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Journal of the Physical Society of Japan

A Note on the Photon Echo Study of the Solvable Model of Microscopic Phase Modulation

Toshihico Arimitsu, Masashi Ban

Published Jan 1, 1984• 8 citations
Publisher

Abstract

The solvable model of the microscopic phase modulation, which was proposed previously by the authors, is investigated by the two-pulse photon echo.
DOI
10.1143/jpsj.53.74

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Two-pulse photon echo electron-nuclear double resonance (or PENDOR) has been used to measure the second-order hyperfine splittings in the ground state and the lowest component of the excited 1D2^{1}D_{2}1D2​ state of YAlO3{\mathrm{O}}_{3}O3​:Pr3+{\mathrm{Pr}}^{3+}Pr3+. The excited-state splittings are 0.923 and 1.565 MHz and are significantly different from previous hole-burning results because of greatly increased resolution. The mechanism for two-pulse PENDOR involves a modulation of the photon echo decay at the rf Rabi frequency. This modulation has been observed directly. A brief theoretical analysis is given which shows that the echo modulation is a result of phase and amplitude changes in the oscillating opitical dipole moment which are indirectly produced by the rf field.