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Applied Physics Letters

Toward quantum interference of photons from independent quantum dots

Mohamed Benyoucef, L. Wang, Armando Rastelli, Oliver G. Schmidt

Published Dec 28, 2009• 12 citations
Publisher

Abstract

The authors present steps toward the experimental realization of indistinguishable single photon sources based on independent unstrained GaAs quantum dots (QDs), which are embedded in planar cavities to improve the light collection efficiency. The emission lines of two QDs are brought into resonance and overlapped at a beam splitter. The coherence properties of the emitted photons are investigated by measuring the first-order field correlation function. Despite the fact that the short dephasing time of the selected QDs prevents us to observe quantum interference between the two photons, the approach could be applied to other QDs.

DOI
10.1063/1.3275702

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The authors present steps toward the experimental realization of indistinguishable single photon sources based on independent unstrained GaAs quantum dots (QDs), which are embedded in planar cavities to improve the light collection efficiency. The emission lines of two QDs are brought into resonance and overlapped at a beam splitter. The coherence properties of the emitted photons are investigated by measuring the first-order field correlation function. Despite the fact that the short dephasing time of the selected QDs prevents us to observe quantum interference between the two photons, the approach could be applied to other QDs.
Abstract We report a set of experiments designed to test the quantum indistinguishability of single photons emitted by a resonantly pumped InAs/GaAs quantum dot, embedded in a microcavity. We first performed high resolution interferometric measurements on the source to infer its coherence time. By comparison with the exciton lifetime, obtained by time‐resolved spectroscopy, we found that some quantum dots were emitting almost transform‐limited photons. The measured ratio of the coherence time to the pulse duration gives a lower bound on the dephasing time which agrees well with previous studies. We then directly measured the mean overlap between wave packets of consecutive photons emitted 2 ns apart, through a Hong–Ou–Mandel type two‐photon interference experiment. For the best dot, an overlap as high as 0.81 was inferred. This result suggests that quantum dots could be a practical single photon source to perform quantum information processing experiments. We stress the importance of the microcavity for identical photon generation.
Single photon emission is one of the most striking optical properties of semiconductor quantum dots (QDs), and the corresponding photon anti-bunching effect was observed by non-resonant and resonant photoluminescence experiments in single QDs [1,2,3,4]. Other experiments demonstrated the possibility to use single QDs for the generation of indistinguishable single photons [3]. An important general issue is to reach the so-called fundamental radiative limit. Several strategies have been followed in that sense such as the shortening of population lifetime induced by the Purcell effect [5] or the reduction of pure dephasing by resonant excitation [2,3,4]. Up to now, all the measurements reported in the literature focus on the incoherent photoluminescence signal for achieving single photon emission. In this regime, the linewidth of the photoluminescence spectrum is always limited to the radiative limit. In this paper, we report on the resonant emission (RE) of the exciton in single InAs/GaAs QDs embedded in a planar microcavity, in an orthogonal excitation-detection geometry [4]. We present an original type of single photon source based on the coherent laser light scattering by a single QD [6]. Besides the antibunching effect showing the non-classical nature of the emitted light, we observe that the QD emission spectrum is determined by the spectrum of the resonant excitation laser. We present high-resolution measurements by Fourier transform spectroscopy of the RE where the data are fitted to the first-order correlation function g(1)(τ) of the RE of a two-level system. The inverse Fourier transform of the g(1)(τ) function allows a direct comparison of the different RE emission profiles. We show that, by reducing the resonant excitation power, the so-called Mollow triplet shrinks to a single narrow Lorentzian line, while the relative intensity of this narrow peak increases and tends to overwhelm the RE spectrum. This implies that single QDs can produce single photons with a coherence time that is not limited anymore by the QD electronic properties, resulting in an ultra-coherent character [6]. In conclusion, the resulting " ultra-coherent single photon source " promises high degrees of indistinguishability of the emitted photons which is a crucial requirement for quantum information applications. [1] P. Michler et al., Science 290, 2282 (2000). [2] A. Muller et al., Phys. Rev. Lett. 99, 187402 (2007). [3] S. Ates et al., Phys. Rev. Lett. 103, 167402 (2009). [4] H. S. Nguyen et al., Phys. Rev. Lett. 108, 057401 (2012). [5] C. Santori et al., Nature 419, 594 (2002). [6] H. S. Nguyen et al., Appl. Phys. Lett. 99, 261904 (2011).
Semiconductor quantum dots (QDs) are commonly considered as artificial atoms and these nanostructures are very promising for the realization of integrated devices such as single photon sources for quantum cryptography applications [1,2]. However, contrarily to genuine atoms, QDs are condensed matter systems and they consequently suffer from the coupling to their environment that acts as a fluctuating reservoir for spectral diffusion [3] and degrades the indistinguishability of the emitted photons. One way to circumvent this coupling in order to reach the so-called fundamental radiative limit is to excite strictly resonantly the QD at low temperature [4-9]. Up to now, the measurements reported in the literature mainly focus on the incoherent photoluminescence signal for achieving single photon emission. In this regime, the linewidth of the photoluminescence spectrum is always limited to the radiative limit. In this paper, we report on the resonant emission (RE) of the exciton in single InAs/GaAs QDs embedded in a planar microcavity, in an orthogonal excitation-detection geometry. We present an original type of single photon source based on the coherent laser light scattering by a single QD [10]. Besides the antibunching effect showing the non-classical nature of the emitted light, we observe that the QD emission spectrum is determined by the spectrum of the resonant excitation laser. We present high-resolution measurements by Fourier transform spectroscopy of the RE where the data are fitted to the first-order correlation function g(1)(τ) of a two-level system. The inverse Fourier transform of the g(1)(τ) function allows a direct comparison of the different RE emission profiles. We show that, by reducing the resonant excitation power, the so-called Mollow triplet shrinks to a single narrow Lorentzian line, while the relative intensity of this narrow peak increases and tends to overwhelm the RE spectrum. This implies that single QDs can produce single photons with a coherence time that is not limited anymore by the QD electronic properties, resulting in what we name an ultra-coherent character [10]. In conclusion, the resulting " ultra-coherent single photon source " promises high degrees of indistinguishability of the emitted photons which is a crucial requirement for quantum information applications. [1] P. Michler et al., Science 290, 2282 (2000). [6] S. Ates et al., PRL 103, 167402 (2009). [2] C. Santori et al., Nature 419, 594 (2002). [7] H. S. Nguyen et al., PRL 108, 057401 (2012). [3] A. Berthelot et al., Nat. Phys. 2, 759 (2006). [8] C. Matthiesen et al., PRL 108, 093602 (2012). [4] A. Muller et al., PRL 99, 187402 (2007). [9] A. Reinhard et al., Nat. Phot. 6, 93 (2012). [5] R. Melet et al., PRB 78, 073301 (2008). [10] H. S. Nguyen et al., APL 99, 261904 (2011).
Abstract In the quest to realize a scalable quantum network, semiconductor quantum dots (QDs) offer distinct advantages including high single-photon efficiency and indistinguishability, high repetition rate (tens of GHz with Purcell enhancement), interconnectivity with spin qubits, and a scalable on-chip platform. However, in the past two decades, the visibility of quantum interference between independent QDs rarely went beyond the classical limit of 50% and the distances were limited from a few meters to kilometers. Here, we report quantum interference between two single photons from independent QDs separated by 302 km optical fiber. The single photons are generated from resonantly driven single QDs deterministically coupled to microcavities. Quantum frequency conversions are used to eliminate the QD inhomogeneity and shift the emission wavelength to the telecommunication band. The observed interference visibility is 0.67\pm0.02 (0.93\pm0.04) without (with) temporal filtering. Feasible improvements can further extend the distance to ~600 km. Our work represents a key step to long-distance solid-state quantum networks.
We demonstrate interference between discrete photons emitted by two different semiconductor quantum dots and quantify their degree of indistinguishability. The quantum dot emission energies are tuned into resonance by straining the samples. Upon interference on a beamsplitter, the photons are shown to be 18.1% indistinguishable, resulting in a coincidence detection rate below the classical limit. Post-selecting only those detections occurring within a short time of each other increases the measured indistinguishability to 47%. The photons are partially distinguishable due to dephasing of the exciton states, and post-selection is also affected by the detector response time.
In the quest to realize a scalable quantum network, semiconductor quantum dots (QDs) offer distinct advantages, including high single-photon efficiency and indistinguishability, high repetition rate (tens of gigahertz with Purcell enhancement), interconnectivity with spin qubits, and a scalable on-chip platform. However, in the past two decades, the visibility of quantum interference between independent QDs rarely went beyond the classical limit of 50%, and the distances were limited from a few meters to kilometers. Here, we report quantum interference between two single photons from independent QDs separated by a 302 km optical fiber. The single photons are generated from resonantly driven single QDs deterministically coupled to microcavities. Quantum frequency conversions are used to eliminate the QD inhomogeneity and shift the emission wavelength to the telecommunication band. The observed interference visibility is 0.67 ± 0.02 (0.93 ± 0.04) without (with) temporal filtering. Feasible improvements can further extend the distance to ∼600 km. Our work represents a key step to long-distance solid-state quantum networks.