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Physical Review B

Exchange frequencies and magnetic ground state of Wigner crystal in anisotropic two-dimensional electron systems

Chenggang Zhou, R. N. Bhatt

Published Nov 20, 2006• 1 citation
Publisher

Abstract

We investigate the effect of mass anisotropy on the magnetic structure of the Wigner crystal of low-density electron systems in two dimensions at $T=0$. The multiparticle exchange frequencies are calculated with effective mass anisotropy, with and without concomitant lattice distortions. Numerical diagonalization of small lattice sizes with two-, three-, and four-spin exchange terms shows a transition from a ferromagnetic to an antiferromagnetic ground state with increasing mass anisotropy. We map out this transition at various electron densities.

DOI
10.1103/physrevb.74.205325

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CRC Press eBooks•Nov 2, 2010•1 citation
We investigate the effect of mass anisotropy on the magnetic structure of the Wigner crystal of low-density electron systems in two dimensions at T=0T=0T=0. The multiparticle exchange frequencies are calculated with effective mass anisotropy, with and without concomitant lattice distortions. Numerical diagonalization of small lattice sizes with two-, three-, and four-spin exchange terms shows a transition from a ferromagnetic to an antiferromagnetic ground state with increasing mass anisotropy. We map out this transition at various electron densities.
We consider a two-dimensional electron or hole system at zero temperature and low carrier densities, where the long-range Coulomb interactions dominate over the kinetic energy. In this limit the clean system will form a Wigner crystal. Nontrivial quantum-mechanical corrections to the classical ground state lead to multiparticle exchange processes that can be expressed as an effective spin Hamiltonian involving competing interactions. Disorder will destroy the Wigner crystal on large length scales, and the resulting state is called a Wigner glass. The notion of multiparticle-exchange processes is still applicable in the Wigner glass, but the exchange frequencies now follow a random distribution. We compute the exchange frequencies for a large number of relevant exchange processes in the Wigner crystal, and the frequency distributions for some important processes in the Wigner glass. The resulting effective low-energy spin Hamiltonian should be the starting point of an analysis of the possible ground-state phases and quantum phase transitions between them. We find that disorder plays a crucial role and speculate on a possible zero-temperature phase diagram.
The two-dimensional Wigner crystals are studied with the variational quantum Monte Carlo method. The close relationship between the ground-state wave function and the collective excitations in the system is illustrated, and used to guide the construction of the ground-state wave function of the strongly correlated solid. Exchange, correlation, and magnetic-field effects all give rise to distinct physical phenomena. In the absence of any external magnetic field, interesting spin orderings are observed in the ground state of the electron crystal in various two-dimensional lattices. In particular, two-dimensional bipartite lattices are shown not to lead necessarily to an antiferromagnetic ground state. In the quantum Hall effect regime, a strong magnetic field introduces energy and length scales. The magnetic field quenches the kinetic energy and poses constraints on how the electrons may correlate with each other. Care is taken to ensure the appropriate translational properties of the wave function when the system is in a uniform magnetic field. We have examined the exchange, intra-Landau-level correlation as well as Landau-level-mixing effects with various variational wave functions. We also determine their dependences on the experimental parameters such as the carrier effective mass at a modulation-doped semiconductor heterojunction. Our results, when combined with some recent calculations for the energy of the fractional quantum Hall liquid including Landau-level-mixing, show quantitatively that in going from n doping to p doping in GaAs/Alx{\mathrm{Al}}_{\mathit{x}}Alx​${\mathrm{Ga}}_{1\mathrm{\ensuremath{-}}\mathit{x}}$As heterojunction systems, the crossover filling factor from the fractional quantum Hall liquid to the Wigner crystal changes from filling factor \ensuremath{\nu}\ensuremath{\sim}1/5 to \ensuremath{\nu}\ensuremath{\sim}1/3. This lends strong support to the claim that the observed reentrant insulating phases around \ensuremath{\nu}=1/5 for n-doped and around \ensuremath{\nu}=1/3 for p-doped high-mobility samples are primarily caused by electron-electron interaction effects. We discuss the possible implications of our theoretical results for some recent experiments carried out in the quantum Hall regime in search of the electron solid.
What are the ground states of an interacting, low-density electron system? In the absence of disorder, it has long been expected that as the electron density is lowered, the exchange energy gained by aligning the electron spins should exceed the enhancement in the kinetic (Fermi) energy, leading to a (Bloch) ferromagnetic transition. At even lower densities, another transition to a (Wigner) solid, an ordered array of electrons, should occur. Experimental access to these regimes, however, has been limited because of the absence of a material platform that supports an electron system with very high quality (low disorder) and low density simultaneously. Here we explore the ground states of interacting electrons in an exceptionally clean, two-dimensional electron system confined to a modulation-doped AlAs quantum well. The large electron effective mass in this system allows us to reach very large values of the interaction parameter [Formula: see text], defined as the ratio of the Coulomb to Fermi energies. As we lower the electron density via gate bias, we find a sequence of phases, qualitatively consistent with the above scenario: a paramagnetic phase at large densities, a spontaneous transition to a ferromagnetic state when [Formula: see text] surpasses 35, and then a phase with strongly nonlinear current-voltage characteristics, suggestive of a pinned Wigner solid, when [Formula: see text] exceeds [Formula: see text] However, our sample makes a transition to an insulating state at [Formula: see text], preceding the onset of the spontaneous ferromagnetism, implying that besides interaction, the role of disorder must also be taken into account in understanding the different phases of a realistic dilute electron system.
Alexander Shashkin Institute of Solid State Physics, Chernogolovka, Moscow District 142432, Russia Sergey Kravchenko Physics Department, Northeastern University, Boston, Massachusetts 02115, U.S.A. Two-dimensional (2D) electron systems are realized when the electrons are free to move in a plane but their motion perpendicular to the plane is quantized in a confining potential well. Quantum phase transitions realized experimentally in such systems so far include metal-insulator transitions in perpendicular magnetic fields, metal-insulator transition in zero magnetic field, and a possible transition to a Wigner crystal. The first transition is governed by the externally controlled electron density or magnetic field, while the other two are governed by the electron density. At low electron densities in 2D systems, the strongly-interacting limit is reached because the kinetic energy is overwhelmed by the energy of electron-electron interactions. The interaction strength is characterized by the ratio between the Coulomb energy and the Fermi energy, r∗s = Eee/EF . Assuming that the effective electron mass is equal to the band mass, the interaction parameter r∗s in the single-valley case reduces to the Wigner-Seitz radius, rs = 1/(πns)1/2aB, and therefore increases as the electron density, ns, decreases (here aB is the Bohr radius in the semiconductor). Possible candidates for the ground state of the system include a Wigner crystal characterized by spatial and spin ordering [1], a ferromagnetic Fermi liquid with spontaneous spin ordering [2], a paramagnetic Fermi liquid [3], etc. In the strongly-interacting limit (rs 1), no analytical theory has been developed to date. According to numerical simulations [4], Wigner crystallization is expected in a very dilute regime, when rs reaches approximately 35. Refined numerical simulations [5] have predicted that prior to the crystallization, in the range of the interaction parameter 25 ≤ rs ≤ 35, the ground state of the system is a strongly correlated ferromagnetic Fermi liquid. At higher electron densities, rs ∼ 1, the electron liquid is expected to be paramagnetic, with the effective mass, m, and Lande´ g factor renormalized by interactions. Apart from the ferromagnetic Fermi liquid, other intermediate phases between the Wigner crystal and the paramagnetic Fermi liquid may also exist.