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Journal of Mathematical Physics

Binary Kernel Formulation of a Heisenberg Model of Ferromagnetism

Newton I. Greenberg

Published Mar 1, 1963• 6 citations
Publisher

Abstract

An ideal Heisenberg model of a ferromagnet for spin 12 is studied by considering the model in terms of a spin-deviation lattice gas. Utilizing the general methods of Yang and Lee, a binary kernel function is obtained in terms of which the thermodynamic properties of the lattice gas can be completely expressed. As an example, Dyson's results are rigorously obtained.

DOI
10.1063/1.1703967

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Physical review. B, Condensed matter•Feb 1, 1995•7 citations
An ideal Heisenberg model of a ferromagnet for spin 12 is studied by considering the model in terms of a spin-deviation lattice gas. Utilizing the general methods of Yang and Lee, a binary kernel function is obtained in terms of which the thermodynamic properties of the lattice gas can be completely expressed. As an example, Dyson's results are rigorously obtained.
The thermodynamic quantities of finite two- and three-dimensional ferromagnetic X Y -model such as 3×3 and 2×2×2 lattices have been calculated for the purpose of investigating the properties of liquid Helium II. The density dependence of the λ-line for the finite quantum lattice gas model agrees with the results of molecular field approximation and the experimental data of pure He 4 liquid near the λ-transition. The possibility of the occurrence of negative thermal expansion coefficient below the λ-point was roughly discussed with the use of the same consideration as the Ising model of Lee and Yang. The magnetization versus field curve tends to a step function when the temperature becomes smaller than the critical temperature estimated from the maximum of the specific heat. There exists a great difference between the pure isotropic Heisenberg model and X Y -model in the case of ferro-magnetic interaction at zero-temperature.
The Green's function formalism proposed by Kondo and Yamaji for low-dimensional spin systems with S =1/2 has been extended to the cases of S >1/2. We apply this formalism to the study of one- and two-dimensional Heisenberg ferromagnets over the whole temperature range. It is shown that our theory can reproduce the correct results obtained by the high-temperature expansion method. On the other hand, the results at low temperatures are similar to those of the modified spin-wave theory, which is considered to predict the low-temperature properties of such systems rather correctly. The gross behaviors of the calculated thermodynamic quantities of ferromagnetic Heisenberg chains agree with those obtained by the exact diagonalization method.
Abstract The infinite interaction range model (IIRM) for ferromagnetic systems is presented in its spin‐free formulation. In this formulation the states are labelled by partitions which provide a natural variable for thermodynamic computation. We have extended the calculations of Kittel and Shore by computing to a practical thermodynamic limit (N ∼ 100,000). The heat capacity, magnetic susceptibility and the magnetization of the first two functions exhibit a critical temperature while the magnetization is zero at zero field for all temperatures. Spontaneous magnetization is obtained by linear extrapolation from high field or equivalently by a polarized partition function. Relationships are explored among IIRM, the Heisenberg model and the mean field model. Application to IIRM of the Yang‐Lee condition for a phase transition yields a critical temperature identical to that obtained by the direct calculation.
Thermodynamic properties of the spin-1/2 Heisenberg ferromagnet are calculated by using Handscomb's Monte Carlo method. Several methods of analyses are used to determine critical properties of the model. For a square lattice we find that the susceptibility diverges exponentially at zero temperature. That is, \ensuremath{\chi}\ensuremath{\sim}exp[b(J/kB{\mathit{k}}_{\mathit{B}}kB​T)] with the constant b=4.5\ifmmode\pm\else\textpm\fi{}0.5, which is lower than the prediction (b=2\ensuremath{\pi}) of a modified spin-wave theory. For the simple-cubic lattice, we find that the critical temperature kB{\mathit{k}}_{\mathit{B}}kB​Tc{\mathit{T}}_{\mathit{c}}Tc​/J=1.68\ifmmode\pm\else\textpm\fi{}0.01, and the ratio of the exponents \ensuremath{\gamma}/\ensuremath{\nu}=2.0\ifmmode\pm\else\textpm\fi{}0.05, which are in good agreement with the estimates of the high-temperature series-expansion method.
The thermodynamic properties of the classical Heisenberg model on 3-d lattices are calculated in the approximation of the first order in 1/z (z is the number of nearest neighbours) which takes into account the two-point spin correlations resulting in the Gaussian fluctuations of the molecular field components. The numerical solution for the magnetization, susceptibility and the internal energy is valid in the whole plane (H, T) excluding the close vicinity of the critical point (| τ |≲ 1/z2) and agrees well with available series results. The extension of the method to the quantum case is proposed.
The one-dimensional spin-1/2 Ising-Heisenberg ferromagnets are studied by the Green's function method at finite temperatures. The Green's function is decoupled in terms of the correlation functions of 〈S0z{\mathit{S}}_{0}^{\mathit{z}}S0z​Snz{\mathit{S}}_{\mathit{n}}^{\mathit{z}}Snz​〉 and 〈S0+{\mathit{S}}_{0}^{+}S0+​${\mathit{S}}_{\mathit{n}}^{\mathrm{\ensuremath{-}}}$〉 under the constraint of 〈Sz{\mathit{S}}^{\mathit{z}}Sz〉=0, from which a set of self-consistent equations are derived and solved numerically. The thermodynamic properties such as internal energy, specific heat, and zero-field parallel susceptibility are calculated. Our results predict the correct behavior for the correlation functions and thermodynamic quantities in the entire temperature region, in agreement both with the exact numerical results on the finite chain and the experimental data.