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Journal of Low Temperature Physics

Dissociation Dynamics of Ultracold Atom-Molecule Mixtures in an Optical Lattice

Takahiko Miyakawa, Pierre Meystre

Published May 30, 2007• 2 citations
Publisher
DOI
10.1007/s10909-007-9408-8

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The quantum dynamics of an ultracold diatomic molecule tunneling and diffusing in a one-dimensional optical lattice exhibits unusual features. While it is known that the process of quantum tunneling through potential barriers can break up a bound-state molecule into a pair of dissociated atoms, interference and reassociation produce intricate patterns in the time-evolving site-dependent probability distribution for finding atoms and bound-state molecules. We find that the bound-state molecule is unusually resilient against break up at ultralow binding energy Eb{E}_{b}Eb​ (Eb{E}_{b}Eb​ much smaller than the barrier height of the lattice potential). After an initial transient, the bound-state molecule spreads with a width that grows as the square root of time. Surprisingly, the width of the probability of finding dissociated atoms does not increase with time as a power law.
The quantum dynamics of an ultracold diatomic molecule tunneling and diffusing in a one-dimensional optical lattice exhibits unusual features. While it is known that the process of quantum tunneling through potential barriers can break up a bound-state molecule into a pair of dissociated atoms, interference and reassociation produce intricate patterns in the time-evolving site-dependent probability distribution for finding atoms and bound-state molecules. We find that the bound-state molecule is unusually resilient against break up at ultralow binding energy Eb (Eb much smaller than the barrier height of the lattice potential). After an initial transient, the bound-state molecule spreads with a width that grows as the square root of time. Surprisingly, the width of the probability of finding dissociated atoms does not increase with time as a power law.
We consider the photodissociation of ground-state bosonic molecules trapped in an optical lattice potential into a two-component gas of fermionic atoms. The system is assumed to be described by a single-band resonantly coupled Bose-Fermi Hubbard model. We show that in the strong fermion-fermion interaction limit the dissociation dynamics is governed by a spin-boson lattice Hamiltonian. In the framework of a mean-field analysis based on a generalized Gutzwiller ansatz, we then examine the crossover of the dissociation from a regime of independent single-site dynamics to a regime of cooperative dynamics as the molecular tunneling increases. We also show that in the limits of weak and strong intersite tunneling the mean-field solutions agree well with the results from the quantum optical Jaynes-Cummings and Tavis-Cummings models, respectively. Finally, we identify two types of self-trapping transitions, a coherent and an incoherent one, depending on the ratio of the repulsive molecule-molecule interaction strength to molecular tunneling.