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The European Physical Journal D

Differential measurement of the ultracold Cs radiative escape and fine structure changing collision rates

James P. Shaffer, Witek Chalupczak, N. P. Bigelow

Published Jan 1, 1999• 7 citations
Publisher
DOI
10.1007/s100530050575

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We describe a comprehensive investigation of trap loss in a two-species Na-Cs magneto-optical trap. Observed losses, due to the interspecies interactions, are attributed to collisions in which a change in the fine-structure state of the Na partner causes the escape of atoms from the trap. Results are described in terms of the heteronuclear pair potentials and the interaction of the colliding pairs with the radiatively active environment.

Physical Review A•Nov 1, 1999•39 citations
Summary form only given. In a magneto-optical trap (MOT) two main mechanisms contribute to the total trap loss rate. Radiative escape (RE), where the spontaneous emission within the collision duration transforms internal energy into kinetic motion. Fine-structure changing collision (FSC) is an exoergic process where a pair of excited ground state atoms undergoes a change to the lower state of the fine-structure doublet, followed by a release of /spl Delta/E/sub FSC//2 in kinetic energy normally enough to eject the atoms from the trap. In earlier experiments only the total trap loss rate, which is the sum of contributions from RE and FSC, was determined. Distinguishing between these two mechanisms is important because it allows a more precise comparison with the theory, leading to a better understanding of exoergic cold collisions. In this experiment the FSC contribution to the total loss in /sup 85/Rb is measured by direct photoionization of the P/sub 1/2/ fragments.
Accurate measurements are presented of the rate of trap-loss-producing collisions between ultracold magneto-optically trapped 7Li^{7}\mathrm{Li}7Li atoms for a range of trap laser intensities and frequencies. Intensities from near the atomic saturation intensity to well above it are investigated. At low intensities, fine-structure-changing collisions cause trap loss with a rate constant of \ensuremath{\sim}${10}^{\mathrm{\ensuremath{-}}10}$ cm3{\mathrm{cm}}^{3}cm3/s. At sufficiently high intensity, the trap can be deep enough to effectively freeze out the dominant fine-structure-changing collisions as a loss mechanism, enabling an accurate comparison of the radiative escape loss rate with theory. At the lowest intensities of this radiative escape regime, the measured loss rates compare favorably with those calculated using an optical Bloch equation theory and a three-dimensional model of trap depth. However, the intensity dependence of the measured rates does not show the saturation predicted by the optical Bloch equation theory. It is shown that reliable knowledge of trap depth is necessary to accurately compare experiment with theory.