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Physics Reports

Nonlinear susceptibilities and light scattering on free atoms

A. G. Faǐnshteǐn, Nikolai L. Manakov, Vitalii D Ovsiannikov, Л. П. Рапопорт

Published Jan 1, 1992• 43 citations
Publisher
DOI
10.1016/0370-1573(92)90020-z

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We observe a nonlinear optical process in a gas of cold atoms that simultaneously displays the largest reported fifth-order nonlinear susceptibility χ (5) =1.9 × 10 − 12 (m/V) 4 and high transparency. The nonlinearity results from the simultaneous cooling and crystallization of the gas, and gives rise to efficient Bragg scattering in the form of six-wave mixing at low light levels. For large atom-photon coupling strengths, the back-action of the scattered fields influences the light-matter dynamics. We confirm this interpretation by investigating the nonlinearity for different polarization configurations. In addition, we demonstrate excellent agreement between our experimental measurements and a theoretical model with no free parameters, and compare our results to those obtained using alternative approaches. This system may have important applications in many-body physics, quantum information processing, and multidimensional soliton formation.
The realization of tabletop optical analogue experiments of superfluidity relies on the engineering of suitable optical media, with tailored optical properties. This work shows how quantum atomic optical systems can be used to develop highly tunable optical media, with localized control of both linear and nonlinear susceptibility. Introducing the hydrodynamic description of light, the superfluidity of light in these atomic media is investigated through GPU-enhanced numerical simulations, with the numeric observation of the superfluidic signature of suppressed scattering through a defect.
The realization of tabletop optical analogue experiments of superfluidity relies on the engineering of suitable optical media, with tailored optical properties. This work shows how quantum atomic optical systems can be used to develop highly tunable optical media, with localized control of both linear and nonlinear susceptibility. Introducing the hydrodynamic description of light, the superfluidity of light in these atomic media is investigated through GPU-enhanced numerical simulations, with the numeric observation of the superfluidic signature of suppressed scattering through a defect