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Solid State Communications

Nonequilibrium phase transition in laser-active media

V. Dohm

Published Nov 1, 1972• 38 citations
Publisher
DOI
10.1016/0038-1098(72)90841-1

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We show that a divergence in the optical polarizability of a heterogeneous medium with nonlinear amplification and a strong dipole-dipole interaction between particles can lead to a phase transition, for which the dipole momentum of the particles or the dipole radiation rate can be taken as order parameters. The ``dipole laser'' [Phys. Rev. A 71, 063812 (2005)] can be used both as a simple example of such a second-order phase transition and to provide a recipe for its analysis. We show that similar phase transitions may be possible for a nanoparticle on the surface of an optically active medium and at the ``Clausius-Mossotti'' catastrophe in a bulk heterogeneous medium.
We study the direct laser drive of infrared-active phonons that are quadratically coupled to a spinless fermion chain. Feedback is incorporated by phonon dressing of the electronic dispersion, which enables effective nonlinearities in the phonon dynamics. We uncover a first-order phase transition in the phononic steady state in which hysteretic effects allow either large or small phonon occupation depending on the drive protocol. We discuss the implications of these findings for probing phase transitions in real driven materials.
A crowd of nonequilibrium entities can show phase transition behaviors that are prohibited in conventional equilibrium setups. An interesting question is whether similar activity-driven phase transitions also occur in pure quantum systems. Here we investigate a classical anisotropic lattice gas model that undergoes motility-induced phase separation and extend the model to the quantum regime. The resulting model is a quantum many-body model that undergoes quantum phase transitions induced by non-Hermiticity. The quantum phase diagram includes active phase transitions involving phase separation, microphase separation, and flocking. The quantum phase transitions are identified as the transitions of dynamical paths in the classical kinetics upon the application of biasing fields. Our approach sheds light on the useful connection between classical nonequilibrium kinetics and non-Hermitian quantum physics.