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Physical Review A

Velocity-selective coherent population trapping of two-level atoms

James S. Hack, L. Liu, Maxim Olshanii, H. Metcalf

Published Jun 12, 2000• 18 citations
Publisher

Abstract

We have demonstrated velocity-selective coherent population trapping (VSCPT) in a two-level system created by circularly polarized light driving the $2{}^{3}{S}_{1}\ensuremath{\rightarrow}3{}^{3}{P}_{2}$ transition in metastable helium. It is quite different from the usual VSCPT because there need be no consideration of selection rules, polarization, or internal atomic states. This most primitive case elicits the simple nature of VSCPT as a special kind of quantum interference, and demonstrates the presence of VSCPT in a system that has only two internal levels. It is readily observed for this transition because the ratio of the recoil frequency to the natural linewidth is 0.22, two orders of magnitude larger than for most laser cooling experiments. Our trapped state is fed by Doppler cooling, which is unusually effective here because of the large recoil, and is totally absent in previously described VSCPT experiments.

DOI
10.1103/physreva.62.013405

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Cambridge University Press eBooks•Sep 2, 2010•0 citations
We have demonstrated velocity-selective coherent population trapping (VSCPT) in a two-level system created by circularly polarized light driving the 23S1\ensuremath→33P22{}^{3}{S}_{1}\ensuremath{\rightarrow}3{}^{3}{P}_{2}23S1​\ensuremath→33P2​ transition in metastable helium. It is quite different from the usual VSCPT because there need be no consideration of selection rules, polarization, or internal atomic states. This most primitive case elicits the simple nature of VSCPT as a special kind of quantum interference, and demonstrates the presence of VSCPT in a system that has only two internal levels. It is readily observed for this transition because the ratio of the recoil frequency to the natural linewidth is 0.22, two orders of magnitude larger than for most laser cooling experiments. Our trapped state is fed by Doppler cooling, which is unusually effective here because of the large recoil, and is totally absent in previously described VSCPT experiments.
ABSTRACT In this work we present an investigation of velocity-selective coherent population trapping (VSCPT) in asym- metric three-level schemes. The light force in such schemes is of an intrinsically transient character and shouldnot be described in a quasiclassical approach. Instead, results of the full quantum-mechanical calculations are presented with emphasis on their meaning to the efficiency of subrecoil laser cooling. 1 INTRODUCTION Laser cooling of neutral atoms has received significant advances by the introduction of velocity-selectivecoherent population trapping ((VSCPT) some years ago.1 Since it leads to atomic temperatures well below therecoil limit, studies of ultracold atoms and atomic interactions may be improved by magnitudes.The effect of VSCPT relies on optical pumping of atoms into a state WNC) which is a trap state for a certaincenter-of-mass velocity vO. This trap state is created by a destructive superposition of atomic states within amultilevel quantum system. Once being in such a state LWNC) the laser light does not interact anymore with theatom which leads to a decoupling with the rest of the system at vo. Atoms located outside this small velocityregion get a chance to be trapped by the momentum diffusion due to spontaneous emission of photons. Aftera sufficient long interaction time nearly all atoms are trapped inside a narrow momentum distribution whichcan be interpreted as cooling. The theoretical and experimental investigation of VSCPT is usually consideredby use of a three-level A-system as shown in Fig.1. Such a system can be found for example in a symmetrical
We present a fully quantum analysis of velocity selective coherent population trapping (VSCPT) in two schemes for which there is a force which assists in the accumulation of atoms in the trapping state. In the first scheme, the F g =2 to F e =2 transition was studied where the existence of a semiclassical polarization gradient force even for a pure sigma + - sigma - configuration has been demonstrated which gives cooling for blue detuning. We also verify that cooling may be obtained for the F=2 to 1 and F=3 to 2 transitions; our fully quantum mechanical calculations yield a result which is consistent with recent experimental results of Valentin et al. (1992) but differ from previous semiclassical calculations. Secondly, we discuss a scheme of force-assisted VSCPT which combines VSCPT on the F g =1 to F e =1 transition with the coupling to another transition for which a strong sub-Doppler cooling force is present. This scheme allows velocity selective coherent population trapping and the polarization-gradient force to work under optimum conditions simultaneously. We find that both of these two schemes lead to efficient cooling of atoms.
We present a set of exploratory experimental studies of velocity-selective coherent population trapping (VSCPT) on the $2{}^{3}{S}_{1}\ensuremath{\rightarrow}2{}^{3}{P}_{1}$ transition of Helium, including the effect of an external magnetic field along the propagation direction of the light. We also investigate in detail the effects of the laser detuning and the atom-laser interaction time in determining the shape and width of the VSCPT velocity distribution. Our data corroborates some previous theory and calculations. We demonstrate that the only observable effect of a magnetic field applied along the direction of light propagation is to shift the center of the VSCPT peaks in the atomic velocity distribution by an amount proportional to the magnitude of the applied field. We present a semiclassical picture that describes the atomic motion of VSCPT in such a B field.
In recent years, there has been a great deal of interest in velocity selective coherent population trapping (VSCPT).1 However, since VSCPT occurs via a random walk in momentum space, in order to achieve significant VSCPT in three dimensions, it is necessary to precool and confine atoms dose to the recoil momentum. Shahriar et al.2 recently predicted that this type of cooling and velocity confinement assisted VSCPT can be achieved in one, two, or three dimensions when a Λ-system atom is excited by a pair of blue detuned Raman resonant standing waves, with a phase difference of θ = π/4.
One-dimensional laser cooling based on velocity-selective coherent population trapping (VSCPT) has been investigated numerically through the solution of the optical Bloch equations and through a Monte Carlo analysis. The 1\ensuremath{\rightarrow}1 and 2\ensuremath{\rightarrow}2 transitions have been examined as a function of the atomic recoil frequency, the spontaneous-emission decay rate, and the Rabi frequency of the cooling laser. It has been found that for a large set of those parameters, the VSCPT cooling process may be described through scaling-law relations. The scaling laws are not valid at long atom-laser interaction times or large Rabi frequencies, where the atomic Doppler shift plays a significant role in the atomic motion evolution. Similar results for two atomic transitions suggest the validity of the scaling law for any one-dimensional VSCPT process. \textcopyright{} 1996 The American Physical Society.
In Section 8.3.9, we mentioned that the recoil temperature was not the ultimate barrier to cooling. Several mechanisms have been conceived and implemented to concentrate the atomic velocity distribution in a range of values of width less than V R . In contrast to Doppler or Sisyphus cooling, these mechanisms do not appeal to a friction force, but rather to an optical pumping process (see Complement 2B), able to accumulate the atoms in this narrow range of velocities. We now present one such mechanism called ‘velocity-selective coherent population trapping’, considering only the case where the motion occurs in one space direction (the O z -axis). Note, however, that the method generalizes to two or three dimensions. Coherent population trapping Coherent population trapping is a phenomenon that occurs when an atom has a system of three energy levels in the ∧ configuration shown in Figure 8A.1, where each leg of the ∧ interacts with a laser L − or L + . This was discussed in detail in Section 2D.2 of Complement 2D. Here we consider the case where the two ground states g + and L − , have exactly the same energy, and the two lasers have frequencies ω + and ω − , very close to the resonance frequency ω 0 . In this situation, the selectivity of the interactions is obtained via the polarization selection rules (see Complement 2B): if g − , g + and e have magnetic quantum numbers m = −1, +1 and 0, respectively, the laser wave L − is right-circularly polarized (σ + polarization), while the laser wave L + is left-circularly polarized (σ − polarization).