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Physical review. B, Solid state

Self-Induced Transparency in Acoustic Paramagnetic Resonance

N. S. Shiren

Published Oct 1, 1970• 108 citations
Publisher

Abstract

Experiments on the propagation of microwave ultrasonic pulses through a resonant absorber are described. The principal features of self-induced transparency as described by McCall and Hahn for light pulses are observed. Quantitative measurements of pulse delay, output pulse width, energy, and area are in fair agreement with a calculation by Hopf which accounts approximately for the effect of the single reflection present in most of the experiments. Multiply reflected pulses exhibited linearly cumulative delay times, indicating constant reduced velocity during successive traversals through the absorber. Coherence-induced pulse breakup is shown to be a possible explanation of the pulse distortion and modulation observed in acoustic-paramagnetic-resonance experiments on ${\mathrm{Fe}}^{2+}$.

DOI
10.1103/physrevb.2.2471

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Self-Induced Transparency

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Above a critical power threshold for a given pulse width, a short pulse of coherent traveling-wave optical radiation is observed to propagate with anomalously low energy loss while at resonance with a two-quantum-level system of absorbers. The line shape of the resonant system is determined by inhomogeneous broadening, and the pulse width is short compared to dissipative relaxation times. A new mechanism of self-induced transparency, which accounts for the low energy loss, is analyzed in the ideal limit of a plane wave which excites a resonant medium with no damping present. The stable condition of transparency results after the traversal of the pulse through a few classical absorption lengths into the medium. This condition exists when the initial pulse has evolved into a symmetric hyperbolic-secant pulse function of time and distance, and has the area characteristic of a "$2\ensuremath{\pi}$ pulse." Ideal transparency then persists when coherent induced absorption of pulse energy during the first half of the pulse is followed by coherent induced emission of the same amount of energy back into the beam direction during the second half of the pulse. The effects of dissipative relaxation times upon pulse energy, pulse area, and pulse delay time are analyzed to first order in the ratio of short pulse width to long damping time. The analysis shows that the $2\ensuremath{\pi}$ pulse condition can be maintained if losses caused by damping are compensated by beam focusing. In an amplifying inhomogeneously broadened medium an analytic "$\ensuremath{\pi}$ pulse area" solution is presented in the limit of a sharp leading edge of the pulse. The dynamics of self-induced transparency are studied for the particular effects of Doppler velocities upon a resonant gas. The analysis of transparency for random orientations of dipole moments associated with degenerate rotational states yields modified forms of self-induced transparency behavior, which indicates a finite pulse energy loss as a function of distance in some cases. The effect of self-induced transparency on the photon echo is considered. Experimental observations of self-induced transparency have been made in a ruby sample at resonance with a pulsed ruby-laser beam. Single and multiple $2\ensuremath{\pi}$ pulse outputs have been observed, and pulse areas measured in the range of $2\ensuremath{\pi}$. The experimental results are compared with the predictions of the ideal-plane-wave theory. Deviations from the ideal-plane-wave theory are discussed. An analysis is made of the effect of a transverse mode of the propagating beam upon the transparency properties of the pulse.

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Self-induced transparency in self-chirped media

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Resonant absorbing media having many atoms within a cubic resonance wavelength can exhibit large frequency chirps in pulse propagation due to dipole-dipole interactions among the atoms. Analytic solutions are obtained for invariant pulse propagation in such a medium consisting of interacting two-level atoms. Departures from the McCall-Hahn results include nonhyperbolic secant pulse shapes and different than 2π-area pulses. In addition, the excitation of the medium is comparatively suppressed for the same group velocity. The results are interpreted to suggest new experiments.

Optics Communications•Aug 1, 1988•51 citations
Experiments on the propagation of microwave ultrasonic pulses through a resonant absorber are described. The principal features of self-induced transparency as described by McCall and Hahn for light pulses are observed. Quantitative measurements of pulse delay, output pulse width, energy, and area are in fair agreement with a calculation by Hopf which accounts approximately for the effect of the single reflection present in most of the experiments. Multiply reflected pulses exhibited linearly cumulative delay times, indicating constant reduced velocity during successive traversals through the absorber. Coherence-induced pulse breakup is shown to be a possible explanation of the pulse distortion and modulation observed in acoustic-paramagnetic-resonance experiments on Fe2+{\mathrm{Fe}}^{2+}Fe2+.
Above a critical power threshold for a given pulse width, a short pulse of coherent traveling-wave optical radiation is observed to propagate with anomalously low energy loss while at resonance with a two-quantum-level system of absorbers. The line shape of the resonant system is determined by inhomogeneous broadening, and the pulse width is short compared to dissipative relaxation times. A new mechanism of self-induced transparency, which accounts for the low energy loss, is analyzed in the ideal limit of a plane wave which excites a resonant medium with no damping present. The stable condition of transparency results after the traversal of the pulse through a few classical absorption lengths into the medium. This condition exists when the initial pulse has evolved into a symmetric hyperbolic-secant pulse function of time and distance, and has the area characteristic of a "$2\ensuremath{\pi}$ pulse." Ideal transparency then persists when coherent induced absorption of pulse energy during the first half of the pulse is followed by coherent induced emission of the same amount of energy back into the beam direction during the second half of the pulse. The effects of dissipative relaxation times upon pulse energy, pulse area, and pulse delay time are analyzed to first order in the ratio of short pulse width to long damping time. The analysis shows that the $2\ensuremath{\pi}$ pulse condition can be maintained if losses caused by damping are compensated by beam focusing. In an amplifying inhomogeneously broadened medium an analytic "$\ensuremath{\pi}$ pulse area" solution is presented in the limit of a sharp leading edge of the pulse. The dynamics of self-induced transparency are studied for the particular effects of Doppler velocities upon a resonant gas. The analysis of transparency for random orientations of dipole moments associated with degenerate rotational states yields modified forms of self-induced transparency behavior, which indicates a finite pulse energy loss as a function of distance in some cases. The effect of self-induced transparency on the photon echo is considered. Experimental observations of self-induced transparency have been made in a ruby sample at resonance with a pulsed ruby-laser beam. Single and multiple $2\ensuremath{\pi}$ pulse outputs have been observed, and pulse areas measured in the range of $2\ensuremath{\pi}$. The experimental results are compared with the predictions of the ideal-plane-wave theory. Deviations from the ideal-plane-wave theory are discussed. An analysis is made of the effect of a transverse mode of the propagating beam upon the transparency properties of the pulse.
Self-induced transparency has been studied in detail experimentally for a simple two-level atomic absorption. A Hg II laser pulse is used at resonance with the D1{D}_{1}D1​ line of Rb. This system eliminates many previous experimental problems such as nonuniform wave fronts and degenerate off-resonant absorbers. Nonlinear transmission, pulse delays, pulse breakup, peak amplification, incoherent-decay effects, off-resonance effects, and focusing effects have been observed. Quantitative comparison with theory is obtained by computer solutions which include the incoherent decay and optical-pulse shapes of the Hg-Rb system. Good agreement is obtained with the theory of McCall and Hahn. Pulse compression by an order of magnitude is obtained by focusing in the resonant absorber. The theory predicting preferred pulse widths and velocities proposed by Davidovich and Eberly is discussed and found inappropriate for the Hg-Rb and other similar systems.
The waveguide propagation of a microwave magnetic field pulse at electron paramagnetic resonance (EPR) with a free radical sample of electron spins distributed along the guide displays the phenomenon of self-induced transparency (SIT). Predictions of plane-wave optical SIT are modified by summation of the magnetic-moment-microwave-field coupling over the transverse waveguide mode for specific sample geometries. Mode modified pulse area theorems are presented. Observed output pulse areas and shapes are compared with computer predictions. After pulse propagation over several absorption lengths a spontaneous zero-area pulse propagation effect is observed for a short weak input pulse with spectral width comparable to or larger than the spin-resonance linewidth. Alternating 180\ifmmode^\circ\else\textdegree\fi{} phase shifts in the pulse carrier wave, accounting for zero area, signify magnetic dipole transitions which alternate between coherent absorption and emission to some extent, and therefore anomalous pulse propagation is observed. For pulses applied off-resonance, linear and nonlinear shifts of the average carrier frequency occur toward the center of the spin resonance.
A review is given of the investigations of the coherent interaction of light pulses with resonantly absorbing two-level media. An analysis is made of the self-induced transparency discovered by McCall and Hahn and of its importance in quantum electronics. Bleached states associated with the phase modulation are considered in detail. A comparison is made with the theory of nonlinear waves of different physical origin. A review is given of some possible physical applications associated with the discriminatory nature of the transmission and delay of light in the self-induced transparency effect.
A systematic perturbation expansion with respect to the small parameter ${(\ensuremath{\Delta}\ensuremath{\tau}\ensuremath{\omega})}^{\ensuremath{-}1}$, $\ensuremath{\Delta}\ensuremath{\tau}$ being the duration of the pulse and $\ensuremath{\omega}$ the optical frequency, is introduced. This method is applied to the problem of self-induced transparency for sharp-line absorbers at exact resonance. Corrections to the McCall and Hahn solution are obtained which describe the propagation of the form-preserving pulse with modulated frequency and slightly changed shape, group velocity, and wave vector. Earlier results by Marth, Holmes, and Eberly on phase modulation and wave-vector shift are confirmed.
Resonant absorbing media having many atoms within a cubic resonance wavelength can exhibit large frequency chirps in pulse propagation due to dipole-dipole interactions among the atoms. Analytic solutions are obtained for invariant pulse propagation in such a medium consisting of interacting two-level atoms. Departures from the McCall-Hahn results include nonhyperbolic secant pulse shapes and different than 2π-area pulses. In addition, the excitation of the medium is comparatively suppressed for the same group velocity. The results are interpreted to suggest new experiments.