Solid-state sources capable of emitting single photons on demand are of great interest in quantum information applications. Ideally, such a source should emit exactly one photon into the collection optics per trigger, the emitted photons should be indistinguishable, and the source should be electrically driven. Several design strategies addressing these requirements have been proposed. In the cavity-based source, light emission is controlled using resonant cavity quantum electrodynamics effects, whereas in the waveguide-based source, broadband electric field screening effects are employed to direct the light emission into the optical mode of interest. For all the strategies, accurate modeling and careful optical engineering is required to achieve high performance. In this study, we discuss the models and numerical techniques used to analyze such structures. The physical effects governing the light emission profile and the possibilities of tailoring it as well as the mechanisms governing the coherence are elucidated. The major design strategies pursued to optimize the single-photon source performance and the remaining challenges are reviewed.
Solid-state sources capable of emitting single photons on demand are of great interest in quantum information applications. Ideally, such a source should emit exactly one photon into the collection optics per trigger, the emitted photons should be indistinguishable and the source should be electrically driven. Several design strategies addressing these requirements have been proposed. In the cavity-based source, light emission is controlled using resonant cavity quantum electrodynamics effects, whereas in the waveguide-based source, broadband electric field screening effects are employed to direct the light emission into the optical mode of interest. For all the strategies, accurate modeling and careful optical engineering is required to achieve high performance.
This chapter reviews the characteristic figure of merits of the deterministic single-photon source (SPS) based on a quantum emitter in a semiconductor solid-state system. SPS is a solid-state device capable of emitting single photons on demand. The most fundamental characteristic of the SPS is that it should emit only one photon at a time. This ability is tested in the so-called Hanbury, Brown, and Twiss experiment. A second characteristic for the SPS is that the emitted photons should be quantum mechanically indistinguishable, meaning that the emitted photons should have the same wavelength, phase variation across the pulse, polarization, optical mode profile, etc. The third important characteristic of the SPS is its efficiency or brightness. The ideal SPS should be deterministic and provide single photons on demand. It should act as a "single-photon gun" such that every trigger releases exactly one photon into the collection optics. A major workhorse for generating single photons has been the spontaneous parametric down-conversion process.
The development of single-photon sources has been nothing but rapid in recent years, with quantum emitter-based systems showing especially impressive progress. In this article, we give an overview of the developments in single-photon sources based on single molecules. We will introduce polycyclic hydrocarbons as the most commonly used emitter systems for the realization of an organic solid-state single-photon source. At cryogenic temperatures this special class of fluorescent molecules demonstrates remarkable optical properties such as negligible dephasing, indefinite photostability, and high photon rates, which make them attractive as fundamental building blocks in emerging quantum technologies. To better understand the general properties and limitations of these molecules, we discuss sample preparation and relevant emitter parameters such as absorption and emission spectra, lifetime, and dephasing. We will also give an overview of light extraction strategies as a crucial part of a single-photon source. Finally, we conclude with a look into the future, displaying current challenges and possible solutions.