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International Photonics and Optoelectronics Meetings

On-demand semiconductor single-photon source with near-unity indistinguishability

Yuming He, Yu He, Yu-Jia Wei, Dian Wu, Mete Atatüre, Christian Schneider, Sven Höfling, Martin Kamp, Chao‐Yang Lu, Jian-Wei Pan

Published Jan 1, 2012• 42 citations
Publisher

Abstract

We generate pulsed RF single photons on demand from a single, microcavity-embedded quantum dot under s-shell excitation with 3-ps laser pulses. The deterministically pi-pulse excited RF photons have less than 0.3% background contributions and a vanishing two-photon emission probability of 0.012(2). Non-postselective Hong-Ou-Mandel interference between two successively emitted photons is observed with a visibility of 0.970(19). Two single photons are further used to implement a high-fidelity quantum controlled-NOT gate.

DOI
10.1364/iont.2012.if1a.3

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We generate pulsed RF single photons on demand from a single, microcavity-embedded quantum dot under s-shell excitation with 3-ps laser pulses. The deterministically pi-pulse excited RF photons have less than 0.3% background contributions and a vanishing two-photon emission probability of 0.012(2). Non-postselective Hong-Ou-Mandel interference between two successively emitted photons is observed with a visibility of 0.970(19). Two single photons are further used to implement a high-fidelity quantum controlled-NOT gate.
We report on two-photon interference of highly indistinguishable single photons emitted by a quantum dot. Strictly resonant excitation with picosecond laser pulses has been used to prepare coherent states with a significantly increased coherence time $({T}_{2}\ensuremath{\sim}1\text{ns})$ and reduced lifetime $({T}_{1}\ensuremath{\sim}650\text{ps})$, as compared to a nonresonant excitation scheme. Indistinguishable photons, with visibilities greater than 70%, have been observed by measuring the Hong-Ou-Mandel dip without postselection of the interfering photons. Near-unity indistinguishable photons should be achievable by preventing fluctuations in the electrostatic environment in the vicinity of the dots, considered as an important source of decoherence.
Scalable photonic quantum technologies require on-demand single-photon sources with simultaneously high levels of purity, indistinguishability, and efficiency. These key features, however, have only been demonstrated separately in previous experiments. Here, by s-shell pulsed resonant excitation of a Purcell-enhanced quantum dot-micropillar system, we deterministically generate resonance fluorescence single photons which, at π pulse excitation, have an extraction efficiency of 66%, single-photon purity of 99.1%, and photon indistinguishability of 98.5%. Such a single-photon source for the first time combines the features of high efficiency and near-perfect levels of purity and indistinguishabilty, and thus opens the way to multiphoton experiments with semiconductor quantum dots.
Applying continuous-wave pure resonant s-shell optical excitation of individual quantum dots in a high-quality micropillar cavity, we demonstrate the generation of post-selected indistinguishable photons in resonance fluorescence. Close to ideal visibility contrast of 90% is verified by polarization-dependent Hong-Ou-Mandel two-photon interference measurements. Furthermore, a strictly resonant continuous-wave excitation together with controlling the spontaneous emission lifetime of the single quantum dots via tunable emitter-mode coupling (Purcell) is proven as a versatile scheme to generate close to Fourier transform-limited (T2/(2T1)=0.91) single photons even at 80% of the emission saturation level.
Summary form only given. Single-photon sources have recently been demonstrated using a variety of devices, including molecules, mesoscopic quantum wells, colour centers, trapped ions, and semiconductor quantum dots. These sources rarely emit two or more photons in the same pulse, compared to a Poisson-distributed source of the same intensity. Numerous applications for single-photon sources have been proposed in the field of quantum information. However, most, including linear-optical quantum computation, also require that consecutive photons have identical wave packets. For a source based on a single quantum emitter, the emitter must therefore be excited in a rapid or deterministic way, and interact little with its surrounding environment. Here, we test the indistinguishability of photons emitted by a semiconductor quantum dot in a microcavity through a Hong-Ou-Mandel-type two-photon interference experiment. We find that consecutive photons are largely indistinguishable, with a mean wave-packet overlap as large as 0.81, making this source useful in a variety of experiments in quantum optics and quantum information.
A single-photon source capable of emitting indistinguishable photons is a key element in schemes for scalable quantum information processing with linear optics. Whilst several groups have reported such sources, up until now an electrically driven source capable of making these protocols technologically viable has yet to be reported. We present the first demonstration of an electrically driven single-photon source emitting indistinguishable photons. Our sample consists of a layer of InAs/GaAs quantum dots embedded in the intrinsic region of a p-i-n microcavity diode. We test the indistinguishability of consecutive photons by carrying out a Hong-Ou- Mandel-type two-photon interference experiment whereby two identical photons arriving simultaneously at two input ports of a 50:50 beamsplitter exit together. The device was operated under two modes, continuous and pulsed current injection. In the former case, we measured a coherence time of up to 400 ps at low pump current - the longest reported under these excitation conditions. A two-photon interference visibility was measured, limited only by the timing resolution of our detection system and further suggesting a 100% overlap of photon wavepackets at the output beamsplitter. In the case of pulsed injection, we employed a two-pulse voltage sequence which allowed us to carry out temporal filtering of photons which had undergone dephasing. The characteristic Hong-Ou-Mandel "dip" was measured resulting in a visibility of 64 ± 4%.