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Physical Review A

Single-photon pulse propagation in and into a medium of two-level atoms: Microscopic Fresnel equations

P. R. Berman, C. H. Raymond Ooi

Published Dec 30, 2011• 3 citations
Publisher

Abstract

The propagation of an off-resonant, single-photon pulse in and into a medium of two-level atoms is considered. When the pulse is launched from within the medium, there are two propagation speeds, neither of which is the normal group velocity. For densities as small as 10${}^{11}$ atoms/cm${}^{3}$ and detunings of order 10${}^{11}$ s${}^{\ensuremath{-}1}$, both propagation speeds approach one half the speed of light in vacuum. Moreover, rather remarkably, there are Rabi oscillations between the field and atomic excitation, even for this single-photon pulse. In contrast, for a pulse sent into the medium, the atom-field system remains adiabatically in a dressed state that propagates with the normal group velocity. In the limit that the index of refraction is approximately equal to unity, we obtain the Fresnel equations for the reflection and transmission coefficients based on this microscopic model. The transmission coefficient differs from the conventional result owing to the fact that we quantize the field in free space.

DOI
10.1103/physreva.84.063851

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The propagation of an off-resonant, single-photon pulse in and into a medium of two-level atoms is considered. When the pulse is launched from within the medium, there are two propagation speeds, neither of which is the normal group velocity. For densities as small as 1011{}^{11}11 atoms/cm3{}^{3}3 and detunings of order 1011{}^{11}11 s\ensuremath−1{}^{\ensuremath{-}1}\ensuremath−1, both propagation speeds approach one half the speed of light in vacuum. Moreover, rather remarkably, there are Rabi oscillations between the field and atomic excitation, even for this single-photon pulse. In contrast, for a pulse sent into the medium, the atom-field system remains adiabatically in a dressed state that propagates with the normal group velocity. In the limit that the index of refraction is approximately equal to unity, we obtain the Fresnel equations for the reflection and transmission coefficients based on this microscopic model. The transmission coefficient differs from the conventional result owing to the fact that we quantize the field in free space.
By comparing the numerical solutions of Maxwell-Bloch equations beyond and within the slowly-varying envelope approximation and the rotating-wave approximation for the propagation of a few-cycle pulse laser in a resonant two-level atom medium, we found that both the Rabi flopping and the refractive index, and subsequently the carrier and the propagation velocity of the few-cycle pulse, are closely connected with the time-derivative behaviour of the electric field. This is because the Rabi flopping is such that the soliton pulse splits during propagation and that a shorter pulse propagates faster than a broader one.
The refractive index of a system is often viewed as the collective response of a medium to an electromagnetic field. Nevertheless, even if targeted at a single atom, the incoming light undergoes the dispersion. By studying the propagation of a single photon interacting with a two-level atom, we examine the dispersion behavior, calculate the phase and group velocity of the photon wave packet, and further analyze the dispersion experienced by the photon. These findings are critical for advancing long-distance quantum communications.
The propagation of a weak-field pulse through a medium of three-level atoms is considered. Each atom has a $\ensuremath{\Lambda}$-type level scheme in which the two lower levels are stable. A strong control field drives one of the electronic transitions while the signal field drives the coupled transition under conditions where EIT (electromagnetically induced transparency) is usually operative. The input pulse is slowed and compressed as it enters the medium, adiabatically following the EIT solution. However, if the control field is changed suddenly when the pulse is in the medium, the signal field is transformed into two pulses, one of which propagates as a normal EIT pulse and the other with a different speed and an amplitude that oscillates in time. The temporal oscillations are transformed into both spatial and temporal oscillations as the pulse exits the medium. An analytic expression is derived for the pulse intensity which provides a good approximation to the exact result at all times. It is shown that the oscillating component of the exiting pulse can be spatially compressed in comparison with the input pulse.
Coherent propagation of a circularly polarized pulse which is two-photon quasi-resonant with a medium of multi-level atoms is considered in the adiabatic following limit. The relevant pair of non-linear coupled partial differential equations are solved exactly for arbitrary pulse shapes. The development of the envelope and the phase of the pulse as it propagates through the medium is described analytically. Perturbation theoretical results are shown to apply only for small intensity or small distance of propagation or both. Qualitatively different results apply for higher intensities and longer distances of propagation. These include strong self-phase-modulation effects as well as reshaping of the pulse envelope.
We describe the interaction of two two-level atoms in free space with propagating modes of the quantized electromagnetic field, using the time-dependent Heisenberg-Langevin method. For single- photon pulses, we consider the effect of the pulse's spatial and temporal profiles on the atomic excitation. In particular, we find the ideal shape for a pulse to put exactly one excitation in any desired state of the bi-atomic system. Furthermore, we analyze the differences in the atomic dynamics between the cases of Fock state pulses and coherent state pulses.
A quantum theory of formation and propagation of superfluorescence and Stokes pulses in samples of small Fresnel numbers is presented. Linearized Maxwell-Heisenberg equations for the system of two-level atoms and a quantized electromagnetic field are solved analytically in the second-order Debye approximation. Under this approximation paths of rays which undergo one reflection from the sides of the sample and those which propagate without reflections are studied. We point out that due to guiding effects, if the Fresnel number is smaller than unity, the contribution from totally reflected rays is not negligible with respect to that from nonreflected rays. This leads to the interference between reflected and nonreflected rays which affects spatial properties of superfluorescence and Stokes pulses. Moreover, as a consequence of guiding effects, the spectral density of light becomes asymmetric and shifted from the atomic resonance frequency.