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Physical Review A

Inversionless lasing with self-generated driving field

Alexey A. Belyanin, Cleo L. Bentley, Federico Capasso, Olga A. Kocharovskaya, Marlan O. Scully

Published Jun 12, 2001• 27 citations
Publisher

Abstract

We propose and study resonant ladder schemes of inversionless lasing on a fast-decaying transition when the population inversion is not possible or very difficult to achieve. The driving field on a neighboring, slowly decaying transition is not imposed externally, but is self generated in the same active medium. Inversionless lasing in such schemes avoids the problem of driving-field absorption and leads to considerable reduction in the required pumping rate. Applications of such schemes include inversionless ultraviolet and soft x-ray lasing in gas lasers and inversionless generation of coherent mid/far-infrared emission on intersubband (interlevel) transitions in multiple quantum-well or quantum-dot laser diodes.

DOI
10.1103/physreva.64.013814

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Journal of Physics B Atomic Molecular and Optical Physics•Sep 21, 2020•2 citations
We propose and study resonant ladder schemes of inversionless lasing on a fast-decaying transition when the population inversion is not possible or very difficult to achieve. The driving field on a neighboring, slowly decaying transition is not imposed externally, but is self generated in the same active medium. Inversionless lasing in such schemes avoids the problem of driving-field absorption and leads to considerable reduction in the required pumping rate. Applications of such schemes include inversionless ultraviolet and soft x-ray lasing in gas lasers and inversionless generation of coherent mid/far-infrared emission on intersubband (interlevel) transitions in multiple quantum-well or quantum-dot laser diodes.
We have studied an incoherently pumped laser operating with a Doppler-broadened three-level system placed in a doubly resonant cavity. This system generates two laser fields, one of them without population inversion. Both ladder and V-type three-level schemes are considered with a ratio $R={\ensuremath{\omega}}_{\ensuremath{\alpha}}/{\ensuremath{\omega}}_{\ensuremath{\beta}}$ of inversionless laser frequency ${\ensuremath{\omega}}_{\ensuremath{\alpha}}$ to ordinary laser frequency ${\ensuremath{\omega}}_{\ensuremath{\beta}}$ of R=0.67R=0.67R=0.67 and R=1.88,R=1.88,R=1.88, respectively. Dual-wavelength lasing extends up to Doppler-broadening values for optical transitions of atoms in a vapor cell. Some considerations for the practical realization of this dual-wavelength laser are discussed.
We propose a new scheme for lasing without population inversion that utilizes interferences in double-quantum-well intersubband transitions. In contrast to the previous inversionless laser schemes based on atomic systems, the new proposal permits us to use band-gap engineering to choose the subband energies, coupling strengths, and decay rates, as desired, and permits us to create a laser system that does not require population inversion. We present detailed calculations on a specific scheme and discuss possible extensions.
A scheme for obtaining a laser without inversion in the deep X-ray regime is proposed based on the principle of gain without inversion. A ladder scheme is proposed in the Ar 8+ system. In this system, conventional lasing with population inversion in a neonlike scheme is used. This lasing field is proposed for the drive field on the higher transition of the ladder. A coherent field obtained in the high harmonics ultrashort laser provides the probe field to be amplified. The ground level is incoherently pumped into the highest level, while the latter is incoherently depumped into the ground level, at a different adjustable rate. A detailed density matrix calculation of the ladder configuration is performed [3], and the conditions under which the system exhibits inversionless gain, as well as regular gain, are derived. Numerical calculations in the bare state picture exhibits gain without inversion both at resonance and at the generalized Rabi side bands. The probe lineshape is shown to be constructed of two symmetrical dispersionlike features each centered at the generalized Rabi side bands. This is evidence of the quantum interference occurring at these locations and the basis for the gain without inversion.
A scheme for infrared generation without population inversion between subbands in quantum-well and quantum-dot lasers is presented. The scheme is based on the resonant nonlinear mixing of the optical laser fields on the two interband transitions that are generated in the same active region and that serve as the coherent drive for the infrared field. This mechanism for frequency down-conversion does not rely upon any ad hoc assumptions of long-lived coherences in the semiconductor active medium, and it should work efficiently at room temperature with injection current pumping. For optimized waveguide and cavity parameters, the intrinsic efficiency of the down-conversion process can reach the limiting quantum value corresponding to one infrared photon per one optical photon. Due to the parametric nature of infrared generation, the proposed inversionless scheme is especially promising for long-wavelength (far-infrared) operation.
A scheme for obtaining laser in the deep x-ray regime is proposed based on the principle of gain without inversion. A ladder scheme is proposed in Ar+8{\mathrm{Ar}}^{+8}Ar+8 system. In this system, conventional lasing with population inversion has been obtained in a neonlike fashion. This lasing field is proposed for the drive field on the higher transition of the ladder. A coherent field obtained in the high harmonics ultrashort laser provides the probe field to be amplified. This will be selected to best match the frequency needed for the transition from lower level of the present x-ray lasing to the ground state. Numerical calculations in the bare state picture exhibit possible gain at resonance, and at the Rabi side bands, for appropriate choice of system parameters, i.e., the strength of the driving field, the strength of the incoherent pump that provides the required energy needed for the inversionless amplification and the deexcitation rate. The latter rate is detrimental to lasing as it increases. It is quite interesting to note that the system exhibits surprisingly high stability for gain without inversion even for quite high rate of the incoherent deexcitation processes. Real and imaginary parts of the coherences were also obtained for detuned drive and probe fields. These provide insight into the role played by the quantum interference. The present theoretical calculations give high confidence in the quantum interference process as a candidate for realizing very short wavelength laser.
Abstract We show that it is possible to get gain without inversion at high frequency in a three-level ladder type scheme driven by a single driving laser. The transition from the ground state to first excited state is driven by a low-frequency resonant laser field. The next excited state lies far above the first one; therefore its resonant frequency can be much higher than that of the lower transition, and hence one should go beyond the most commonly used rotating wave approximation consisting of retaining only resonant terms (slowly oscillating) in the Hamiltonian. We solve the master equation, both analytically (under proper approximations) and numerically, with the full Hamiltonian keeping counter-rotating highly non-resonant terms. We show a dressed state picture explaining spectral features of gain-absorption profiles. Also we present a kind of phase diagram in the plane γ –Λ, where γ and Λ are spontaneous emission rate and incoherent pumping rate, respectively. The whole γ –Λ plane is divided into four areas: gain-inversion, absorption-no inversion, gain without inversion and absorption with inversion. The first two are usual regimes of incoherently pumped lasers, while the last two stem from the quantum interference phenomena. We analyse the parameter areas where such quantum regimes are possible. The exact numerical solution of the time-dependent master equation shows that keeping counter-rotating terms (no rotating wave approximation) gives rise to new spectral features in the form of additional peaks at combination frequencies. Actually the considered system works as a coherent frequency up-converter.