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Journal of Experimental and Theoretical Physics

Resonant transparency regimes under conditions of long/short-wave coupling

С. В. Сазонов, N. V. Ustinov

Published Feb 1, 2005• 18 citations
Publisher

Abstract

Nonlinear two-component electromagnetic pulse propagation through a resonant axially symmetric anisotropic medium having a permanent dipole moment is analyzed under conditions of strong coupling between the ordinary (short-wavelength) and extraordinary (long-wavelength) pulse components. It is shown that a pulse can propagate through the medium in regimes different from self-induced transparency if its ordinary component is detuned off resonance. In particular, a pulse propagating in the regime of self-induced super-transparency substantially changes quantum-level populations, but its group velocity remains almost equal to the linear velocity. If a pulse propagates in the extraordinary transparency regime and the carrier-frequency detuning from resonance is small, then its group velocity is substantially lower, while the level populations remain virtually invariant. Regimes of propagation through weakly excited media under quasi-resonance conditions are also identified.

DOI
10.1134/1.1884667

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Conference on Lasers and Electro-Optics•Aug 29, 2005•2 citations
Nonlinear two-component electromagnetic pulse propagation through a resonant axially symmetric anisotropic medium having a permanent dipole moment is analyzed under conditions of strong coupling between the ordinary (short-wavelength) and extraordinary (long-wavelength) pulse components. It is shown that a pulse can propagate through the medium in regimes different from self-induced transparency if its ordinary component is detuned off resonance. In particular, a pulse propagating in the regime of self-induced super-transparency substantially changes quantum-level populations, but its group velocity remains almost equal to the linear velocity. If a pulse propagates in the extraordinary transparency regime and the carrier-frequency detuning from resonance is small, then its group velocity is substantially lower, while the level populations remain virtually invariant. Regimes of propagation through weakly excited media under quasi-resonance conditions are also identified.
The distinctive features of the propagation of the two-component electromagnetic pulses in an anisotropic media are studied in the frameworks of the system of equations of the resonance of long and short waves. It is shown that an interaction of the light with the quantum systems, which have a constant dipole momentum nonequal to zero, occurs not only in the usual mode of the self-induced transparency, but also in two new modes. In the first one (supertransparency), the pulse propagation causes the significant change of the population density of quantum levels, while its group velocity remains close to linear one. In the second mode (extraordinary transparency), the group velocity of the pulse changes significantly, but the population of the levels is practically invariable. It is also noted that the largest change of the population takes place, if the carrier frequency of the solitons is less than the resonant frequency, at that the detuning value depends on the duration of the pulses.
The propagation of a two-component laser pulse in an optically uniaxial medium is investigated under the conditions of the Zakharov-Benney resonance (viz., resonance of long and short waves). The short-wave ordinary component of the pulse, which is in resonance with the atomic subsystem, effectively generates a video pulse of the extraordinary wave (long-wave component). The latter dynamically detunes the ordinary pulse from the resonance and causes its phase modulation due to nonzero diagonal matrix elements of the dipole moment. An approximate operator approach is proposed for solving constitutive equations for the density matrix, which is equivalent to the asymptotic WKB method and makes it possible to reduce the analysis to solving a system of nonlinear wave equations for both components of the pulse. The possibility an extraordinary wave video pulse being generated with the help of a quasimonochromatic ordinary pulse with a longer wave-length. It is shown that, when the ordinary component dominates, the self-induced transparency mode is realized; in the opposite limit, the effect known as extraordinary transparency takes place. Solitary pulses corresponding to the latter case experience a decrease in the velocity of propagation, which is similar to that observed for self-induced transparency and practically do not change the population of quantum levels. Physical situations reducing the initial system of constituent and wave equations to familiar integrable models are analyzed.
Resonant absorbing media having many atoms within a cubic resonance wavelength can exhibit large frequency chirps in pulse propagation due to dipole-dipole interactions among the atoms. Analytic solutions are obtained for invariant pulse propagation in such a medium consisting of interacting two-level atoms. Departures from the McCall-Hahn results include nonhyperbolic secant pulse shapes and different than 2π-area pulses. In addition, the excitation of the medium is comparatively suppressed for the same group velocity. The results are interpreted to suggest new experiments.
This thesis deals with the study of propagation effects experienced by weak light pulses as they propagate in atomic media driven by strong pulses. We explore both the ultra-short and long pulse regime and investigate the phenomena that arise at these different time scales. In the short pulse regime, a strongly driven two level atomic system presents transient light shifts, and non-adiabatic transitions occur between these adiabatic levels. We have studied a method to probe these light shifts in real time by propagating a weak probe through the medium. The light shifts enrich the spectrum of the probe and the probe gets shaped as a result. In this way a strongly driven two-level system can act as an active pulse shaper, and can introduce oscillations in the temporal profile of an ultra-short pulse at a time scale shorter than the pulse duration. We also show that by driving the system with two time delayed non-resonant strong fields, the non-adiabatic effects can be rendered phase dependent. This gives very sensitive phase control of the excited state population and can be used to formulate new techniques in interferometry. In the long pulse regime we present a new method of slowing light that can be realized in a double two-level system interacting with two orthogonally polarized light pulses that propagate along different axis. Spatio-temporal dependence of the total polarization induces a grating in the ground Zeeman coherence. The stronger of the two fields (the control field) is diffracted from this grating into the direction of the weak probe field compensating for the absorption of this latter field. A transparency window is thus created in the absorption spectrum of the probe leading to the slowing down of light. The transparency window exhibits characteristics similar to the one obtained by EIT (electromagnetic induced transparency) method. However, the important difference between our method and the traditional EIT method, is that ours doesn't rely on realizing dark state in the system. This may open the possibility of slowing down light in more complex atomic media. Moreover, when the linear absorptive response of the medium is cancelled in this manner, the nonlinear response becomes more important. In the situation where fields propagate in the same direction and have same frequency, two regimes have been investigated. For small optical depths, the effective susceptibility behaves as chi_lin exp[2 i phi] (with phi the phase difference between two fields). This renders phase control of the medium response, and the medium can be changed from an absorber to an amplifier, with normal or anomalous dispersion, by adjusting the relative phase phi.  In the regime of large optical thickness, phase saturation takes place and the effective susceptibility turns into chi_lin*, changing an absorber into an amplifier without effecting the dispersive response (chi_lin is linear susceptibility).