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Optics Communications

Enhancement of stimulated Raman scattering by E-V energy transfer and laser deexcitation

Zhaolin Li, Guo-qing Zheng, Daozhong Zhang

Published Jun 1, 1993• 1 citation
Publisher
DOI
10.1016/0030-4018(93)90077-i

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We show that the sensitivity and robustness of a label-free optical imaging technique based on stimulated Raman scattering (SRS) can be enhanced by using resonant optical transitions in a Raman adiabatic passage scheme. Our approach is based on the consideration that any enhancement of the flow of energy between two light beams involved in the SRS process is related to an increase in atomic population transfer between the energy levels of interest. One can thus profit from techniques developed in quantum optics to maximize such atomic population transfer for enhancing the sensitivity and robustness of optical imaging techniques.
Impulsive stimulated Raman scattering (ISRS) plays a key role in coherent control of low-energy rotational resonances. Femtosecond laser pulses are widely employed to utilize ISRS because they are broadband and can cover the needed frequencies in a single pulse. Here, we show theoretically that the ISRS process is expressed as a linear response to the instantaneous Stokes parameters (ISPs) of the laser pulse. These IPSs expressed in rotational coordinates are then shown to be responsible for the angular momentum transfer from light to matter. These relationships have led to the designs of spectral profiles and polarization states of light pulses that should selectively excite particular rotational modes.