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Optics Communications

A single-molecule interferometer for measurement of femtosecond laser pulse duration

Aleksandr V Vinogradov, József Janszky, Takashi Kobayashi

Published Jun 1, 1996• 2 citations
Publisher
DOI
10.1016/0030-4018(95)00709-1

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The paper explores the prospects of observing the phenomenon of dynamical Anderson localization via nonresonant Raman-type rotational excitation of molecules by periodic trains of short laser pulses. We define conditions for such an experiment and show that current femtosecond technology used for nonadiabatic laser alignment of linear molecules is sufficient for this task. Several observables which can serve as indicators for Anderson localization are suggested for measurement, and the influence of experimental limitations imposed by the laser intensity noise, finite pulse duration, limited number of pulses in a train, and thermal effects is analyzed.