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ISRN Optics

Probability Densities for Fluorescent Photons Emitted by a Two-State Atom Driven by a Laser

Robertsen A. Riehle, Henk F. Arnoldus

Published Dec 11, 2012• 1 citation
Publisher

Abstract

Fluorescent photons emitted by a two-state atom in a laser beam are correlated. We have obtained the probability density for the emission of the th photon after a random initial time . It is shown that the correlations between the photons lead to a deviation from the poissonian value for this function (the probability density for independent events), although the deviation is not as significant as one may expect.

DOI
10.5402/2012/745871

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Fluorescent photons emitted by a two-state atom in a laser beam are correlated. We have obtained the probability density for the emission of the th photon after a random initial time . It is shown that the correlations between the photons lead to a deviation from the poissonian value for this function (the probability density for independent events), although the deviation is not as significant as one may expect.
We study the general properties of the photon statistics of fluorescence radiation, emitted by a two-level atom in a strong laser field and a perturber bath. We investigate the deviation of the factorial moments from a Poisson distribution, and we show that for long counting times the lowest-order correction can be expressed entirely by the quantity Q, which represents the deviation of the variance from the average. We introduce and evaluate the quantities gn(t), which serve as a measure for the deviation of the higher-order statistics from Poissonian statistics. Subsequently we obtain explicit expressions for the average waiting time for the appearance of the n th photon, after an arbitrary initialization of the counting process. It turns out that the average time delay is again determined by Q. Hence this parameter can be measured in a photon-counting experiment, which involves only the observation of a single photon, rather than an (in principle) infinite number of photons.
Statistics of fluorescence photons emitted by a single two-level atom interacting with a continuous wave laser field are analyzed. The photon-counting distribution is calculated for the so-called intermediate fluorescence photons, i.e., those counted during the time interval between instants at which photons are emitted. The result is a sub-Poissonian (narrower than Poisson) distribution, which agrees with experimental observations. This intermediate-photon distribution is used to calculate the average number of fluorescence photons, the second factorial moment of the photon-counting distribution, and Mandel’s Q parameter commonly used to evaluate the deviation of photon statistics from the Poisson distribution. The theoretical expressions obtained for moments of the intermediate-photon distribution are different from well-known Mandel’s formulas.
We have studied the statistics of fluorescent photons emitted by a two-state atom in a laser beam in the limit where either the detuning or the Rabi frequency is large. For this case, the spectrum of resonance fluorescence has three separated lines. We have obtained closed form expressions for the conditional probability density for the emission of the nth photon and for the probability for emission of n photons in a time interval [0,T]. Our solutions are complementary to the known solutions for the case of perfect resonance.
The photon correlations of resonance fluorescence emitted by a degenerate two-level atom near a metal surface are studied. An intense non-monochromatic optical laser drives a low-lying atomic transition, and the emitted fluorescence is detected by a photon counter. An expression for the spontaneous decay operator is derived, and it appears that the various substates of the upper level have a different lifetime due to the presence of the surface, or equivalently, due to the loss of spherical symmetry. The temporal photon correlation function is then evaluated in terms of a photon-emission operator and the time evolution operator for the atomic density matrix. The general theory is exemplified with a detailed elaboration of the j/sub g/ = 0 yields j/sub e/ = 1 transition, for which the two-photon correlation is obtained explicitly as a function of the lifetime A(h), depending on the atom surface distance h, the laser linewidth, the detuning from resonance, and the dipole-coupling strength with the external field.
Abstract We discuss the statistics of emission of photons by a single atom or ion illuminated by a laser beam at the frequency of quasi-resonance between two energy levels, a situation that corresponds to real experiments. We extend this to the case of two laser beams resonant with the energy differences between two excited levels and the ground state (three level atom in V-configuration). We use a novel approach to this type of problem by considering a Kolmogorov equation for the probability distribution of the atomic state, which takes into account first the deterministic evolution of this state under the effect of the incoming laser beam and second the random emission of photons during the spontaneous decay of the excited state(s) to the ground state. This approach yields solvable equations in the two level atom case. For the three level atom case we set the problem and clearly define its frame. The results obtained are valid in both opposite limits of rare and frequent spontaneous decay, compared to the period of the optical Rabi oscillations due to the interaction between resonant excitation and atomic levels. Our analysis gives access to various statistical properties of the fluorescence light, including one showing that its fluctuations in time are not invariants under time reversal. This result makes evident the fundamentally irreversible character of quantum measurements, represented here by the emission of photons of fluorescence.
The fluorescence radiation, emitted by a two-level atom in a perturber bath, is considered. The atom is driven by a single-mode laser with a Lorentzian profile, which is brought about by a fluctuating phase. The stochastics of this phase is taken to be the Markovian random-jump process. The authors derive explicit expressions for the atomic density matrix, the temporal photon correlations and the fluorescence spectrum. The results greatly resemble the results for a non-Gaussian diffusive phase, but deviate slightly from the corresponding expressions in the Wiener-Levy limit of the diffusion process.