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Physical review. B, Condensed matter

Kinetic theory of a normal quantum fluid. II. Transport properties

Charles D. Boley, Jeffrey B. Smith

Published Jun 1, 1978• 11 citations
Publisher

Abstract

Renormalized expressions for the transport coefficients of a normal quantum fluid are derived from a nonlocal kinetic equation. As was shown in the classical case by Forster and Martin and by R\'esibois, the expressions for the transport coefficients separate naturally into "kinetic" and "direct" parts. The kinetic terms are proportional to matrix elements of the inverse of the kinetic kernel, and have the same general structure as the "bare" transport coefficients obtained from a local Boltzmann equation. The direct terms are proportional to matrix elements of the kernel itself, and have no counterpart in calculations based on a local kinetic equation, as in the kinetic theory of gases. We evaluate the transport coefficients using the weak-coupling approximation to the kernel derived in a previous paper. Results are given, first, for both Bose and Fermi fluids at arbitrary temperature, and then for the Fermi fluid near $T=0$, where complete solutions are obtained. It is found that the direct parts of the shear viscosity and thermal conductivity are of higher order in $T$ than the kinetic parts, and are therefore negligible at very low temperature. The kinetic parts have the same leading temperature dependence as the predictions of the Landau theory. For the bulk viscosity, however, the direct and kinetic contributions begin at the same order (${T}^{2}$) in the temperature.

DOI
10.1103/physrevb.17.4260

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•Jan 1, 1981•0 citations
Renormalized expressions for the transport coefficients of a normal quantum fluid are derived from a nonlocal kinetic equation. As was shown in the classical case by Forster and Martin and by R'esibois, the expressions for the transport coefficients separate naturally into "kinetic" and "direct" parts. The kinetic terms are proportional to matrix elements of the inverse of the kinetic kernel, and have the same general structure as the "bare" transport coefficients obtained from a local Boltzmann equation. The direct terms are proportional to matrix elements of the kernel itself, and have no counterpart in calculations based on a local kinetic equation, as in the kinetic theory of gases. We evaluate the transport coefficients using the weak-coupling approximation to the kernel derived in a previous paper. Results are given, first, for both Bose and Fermi fluids at arbitrary temperature, and then for the Fermi fluid near T=0T=0T=0, where complete solutions are obtained. It is found that the direct parts of the shear viscosity and thermal conductivity are of higher order in TTT than the kinetic parts, and are therefore negligible at very low temperature. The kinetic parts have the same leading temperature dependence as the predictions of the Landau theory. For the bulk viscosity, however, the direct and kinetic contributions begin at the same order (T2{T}^{2}T2) in the temperature.
Close to equilibrium, a normal Bose or Fermi fluid can be described by an exact kinetic equation whose kernel is nonlocal in space and time. The general expression derived for the kernel is evaluated to second order in the interparticle potential. The result is a wavevector- and frequency-dependent generalization of the linear Uehling-Uhlenbeck kernel with the Born approximation cross section. The theory is formulated in terms of second-quantized phase space operators whose equilibrium averages are the n-particle Wigner distribution functions. Convenient expressions for the commutators and anticommutators of the phase space operators are obtained. The two-particle equilibrium distribution function is analyzed in terms of momentum-dependent quantum generalizations of the classical pair distribution function h(k) and direct correlation function c(k). The kinetic equation is presented as the equation of motion of a two -particle correlation function, the phase space density-density anticommutator, and is derived by a formal closure of the quantum BBGKY hierarchy. An alternative derivation using a projection operator is also given. It is shown that the method used for approximating the kernel by a second order expansion preserves all the sum rules to the same order, and that the second-order kernel satisfies the appropriate positivity and symmetry conditions.
In the linear-response regime, a normal Bose or Fermi fluid can be described by an exact kinetic equation whose kernel is nonlocal in space and time. We derive a general expression for this kernel and evaluate it explicitly to second order in the interparticle potential. The result is a wave-vector- and frequency-dependent generalization of the linear Uehling-Uhlenbeck kernel with the Born-approximation cross section. Our theory is developed in terms of a second-quantized form of the Wigner representation. Convenient expressions are obtained for the commutators and anticommutators of the phase-space density operators, and the equilibrium averages of these operators are analyzed in terms of momentum-dependent generalizations of the classical pair distribution function h(k)h(k)h(k) and direct correlation function c(k)c(k)c(k). The central quantity in this study is a two-particle equilibrium correlation function, the phase-space density-density anticommutator, whose Fourier transform $S(k\ensuremath{\omega}p{p}^{\ensuremath{'}})$ gives the symmetrized scattering function $S(k\ensuremath{\omega})$ by integration over the momenta. The kinetic equation is obtained by a formal closure of the quantum BBGKY hierarchy, with the nonlocal kernel expressed in terms of correlation functions involving two, three, and four particles. We show that our method for approximating the kernel and initial condition by a second-order expansion preserves all the sum rules of $S(k\ensuremath{\omega}p{p}^{\ensuremath{'}})$ to the same order and that the result satisfies the appropriate positivity and symmetry conditions.
We compute second-order transport coefficients of the dilute Fermi gas at unitarity. The calculation is based on kinetic theory and the Boltzmann equation at second order in the Knudsen expansion. The second-order transport coefficients describe the shear stress relaxation time, nonlinear terms in the strain-stress relation, and nonlinear couplings between vorticity and strain. An exact calculation in the dilute limit gives ${\ensuremath{\tau}}_{R}=\ensuremath{\eta}/P$, where ${\ensuremath{\tau}}_{R}$ is the shear stress relaxation time, $\ensuremath{\eta}$ is the shear viscosity, and PPP is pressure. This relation is identical to the result obtained using the Bhatnagar-Gross-Krook approximation to the collision term, but other transport coefficients are sensitive to the exact collision integral.
Motivated by the recently observed failure of the kinetic theory for the bulk viscosity, we in turn revisit the shear viscosity and the thermal conductivity of two-component fermions with a zero-range interaction both in two and three dimensions. In particular, we show that their Kubo formula evaluated exactly in the high-temperature limit to the lowest order in fugacity is reduced to the linearized Boltzmann equation. Previously, such a microscopic derivation of the latter was achieved only incompletely corresponding to the relaxation-time approximation. Here, we complete it by resuming all contributions that are naively higher orders in fugacity but become comparable in the zero-frequency limit due to the pinch singularity, leading to a self-consistent equation for a vertex function identical to the linearized Boltzmann equation. We then compute the shear viscosity and the thermal conductivity in the high-temperature limit for an arbitrary scattering length and find that the Prandtl number exhibits a nonmonotonic behavior slightly below the constant value in the relaxation-time approximation.
The memory kernel of the kinetic equation for the time correlation function of a quantum fluid is determined both in third order of the interaction strength and in the low-density approximation. The results are obtained with the help of a diagram representation for the kernel. The connexion with the kinetic theory for classical fluids is established. The properties of a nonequilibrium fluid may be studied with the help of the kinetic theory of time correlation functions. These functions are determined by specifying the memory kernel in the kinetic equation that governs their time evolution. For classical fluids a suitable formalism that permits the approximate evaluation of this kernel has been developed several years ago (for a review see ref. 1). The generalization of these methods to the case of quantum fluids was considered in a few recent papers2f3). In particular, the memory kernel was established for a normal quantum fluid in the weakcoupling approximation. In the long-time and large-distance limit this kernel reduces to that of the linearized Uehling-Uhlenbeck equation4) in which the scattering amplitude is replaced by its first Born approximation. The purpose of the present paper is to extend the available results by employing higher-order perturbation theory for the evaluation of the memory kernel. An essential ingredient of the treatment will consist in the introduction of four-point diagrams that represent the various contributions to the kernel. With the use of this diagram representation we shall derive the memory kernel in third order of the interaction strength. In this order the kernel still has the same general form as the weak-coupling kernel, but with shifted energies and a generalized transition probability. Its relation to the kernel of the linearized Bogoliubov-Gurov’) equation will be established. An alternative approach to the approximate evaluation of the memory kernel makes use of an expansion in the density. The low-density limit of the