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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Peculiarities of dynamics of molecular multilevel systems in a powerful laser field: anaytical solutions

В. А. Савва, V. I. Zelenkov, O. V. Khlus

Published May 31, 2002• 0 citations
Publisher

Abstract

Analytical solutions of the equations describing coherent dynamics of various multilevel systems excited by radiation are given. The peculiarities of dynamics related with detuning from resonance, with arrangement and amount of levels, with dipole moment dependence on level number, along with excitation in a pulse laser field are studied.

DOI
10.1117/12.468920

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Analytical solutions of the equations describing coherent dynamics of various multilevel systems excited by radiation are given. The peculiarities of dynamics related with detuning from resonance, with arrangement and amount of levels, with dipole moment dependence on level number, along with excitation in a pulse laser field are studied.
A method based on the use of integral transform and orthogonal polynomials is presented to obtain the analytic solutions of the equations for coherent dynamics of multilevel quantum systems as simple molecular models describing molecule-radiation interactions in the high-power laser field and many other processes. As an example the Jacobi polynomials have been used and exact analytic solution has been obtained for dynamics of the family of multilevel Jacobi systems with both equidistant and nonequidistant energy levels, with various dependencies of dipole transition moments on energy, with both resonant and non-resonant laser excitation. Some special cases of the solution for definite systems from the family are given.
The Maxwell–Schrödinger equations describing the ultrashort laser pulse propagation in multilevel molecular media are shown to be analytically solvable and to reduce to nonlinear multisine-Gordon equations for certain models of the field–molecule system. Special cases of level schemes are shown to lead to soliton propagation. A numerical study is presented in order to examine the effect of nonresonant (virtual) transitions on pulse propagation and amplification in a three-level molecular system as a function of intensity and detuning.
A method to build various integrable models for description of coherent excitation of multilevel media by laser pulses is suggested. Distribution functions over the energy levels of quantum systems depending on the time and frequency detuning are obtained. The distributions follow from Schrödinger equation exact solutions and give the complete dynamical description of laser-excited quantum multilevel systems. Interpretation based on the Fourier spectra of the probability amplitudes of a quantum system is presented. The spectra are expressed in terms of orthonormal polynomials and their weight functions. Matrix elements of the dipole transitions between levels are equal to coefficients of the recurrence formula for the orthonormal polynomial system. Some examples are presented. The Kravchuk oscillator family as an integrable model is constructed to describe the coherent excitation dynamics of multilevel resonance media. It is based on the use of the Kravchuk orthogonal polynomials. The Kravchuk oscillator excitation dynamics is described by the binomial distribution of energy level populations and the distribution parameter depends on excitation conditions. Two known basic models in quantum physics -- the harmonic oscillator and two-level system are the special representatives of the Kravchuk oscillator family.
A pragmatic mechanism to obtain exact analytical solutions of equations describing the coherent dynamics of quantum multilevel systems by laser radiation is implemented. The technique shows interesting features and significant connections between different mathematical structures for constructing exact solutions for a large family of quantum systems, and is based on discrete orthogonal polynomials which are used to express the Fourier spectra of the probability amplitudes of an excited quantum system.