exhibits large (theoretically unlimited) amplification of a probe beam when the two pumping beams have their intensities slightly below the threshold. This is in contrast to the conventional phase conjugation due to four-wave mixing in a nondispersive Kerr nonlinear medium. The mechanism of amplification in our system can be explained in terms of positive distributed feedback from the Kerr nonlinear index grating formed by two strong pumping laser beams in the presence of dispersion giving rise to a light-induced distributed-feedback resonator. This feedback is attributed to the fact that the weak beams with both signal frequency, ω + δ, and conjugate frequency, ω − δ, propagate with phase speed different (due to dispersion) from that of a pumping wave with frequency ω, which triggers the exponentially increasing energy exchange between weak and strong beams at the nonlinear index grating (this energy exchange is prohibited in nondispersive media). When the probe frequency approaches a frequency of one of the longitudinal modes of the light-induced distributed resonator, and the pumping intensity approaches the threshold of instability, the resonant amplification increases infinitely; for presently available laser intensity stabilities, amplification as large as 104 is feasible.
This paper presents an exact solution to the slowly varying envelope equations for the probe and signal fluxes in degenerate four-wave mixing in Kerr media. The analysis is performed for a noncollinear geometry, and all beams have the same linear polarization in the nonlinear medium. It is assumed that the angle separating the directions of the counterpropagating pumps and probe and signal beams is large enough so that cross-coupled waves do not contribute to the envelope equations describing the spatial evolution of the pump, probe, and signal beams. Multiple values of the transmitted probe are obtained for equal pump fluxes above a threshold determined by the nonlinear phase shift in the medium. Significant pump depletion occurs in this regime, but it can also occur without the appearance of multiple solutions. Since exact optical phase conjugation occurs only in the limit where the pumps are undepleted in Kerr media, this result implies that there are fundamental upper limits on the pump intensity that can be used to increase signal reflectivities in optical phase conjugation.