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Physical Review A

Unitary transformation and the dynamics of a three-level atom interacting with two quantized field modes

Moorad Alexanian, Subir K. Bose

Published Sep 1, 1995• 100 citations
Publisher

Abstract

Starting from a three-level atom coupled to two modes of radiation field, we derive a Raman-coupled Hamiltonian by a unitary transformation, evaluated perturbatively in coupling constants. The Rabi oscillation frequency and the collapse and revival times of the atomic coherence are found to have strikingly different photon-intensity dependence than those found previously.

DOI
10.1103/physreva.52.2218

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Starting from a three-level atom coupled to two modes of radiation field, we derive a Raman-coupled Hamiltonian by a unitary transformation, evaluated perturbatively in coupling constants. The Rabi oscillation frequency and the collapse and revival times of the atomic coherence are found to have strikingly different photon-intensity dependence than those found previously.
We present a general procedure to describe the dynamics of N degenerate quantized fields interacting resonantly with a two–level atom, all coupled with the same strength, within the rotating–wave approximation. Starting from the analysis of the two and three field cases, we generalize the method by identifying dynamical invariants that lead to a factorized form of the time–evolution operator. A unitary transformation reduces the problem to an effective Jaynes–Cummings Hamiltonian, where only one field interacts with the atom and the remaining modes contribute as free fields. Assuming initially coherent fields and an atomic superposition, we compute the atomic inversion and the mean photon number, revealing vacuum Rabi oscillations with a frequency determined by an effective coupling constant that exceeds the individual atom–field coupling, as well as the characteristic collapse-revival behavior.
The Hamiltonian is derived for the interaction of a Λ-type three-level atom with a two-mode quantum cavity field from the general interaction Hamiltonian between a multi-level atom and a multi-mode radiation field, and it is reduced to an effective two-mode Raman-coupled model under a large detuning condition. We propose a modified effective Hamiltonian for the two-mode Raman-coupled model, find the time-dependent state vectors, and present the validity conditions for the involved interaction Hamiltonians. It is shown that in the study of the two-mode Raman-coupled model it is not enough to retain only the usually used effective Hamiltonian, one must also take into account the ac Stark shift of the atomic levels (at least one of the levels). Finally, we study the atomic dynamics in the interaction of a Λ-type three-level atom with a two-mode quantum cavity field and in the two-mode Raman-coupled model. We find that the number of collapse-revivals, the collapse time and the revival time show new characteristics.
We study the quantum dynamics of a two-atom Raman coupled model interacting with a quantized bimodal field with intensity-dependent coupling terms in a lossless cavity. The unitary transformation method used to solve the time-dependent problem also gives the eigensolutions of the interaction Hamiltonian. We study the atomic-population dynamics and dynamics of the photon statistics in the two cavity modes, and present evidence of cooperative effects in the production of antibunching and anticorrelations between the modes. We also investigate the effect of detuning on the evolution of second-order correlation functions and observe that the oscillations become more rapid for large detuning.
The dynamics of a degenerate two-mode electromagnetic field coupled to a single two-level atom is investigated both analytically and numerically. New quantum effects are discussed concerning the time dependence of the photon number and of its fluctuations, assuming that at t = 0 one of the modes is coherent and the other is empty. The field dynamics are dominated by oscillatory net exchanges of a large number of photons between the two modes, displaying amplitude decay. Over a longer time scale, revivals and collapses in the field populations take place. The time scales of these phenomena are much larger than those of the atomic Rabi oscillations decay. Moreover, the system attains a highly non-classical regime in which the field intensity in each mode is subjected to strong fluctuations even for a large initial number of photons in the coherent mode. Various correlations between atomic and field dynamics are pointed out, and the physical origin of the new quantum effects is briefly discussed. Finally, using our fully quantized calculations, we comment on the validity of the atomic homodyne detection proposed by Wilkens and Meystre.
In the preceding chapters concerning the interaction of a radiation field with matter, we assumed the field to be classical. In many situations this assumption is valid. There are, however, many instances where a classical field fails to explain experimentally observed results and a quantized description of the field is required. This is, for example, true of spontaneous emission in an atomic system which was described phenomenologically in Chapter 5. For a rigorous treatment of the atomic level decay in free space, we need to consider the interaction of the atom with the vacuum modes of the universe. Even in the simplest system involving the interaction of a single-mode radiation field with a single two-level atom, the predictions for the dynamics of the atom are quite different in the semiclassical theory and the fully quantum theory. In the absence of the decay process, the semiclassical theory predicts Rabi oscillations for the atomic inversion whereas the quantum theory predicts certain collapse and revival phenomena due to the quantum aspects of the field. These interesting quantum field theoretical predictions have been experimentally verified. In this chapter we discuss the interaction of the quantized radiation field with the two-level atomic system described by a Hamiltonian in the dipole and the rotating-wave approximations. For a single-mode field it reduces to a particularly simple form. This is a very interesting Hamiltonian in quantum optics for several reasons. First, it can be solved exactly for arbitrary coupling constants and exhibits some true quantum dynamical effects such as collapse followed by periodic revivals of the atomic inversion.