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Physical Review A

Study of the optical piston

H. G. C. Werij, Jos E. M. Haverkort, J. P. Woerdman

Published May 1, 1986• 63 citations
Publisher

Abstract

We report an experimental and theoretical study of the optical piston, a consequence of the phenomenon of light-induced drift (LID), observed in binary mixtures of Na vapor and a buffer gas. Good agreement has been found between experiment and existing theory as far as the shape of the Na density profile in the piston is concerned. The piston velocity is anomalously low; this is accounted for by incorporating the effects of adsorption and desorption into the theory. Furthermore, we introduce a rate-equation model for LID which incorporates the fine and hyperfine structure of the level scheme of the Na absorbers; this gives insight into the sublevel velocity distributions and the nonequilibrium part of the total velocity distribution during LID.

DOI
10.1103/physreva.33.3270

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Study of the optical piston

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In the past, interpretation of light-induced drift (LID) effects in alkali–noble gas mixtures in capillary cells has been severely complicated by surface interactions. As an example, the velocity of the optical piston, a spectacular manifestation of LID, is limited by adsorption–desorption processes to a value in the mm/s range.1 Recently, a breakthrough has been made: by coating the capillary wall with paraffin the surface interaction has been completely eliminated leading to transport velocities in the m/s range and allowing a study of LID in its pure form.2 Here we report the first measurements of the detuning and intensity dependence of the drift velocity in Na–noble gas mixtures and compare these to theory.

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The anomalous light-induced drift (LID) of atoms caused by a velocity dependence of collision frequencies has been investigated in the frame of the theory without adjustable parameters. Our results open the possibility of experimental probing of models of interatomic potentials. The extension of the strong-collision model to the case of velocity-dependent collision rates, is the basis of our approach. The obtained model describes the anomalous LID both in the case of arbitrary mass ratio of absorbing- and buffer-gas particles and in the case of arbitrary ratio of the homogeneous and Doppler widths. In particular, we applied our model to describe the anomalous LID in alkali - noble-gas mixtures (Rb - Kr and Li - Ne systems). Qualitatively another anomaly of the LID velocity was also found in the low-pressure region. As pointed out, the optical pumping effect and the hyperfine structure of the ground electronic state, but not the velocity dependence of the collision rates, are the sources of this new anomaly.

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We present results of a numerical model of the optical piston driven by laser-induced drift (LID). The model is based on a drift-velocity formulation of Lawandy, derived from an asymmetric-random-walk argument, and includes resonance-fluorescence effects. The model is applied primarily to the experimental conditions of H. G. C. Werij and co-workers [Phys. Rev. A 33, 3270 (1986)]. It is shown that both the velocity and the shape of the propagating density wave change continuously throughout the traverse of a (finite) diffusion tube under these conditions. In addition, we have numerically verified the contention of G. Nienhuis [Phys. Rev. A 31, 1636 (1985)] that a ``self-preserving'' form of the density wave is indeed possible for the case of a ``finite number of absorbers in an infinite medium,'' both with and without saturation. Finally, we show that resonance fluorescence slows the piston velocity, broadens the density distribution, and decreases its peak height. It is concluded that resonance fluorescence can play a significant role in determining the time evolution and detailed shape of the optical-piston density distribution in sodium.

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This paper is a theoretical study of the spectral features of the velocity of light-induced drift (LID) of lithium atoms ( 7 Li and 6 Li) in a binary mixture of noble gases: Ne + Ar, Ne + Kr, and Ne + Xe. The spectral shape of the LID signal is predicted to depend strongly on the fraction ξ of neon in the buffer mixture in the range ξ≈0.8–0.9 (ξ= N Ne / N b , where N Ne is the neon concentration, and N b is the total concentration of the buffer particles). When the velocity of anomalous LID is treated as a function of the radiation frequency, it is found to have one, three, five, or seven zeros and to differ substantially from the dispersion-curve-like behavior with one zero predicted by the standard LID theory with velocity-independent transport collision rates. The reason for these additional zeros of the drift velocity is the alternating-sign dependence on the lithium-atom velocity of the relative difference of transport rates of collisions between buffer particles and excited and unexcited atoms. What is also established is that the anomalous LID of lithium atoms can be observed at almost all temperatures, depending on the value of ξ. At a fixed temperature, anomalous LID can be observed only in a narrow range of values of the fraction of neon in the buffer mixture, Δξ≈0.02. The results make possible highly precise testing in the LID experiments of the interatomic potentials used in calculations of the velocity spectrum of anomalous LID.

Journal of Experimental and Theoretical Physics•Nov 1, 1999•5 citations
We report an experimental and theoretical study of the optical piston, a consequence of the phenomenon of light-induced drift (LID), observed in binary mixtures of Na vapor and a buffer gas. Good agreement has been found between experiment and existing theory as far as the shape of the Na density profile in the piston is concerned. The piston velocity is anomalously low; this is accounted for by incorporating the effects of adsorption and desorption into the theory. Furthermore, we introduce a rate-equation model for LID which incorporates the fine and hyperfine structure of the level scheme of the Na absorbers; this gives insight into the sublevel velocity distributions and the nonequilibrium part of the total velocity distribution during LID.
In the past, interpretation of light-induced drift (LID) effects in alkali–noble gas mixtures in capillary cells has been severely complicated by surface interactions. As an example, the velocity of the optical piston, a spectacular manifestation of LID, is limited by adsorption–desorption processes to a value in the mm/s range.1 Recently, a breakthrough has been made: by coating the capillary wall with paraffin the surface interaction has been completely eliminated leading to transport velocities in the m/s range and allowing a study of LID in its pure form.2 Here we report the first measurements of the detuning and intensity dependence of the drift velocity in Na–noble gas mixtures and compare these to theory.
We present a model for light-induced drift (LID) in the Na--noble-gas system which should enable direct comparison with experiment. In contrast to previous theories of LID based on a two-level description of the optical absorbers and on a simplified collision treatment, the present model is based on a realistic description of laser-driven Na atoms immersed in a buffer gas. Starting from the generalized Bloch equations, we introduce a rate-equation model for the velocity distributions in the four important Na levels. The velocity-changing and fine-structure-changing collisions are described using composite Keilson-Storer collision kernels in which all adjustable parameters have been eliminated by using available literature data. We apply the model in numerical calculations of LID as a function of all experimentally accessible parameters. It is found that the ground-state hyperfine splitting can have large effects on LID, whereas the excited-state fine-structure splitting has not. The paper establishes criteria for optimum LID effects; when using a single-frequency laser the maximum attainable drift velocity is predicted to be 13.8 m/s. Using a proper set of boundary conditions, we find a pressure dependence of LID qualitatively different from the predictions based on previous work. Finally, the influence of the collision model is investigated. We find that LID is independent of the shape of the collision kernel, indicating that a strong-collision model is always valid.
The anomalous light-induced drift (LID) of atoms caused by a velocity dependence of collision frequencies has been investigated in the frame of the theory without adjustable parameters. Our results open the possibility of experimental probing of models of interatomic potentials. The extension of the strong-collision model to the case of velocity-dependent collision rates, is the basis of our approach. The obtained model describes the anomalous LID both in the case of arbitrary mass ratio of absorbing- and buffer-gas particles and in the case of arbitrary ratio of the homogeneous and Doppler widths. In particular, we applied our model to describe the anomalous LID in alkali - noble-gas mixtures (Rb - Kr and Li - Ne systems). Qualitatively another anomaly of the LID velocity was also found in the low-pressure region. As pointed out, the optical pumping effect and the hyperfine structure of the ground electronic state, but not the velocity dependence of the collision rates, are the sources of this new anomaly.
We present results of a numerical model of the optical piston driven by laser-induced drift (LID). The model is based on a drift-velocity formulation of Lawandy, derived from an asymmetric-random-walk argument, and includes resonance-fluorescence effects. The model is applied primarily to the experimental conditions of H. G. C. Werij and co-workers [Phys. Rev. A 33, 3270 (1986)]. It is shown that both the velocity and the shape of the propagating density wave change continuously throughout the traverse of a (finite) diffusion tube under these conditions. In addition, we have numerically verified the contention of G. Nienhuis [Phys. Rev. A 31, 1636 (1985)] that a ``self-preserving'' form of the density wave is indeed possible for the case of a ``finite number of absorbers in an infinite medium,'' both with and without saturation. Finally, we show that resonance fluorescence slows the piston velocity, broadens the density distribution, and decreases its peak height. It is concluded that resonance fluorescence can play a significant role in determining the time evolution and detailed shape of the optical-piston density distribution in sodium.
This paper is a theoretical study of the spectral features of the velocity of light-induced drift (LID) of lithium atoms ( 7 Li and 6 Li) in a binary mixture of noble gases: Ne + Ar, Ne + Kr, and Ne + Xe. The spectral shape of the LID signal is predicted to depend strongly on the fraction ξ of neon in the buffer mixture in the range ξ≈0.8–0.9 (ξ= N Ne / N b , where N Ne is the neon concentration, and N b is the total concentration of the buffer particles). When the velocity of anomalous LID is treated as a function of the radiation frequency, it is found to have one, three, five, or seven zeros and to differ substantially from the dispersion-curve-like behavior with one zero predicted by the standard LID theory with velocity-independent transport collision rates. The reason for these additional zeros of the drift velocity is the alternating-sign dependence on the lithium-atom velocity of the relative difference of transport rates of collisions between buffer particles and excited and unexcited atoms. What is also established is that the anomalous LID of lithium atoms can be observed at almost all temperatures, depending on the value of ξ. At a fixed temperature, anomalous LID can be observed only in a narrow range of values of the fraction of neon in the buffer mixture, Δξ≈0.02. The results make possible highly precise testing in the LID experiments of the interatomic potentials used in calculations of the velocity spectrum of anomalous LID.