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Optics Communications

Doppler-free monitoring of weak UV transitions by high frequency optical heterodyne three level spectroscopy

S. Le Boiteux, Daniel Bloch, M. Ducloy, A. Pesnelle, S. Runge, M. Perdrix

Published Dec 1, 1984• 8 citations
Publisher
DOI
10.1016/0030-4018(85)90226-3

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Optical heterodyne spectroscopy is one of the ultrasensitive and high resolution laser spectroscopies. During past years, it has extended from saturation absorption to two-photon transitions in a three level quantum system of atoms and ions. The particularly interesting case is the modulation transfer spectroscopy, where the optical heterodyne detection is performed via nearly degenerate four-wave mixing (NDFWM) in the nonlinear medium. In this report, the modulation transfer spectroscopy is used to observe the optical heterodyne saturation absorption and two-photon transition spectra simultaneously in Na2 without Doppler background. The line shapes of optical heterodyne signal are discussed in detail.