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Europhysics Letters (EPL)

Ultrasensitive two-photon spectroscopy based on long spin-relaxation time in a dark optical trap

Lev Khaykovich, Nir Friedman, Stanislav B. Baluschev, D. Fathi, Nir Davidson

Published May 15, 2000• 21 citations
Publisher

Abstract

We propose a new spectroscopic method for measuring weak transitions in cold and trapped atoms, which exploits the long spin relaxation times and tight spatial confinement offered by dark optical traps to achieve extremely high sensitivity. We demonstrate our scheme by measuring a 5 S 1/2 → 5 D 5/2 two-photon transition in cold Rb atoms trapped in a new single-beam dark optical trap, using an extremely weak probe laser power of 25 μW. We were able to measure transitions with as small excitation rate as < 0.1 s −1 , using 10 7 fold quantum amplification of the transition rate due to spin shelving and normalized detection with a strong cycling transition.

DOI
10.1209/epl/i2000-00291-y

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We propose a new spectroscopic method for measuring weak transitions in cold and trapped atoms, which exploits the long spin relaxation times and tight spatial confinement offered by dark optical traps to achieve extremely high sensitivity. We demonstrate our scheme by measuring a 5 S 1/2 → 5 D 5/2 two-photon transition in cold Rb atoms trapped in a new single-beam dark optical trap, using an extremely weak probe laser power of 25 μW. We were able to measure transitions with as small excitation rate as < 0.1 s −1 , using 10 7 fold quantum amplification of the transition rate due to spin shelving and normalized detection with a strong cycling transition.
Summary form only given. Utilizing cold and trapped atoms for precision spectroscopy of weak atomic transitions has two important advantages: the suppression of Doppler and time-of-flight broadenings and a combination of long interaction times, weak perturbations and tight confinement, which can be obtained using dark optical traps. We present a new and extremely sensitive method for measuring weak transitions with cold atoms in a dark optical trap, using electron shelving spectroscopy. Our scheme is based on a /spl Lambda/ system. Atoms with two ground states (for example, two hyperfine levels) are stored in the trap in a level that is coupled to the upper (excited) state, by an extremely weak transition. Atoms that undergo the weak transition may be shelved by a spontaneous Raman transition on the second ground level, which is uncoupled to the excited level by the measured photons. Finally, the detection scheme benefits from the multiply excited fluorescence of a strong closed transition from the uncoupled ground-state, that utilizes quantum amplification due to the electron shelving technique. We realized this scheme on a 5S/sub 1/2//spl rarr/5D/sub 5/2/ two-photon transition in cold and optically trapped /sup 85/Rb atoms.
We describe the apparatus of a dark-line two-dimensional (2D) magneto-optical trap (MOT) of (85)Rb cold atoms with high optical depth (OD). Different from the conventional configuration, two (of three) pairs of trapping laser beams in our 2D MOT setup do not follow the symmetry axes of the quadrupole magnetic field: they are aligned with 45° angles to the longitudinal axis. Two orthogonal repumping laser beams have a dark-line volume in the longitudinal axis at their cross over. With a total trapping laser power of 40 mW and repumping laser power of 18 mW, we obtain an atomic OD up to 160 in an electromagnetically induced transparency (EIT) scheme, which corresponds to an atomic-density-length product NL = 2.05 × 10(15) m(-2). In a closed two-state system, the OD can become as large as more than 600. Our 2D MOT configuration allows full optical access of the atoms in its longitudinal direction without interfering with the trapping and repumping laser beams spatially. Moreover, the zero magnetic field along the longitudinal axis allows the cold atoms maintain a long ground-state coherence time without switching off the MOT magnetic field, which makes it possible to operate the MOT at a high repetition rate and a high duty cycle. Our 2D MOT is ideal for atomic-ensemble-based quantum optics applications, such as EIT, entangled photon pair generation, optical quantum memory, and quantum information processing.
A differential two-photon spectroscopic technique for measurement of atomic temperatures in a working magneto-optical trap was demonstrated. We performed experimental and theoretical studies of two-photon resonances on Rydberg transitions 2S1/2−2P3/2−58S in cold Li7 atoms by using counter- and co-propagating laser beams. By analyzing the spectral shapes, a dependence of Rabi broadening and Doppler broadening on total intensity of cooling laser beams was obtained. We measured the temperature of Li7 atoms in the range from 0.25 to 0.75 mK. Our theoretical and experimental results are in reasonably good agreement. The developed approach for temperature measurements can be applied to cold atoms in different traps, including confined hydrogen and antihydrogen atoms.
We demonstrate confinement of 85Rb^{85}\mathrm{Rb}85Rb atoms in a dark, toroidal optical trap. We use a spatial light modulator to convert a single blue-detuned Gaussian laser beam to a superposition of Laguerre-Gaussian modes that forms a ring-shaped intensity null bounded harmonically in all directions. We measure a 1∕e1∕e1∕e spin-relaxation lifetime of $\ensuremath{\approx}1.5\phantom{\rule{0.3em}{0ex}}\mathrm{s}$ for a trap detuning of 4.0nm4.0\phantom{\rule{0.3em}{0ex}}\mathrm{nm}4.0nm. For smaller detunings, a time-dependent relaxation rate is observed. We use these relaxation rate measurements and imaging diagnostics to optimize trap alignment in a programmable manner with the modulator. The results are compared with numerical simulations.