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Optics Communications

A pulsed, optically-pumped rubidium laser at high pump intensity

Clifford V. Sulham, Glen P. Perram, Michael P. Wilkinson, David A. Hostutler

Published Jun 26, 2010• 36 citations
Publisher
DOI
10.1016/j.optcom.2010.06.038

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A pulsed, optically pumped rubidium laser operating in analogy to the diode pumped alkali laser (DPAL) system at pump intensities as high as 750 kW/cm2 has been demonstrated with output energies of up to 13 μJ/pulse. Output energy is dramatically limited by spin‐orbit relaxation rates under these high intensity pump conditions. More than 250 photons are available for every rubidium atom in the pumped volume, requiring a high number of cycles per atom during the 2–8 ns duration of the pump pulse. At 550 Torr of ethane, the spin‐orbit relaxation rate is too slow to effectively utilize all the incident pump photons. Indeed, a linear dependence of output energy on pump pulse duration for fixed pump energy is demonstrated.

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We have developed a versatile pulsed laser system for high precision magnetometry. The operating wavelength of the system can be configured to optically pump alkali vapors such as rubidium and cesium. The laser system consists of an auto-locked, interference filter stabilized, external cavity diode laser (ECDL), a tapered waveguide amplifier, and a pulsing module. The auto-locking controller can be used by an untrained operator to stabilize the laser frequency with respect to a library of atomic, molecular, and solid-state spectral markers. The ECDL output can be amplified from 20 mW to 2 W in continuous wave (CW) mode. The pulsing module, which includes an acousto-optic modulator (AOM), can generate pulses with durations of 20 ns and repetition rates of several MHz. Accordingly, the laser system is well suited for applications such as gravimetry, magnetometry, and differential absorption lidar. In this work, we focus on magnetometric applications and demonstrate that the laser source is suitable for optically pumping rubidium vapor. We also describe numerical simulations of optical pumping relevant to the rubidium D1 and D2 transitions at 795 nm and 780 nm respectively. These studies are relevant to the design and construction of a new generation of portable, rubidium, spin exchange relaxation-free (SERF) magnetometers, capable of sensitivities of 1 fT Hz-1/2 1.

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Optically Pumped Atomic Rubidium Lasers: Two-Photon and Exciplex Excitation Mechanisms

Jeffrey Gallagher

Abstract : The Doppler-broadened two-photon absorption (TPA) cross-section for the 52S1/2- 52D5/2 transition in Rb is measured using direct absorption methods. A detailed model of the intensity profile was developed to account for a focused Gaussian beam propagating through a two-photon absorption medium. A peak absorbance of 24% was observed for an intensity of 6.28 kW/cm2 at the focus, a Rb density of 4.6 x 1015 cm-3 concentrations from 1.61-8.52 x 10(15) cm-3 line. Extracting the hyperfine-broadened TPA cross-section from 87 test configurations, while varying the pump power, alkali concentration and focal length, yielded an error weighted average of 6.75x10-21 cm4/W. This cross-section is sufficient for a pulsed dye laser to bleach the pump transition in the Two-Photon Pumped Alkali Laser (TPAL) that lases at 420 nm and 5.2 mum. Additionally, optically pumped atomic rubidium lasers pumped in the blue satellite of the D2 line from the ground Rb-Ar or Rb-Kr collision pair to the dissociative B2 sum 1/2 produce laser emission at 780.2 nm. Lasing is achieved for the Rb-Ar system and 757.1 - 760.4 nm for the Rb-Kr system. Slope efficiencies exceed 0.25% using a heat pipe configuration. The gain is very high with photon build-up times of 1-3.7 ns.

•Jun 1, 2013•2 citations
A pulsed, optically pumped rubidium laser operating in analogy to the diode pumped alkali laser (DPAL) system at pump intensities as high as 750 kW/cm2 has been demonstrated with output energies of up to 13 μJ/pulse. Output energy is dramatically limited by spin‐orbit relaxation rates under these high intensity pump conditions. More than 250 photons are available for every rubidium atom in the pumped volume, requiring a high number of cycles per atom during the 2–8 ns duration of the pump pulse. At 550 Torr of ethane, the spin‐orbit relaxation rate is too slow to effectively utilize all the incident pump photons. Indeed, a linear dependence of output energy on pump pulse duration for fixed pump energy is demonstrated.
We have developed a versatile pulsed laser system for high precision magnetometry. The operating wavelength of the system can be configured to optically pump alkali vapors such as rubidium and cesium. The laser system consists of an auto-locked, interference filter stabilized, external cavity diode laser (ECDL), a tapered waveguide amplifier, and a pulsing module. The auto-locking controller can be used by an untrained operator to stabilize the laser frequency with respect to a library of atomic, molecular, and solid-state spectral markers. The ECDL output can be amplified from 20 mW to 2 W in continuous wave (CW) mode. The pulsing module, which includes an acousto-optic modulator (AOM), can generate pulses with durations of 20 ns and repetition rates of several MHz. Accordingly, the laser system is well suited for applications such as gravimetry, magnetometry, and differential absorption lidar. In this work, we focus on magnetometric applications and demonstrate that the laser source is suitable for optically pumping rubidium vapor. We also describe numerical simulations of optical pumping relevant to the rubidium D1 and D2 transitions at 795 nm and 780 nm respectively. These studies are relevant to the design and construction of a new generation of portable, rubidium, spin exchange relaxation-free (SERF) magnetometers, capable of sensitivities of 1 fT Hz-1/2 1.
Abstract : The Doppler-broadened two-photon absorption (TPA) cross-section for the 52S1/2- 52D5/2 transition in Rb is measured using direct absorption methods. A detailed model of the intensity profile was developed to account for a focused Gaussian beam propagating through a two-photon absorption medium. A peak absorbance of 24% was observed for an intensity of 6.28 kW/cm2 at the focus, a Rb density of 4.6 x 1015 cm-3 concentrations from 1.61-8.52 x 10(15) cm-3 line. Extracting the hyperfine-broadened TPA cross-section from 87 test configurations, while varying the pump power, alkali concentration and focal length, yielded an error weighted average of 6.75x10-21 cm4/W. This cross-section is sufficient for a pulsed dye laser to bleach the pump transition in the Two-Photon Pumped Alkali Laser (TPAL) that lases at 420 nm and 5.2 mum. Additionally, optically pumped atomic rubidium lasers pumped in the blue satellite of the D2 line from the ground Rb-Ar or Rb-Kr collision pair to the dissociative B2 sum 1/2 produce laser emission at 780.2 nm. Lasing is achieved for the Rb-Ar system and 757.1 - 760.4 nm for the Rb-Kr system. Slope efficiencies exceed 0.25% using a heat pipe configuration. The gain is very high with photon build-up times of 1-3.7 ns.