Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Journal of Physics B Atomic and Molecular Physics

Photon-scattered-atom coincidence study on K-He with vector polarisation analysis

L Zehnle, E. Clemens, P J Martin, W Schauble, Volker Kempter

Published Aug 28, 1978• 27 citations
Publisher

Abstract

The linear and circular polarisation of the K(4 2 P to 4 2 S) photons detected in delayed coincidence with the inelastically scattered K atoms are presented for K-He collisions at 93 eV as a function of the scattering angle. Data are analysed in terms of the Stokes parameters, and the coherence properties of the excitation process are examined. It is concluded that spin dependent forces do not play an important role in the excitation process. The lambda and chi parameters are also derived. Simple models for the excitation process are discussed in order to explain the impact parameter dependence of chi .

DOI
10.1088/0022-3700/11/16/014

Related papers

Photon Vector Polarization and Coherence Parameters in an Electron-Photon Coincidence Experiment on Helium

M. C. Standage, Hans Kleinpoppen

We present linear and circular polarization measurements of $3^{1}P\ensuremath{-}2^{1}S$ (501.6 nm) photons detected in delayed coincidence with electrons inelastically scattered from the $3^{1}P$ level of helium. Vector polarization and coherence parameters of the coincident radiation provide direct experimental evidence of the coherent nature of the excitation process. Atomic orientation is obtained directly from the circular polarization measurements. Analysis of the data also yields $\ensuremath{\lambda}$ and $\ensuremath{\chi}$ parameters for $3^{1}P$ excitations, which are compared with previous data and theory.

Physical Review Letters•Mar 15, 1976•144 citations

Electron-polarised-photon coincidence experiments on the 31P state of helium

Johannes P. M. Beijers, J P van den Brink, J. van Eck +1 more

The authors present circular-polarisation measurements of 3 1 P to 2 1 S photons (501.6 nm) detected in delayed coincidence with electrons inelastically scattered upon excitation of the 3 1 P state of helium. They performed these experiments as a function of the electron scattering angle at incident electron energies of 80, 60 and 50 eV in order to study the orbital angular momentum transfer during the collision. The experimental results are compared with previous angular correlation data and with theory. For each incident electron energy they found a sign reversal of the angular momentum transfer as a function of the electron scattering angle.

Journal of Physics B Atomic and Molecular Physics•Sep 14, 1986•11 citations

Angular and polarisation correlation measurements on the 21P and 31P states of helium

Khalid Salman Ibraheim

The delayed coincidence technique was applied to investigate angular and polarization correlations between electrons scattered inelastically from helium atoms and photons emitted in the decay of n1P states. \n \nElectron photon angular correlations were studied for the excitation of the 21P and 31P states of helium at an incident electron energy of 50 eV and for electron scattering angles in the range of 20° - 102° and 35° - 55o respectively. From the analysis of these measurements the excitation parameters λ = (|a¬o| 2)/(2| a1| 2+|ao| 2) = σo/σ and the magnitude |x| of the phase difference between the excitation amplitudes a_ML for the M_L = 1 and M_L = 0 states are obtained. \n \nUsing the 3¬¬1P - 21S decay light the electron-photon polarization correlation were measured for the 31P state of helium at electron impact energies 50, 80, 120 and 160 eV and for electron scattering angles between 27.5° and 108°. The Stokes parameters n1, n2 and n3 were derived and the sign change of the angular momentum transfer < Ly > to the atom was investigated using the circular polarization results (n2). A sign change was confirmed for all energies studied and the scattering angle of the sign change was found to increase with decreasing electron energy. The excitation parameters λ and x have been derived and the present results are compared with theoretical calculations and with previous experimental values obtained from angular and polarization correlation measurements.

•Jan 1, 1986•0 citations

Electron impact excitation of 2p states in atomic hydrogen

Marcin L. Gradziel

This thesis presents the results of experimental investigation of coherence in the excitation of the 2p states of atomic hydrogen through a collision with an unpolarised electron. The polarisation correlation variation of the delayed coincidence method has been employed to simultaneously measure the reduced Stokes parameters P1,P2 and P3, which are needed to fully characterise the state of the atom immediately after the collision. This has also allowed the excitation coherence parameter P+ to be determined directly. In the case of the excitation of 2p states of hydrogen, a deviation of P+ from unity is indicative of the importance of spin exchange during the collision. A new Lyman- polarisation analyser, that permits independent rotation of a retarder and a linear polariser, was developed for this work. A novel approach to the analysis of data from electron-photon coincidence measurements has been implemented to improve the quality of the final results. The reduced Stokes parameters P1,P2 and P3 were measured at 54.4 eV electron energy, and in the 4-40 range of electron scattering angles. The P1 and P2 results are consistent with the earlier measurements, and recent theoretical predictions. The new P3 results, however, deviate significantly from the predictions of all modern theories, and also differ from previous experimental results. The newly measured values of P+ also suggest less coherent excitation than predicted by the theory, even at a relatively low scattering angle of 30. Several possible sources of systematic error including resonance radiation trapping, Stark mixing and erroneous phase-shift of the retarder have been considered, but are insufficient to explain the observed deviations from theory. Therefore, we are forced to conclude that spin exchange may play a more significant role during the collision than current theoretical methods predict.

•Jul 1, 2003•0 citations

On the coherence of the excitation of the 32P state in sodium by 100 eV electrons

P. J. O. Teubner, J L Riley, J. E. Furst +1 more

An electron-photon coincidence technique has been used to study the coherence of the excitation of the 3 2 P state in sodium. The total polarisation of the decay photons has been determined by measuring the linear and circular components of the Stokes's vector. Analysis of the reduced degree of polarisation mod P mod shows that the excitation is coherent for electrons which have been scattered through the angular range from 3 to 10 degrees . The concept of reduced polarisation assumes that the Percival-Seaton hypothesis applies to the collision. Thus the authors deduce that the nuclear spin plays no role in the excitation process at this energy and over these scattering angles. Scattering parameters have been deduced from the individual components of the Stokes's vector. These have been compared with those predicted by calculations based on the first Born and distorted-wave polarised orbital approximations. It is found that neither theory adequately describes the interaction.

Journal of Physics B Atomic and Molecular Physics•Jan 28, 1985•11 citations

Electron-photon coincidence studies of the resolved argon resonance lines

I C Malcolm, J. William McConkey

The excitation by electron impact at 50 eV, of the 104.8 and 106.7 nm lines of Ar, have been studied separately using the electron-polarised-photon coincidence technique. Polarisation correlations have been measured for electron scattering angles of 0 and 5 degrees . From the measurements at 5 degrees the authors derived the parameters lambda (0.72+or-0.06, 0.60+or-0.05) and mod chi mod (0.99 rad+or-0.19, 0.0) for the 104.8 and 106.7 nm lines, respectively. Thus, contrary to the assumptions of Arriola et al. (see ibid., vol.8, p.1275 (1975)) significant differences may occur between the two lines. The value of chi obtained for the 106.7 nm line implies total coherence at the energy and angle studied. The measurements at 0 degrees yielded 'threshold' polarisations of 0.41+or-0.13 (104.8 nm) and 0.94+or-0.14 (106.7 nm).

Journal of Physics B Atomic and Molecular Physics•Feb 14, 1979•31 citations
The linear and circular polarisation of the K(4 2 P to 4 2 S) photons detected in delayed coincidence with the inelastically scattered K atoms are presented for K-He collisions at 93 eV as a function of the scattering angle. Data are analysed in terms of the Stokes parameters, and the coherence properties of the excitation process are examined. It is concluded that spin dependent forces do not play an important role in the excitation process. The lambda and chi parameters are also derived. Simple models for the excitation process are discussed in order to explain the impact parameter dependence of chi .
We present linear and circular polarization measurements of $3^{1}P\ensuremath{-}2^{1}S$ (501.6 nm) photons detected in delayed coincidence with electrons inelastically scattered from the 31P3^{1}P31P level of helium. Vector polarization and coherence parameters of the coincident radiation provide direct experimental evidence of the coherent nature of the excitation process. Atomic orientation is obtained directly from the circular polarization measurements. Analysis of the data also yields $\ensuremath{\lambda}$ and $\ensuremath{\chi}$ parameters for 31P3^{1}P31P excitations, which are compared with previous data and theory.
The authors present circular-polarisation measurements of 3 1 P to 2 1 S photons (501.6 nm) detected in delayed coincidence with electrons inelastically scattered upon excitation of the 3 1 P state of helium. They performed these experiments as a function of the electron scattering angle at incident electron energies of 80, 60 and 50 eV in order to study the orbital angular momentum transfer during the collision. The experimental results are compared with previous angular correlation data and with theory. For each incident electron energy they found a sign reversal of the angular momentum transfer as a function of the electron scattering angle.
The delayed coincidence technique was applied to investigate angular and polarization correlations between electrons scattered inelastically from helium atoms and photons emitted in the decay of n1P states. \n \nElectron photon angular correlations were studied for the excitation of the 21P and 31P states of helium at an incident electron energy of 50 eV and for electron scattering angles in the range of 20° - 102° and 35° - 55o respectively. From the analysis of these measurements the excitation parameters λ = (|a¬o| 2)/(2| a1| 2+|ao| 2) = σo/σ and the magnitude |x| of the phase difference between the excitation amplitudes a_ML for the M_L = 1 and M_L = 0 states are obtained. \n \nUsing the 3¬¬1P - 21S decay light the electron-photon polarization correlation were measured for the 31P state of helium at electron impact energies 50, 80, 120 and 160 eV and for electron scattering angles between 27.5° and 108°. The Stokes parameters n1, n2 and n3 were derived and the sign change of the angular momentum transfer < Ly > to the atom was investigated using the circular polarization results (n2). A sign change was confirmed for all energies studied and the scattering angle of the sign change was found to increase with decreasing electron energy. The excitation parameters λ and x have been derived and the present results are compared with theoretical calculations and with previous experimental values obtained from angular and polarization correlation measurements.
This thesis presents the results of experimental investigation of coherence in the excitation of the 2p states of atomic hydrogen through a collision with an unpolarised electron. The polarisation correlation variation of the delayed coincidence method has been employed to simultaneously measure the reduced Stokes parameters P1,P2 and P3, which are needed to fully characterise the state of the atom immediately after the collision. This has also allowed the excitation coherence parameter P+ to be determined directly. In the case of the excitation of 2p states of hydrogen, a deviation of P+ from unity is indicative of the importance of spin exchange during the collision. A new Lyman- polarisation analyser, that permits independent rotation of a retarder and a linear polariser, was developed for this work. A novel approach to the analysis of data from electron-photon coincidence measurements has been implemented to improve the quality of the final results. The reduced Stokes parameters P1,P2 and P3 were measured at 54.4 eV electron energy, and in the 4-40 range of electron scattering angles. The P1 and P2 results are consistent with the earlier measurements, and recent theoretical predictions. The new P3 results, however, deviate significantly from the predictions of all modern theories, and also differ from previous experimental results. The newly measured values of P+ also suggest less coherent excitation than predicted by the theory, even at a relatively low scattering angle of 30. Several possible sources of systematic error including resonance radiation trapping, Stark mixing and erroneous phase-shift of the retarder have been considered, but are insufficient to explain the observed deviations from theory. Therefore, we are forced to conclude that spin exchange may play a more significant role during the collision than current theoretical methods predict.
An electron-photon coincidence technique has been used to study the coherence of the excitation of the 3 2 P state in sodium. The total polarisation of the decay photons has been determined by measuring the linear and circular components of the Stokes's vector. Analysis of the reduced degree of polarisation mod P mod shows that the excitation is coherent for electrons which have been scattered through the angular range from 3 to 10 degrees . The concept of reduced polarisation assumes that the Percival-Seaton hypothesis applies to the collision. Thus the authors deduce that the nuclear spin plays no role in the excitation process at this energy and over these scattering angles. Scattering parameters have been deduced from the individual components of the Stokes's vector. These have been compared with those predicted by calculations based on the first Born and distorted-wave polarised orbital approximations. It is found that neither theory adequately describes the interaction.
The excitation by electron impact at 50 eV, of the 104.8 and 106.7 nm lines of Ar, have been studied separately using the electron-polarised-photon coincidence technique. Polarisation correlations have been measured for electron scattering angles of 0 and 5 degrees . From the measurements at 5 degrees the authors derived the parameters lambda (0.72+or-0.06, 0.60+or-0.05) and mod chi mod (0.99 rad+or-0.19, 0.0) for the 104.8 and 106.7 nm lines, respectively. Thus, contrary to the assumptions of Arriola et al. (see ibid., vol.8, p.1275 (1975)) significant differences may occur between the two lines. The value of chi obtained for the 106.7 nm line implies total coherence at the energy and angle studied. The measurements at 0 degrees yielded 'threshold' polarisations of 0.41+or-0.13 (104.8 nm) and 0.94+or-0.14 (106.7 nm).