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Physical Review Letters

Collective Spin Oscillations in Spin-Polarized Gases: Spin-Polarized Hydrogen

Laurent P. Lévy, Andrei E. Ruckenstein

Published Apr 23, 1984• 87 citations
Publisher

Abstract

The spin dynamics of weakly interacting, spin-polarized quantum gases are discussed in terms of a quasiparticle picture of these systems. Quantum mechanical exchange between identical particles introduces "molecular" magnetic fields which give rise to the precession of the spin current; this in turn leads to coherent oscillations of the magnetization. The theory is used to discuss magnetic resonance experiments in spin-polarized atomic hydrogen.

DOI
10.1103/physrevlett.52.1512

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The spin dynamics of weakly interacting, spin-polarized quantum gases are discussed in terms of a quasiparticle picture of these systems. Quantum mechanical exchange between identical particles introduces "molecular" magnetic fields which give rise to the precession of the spin current; this in turn leads to coherent oscillations of the magnetization. The theory is used to discuss magnetic resonance experiments in spin-polarized atomic hydrogen.
We derive the linearized spin dynamics for paramagnetic quantum liquids. In these systems, the existence of quantum-mechanical exchange in the presence of (an externally induced) broken symmetry in spin space gives rise to a coherent precession of the spins damped by diffusion. Such collective oscillations occur as a result of the precession of the spin current about a macroscopic local exchange field generated either by an external polarizing magnetic field (as in dilute nondegenerate spin-polarized gases) or by the long-lived nonequilibrium polarization (as in degenerate Fermi liquids). We use a unified approach based on the Kadanoff-Baym formulation of the kinetic equations to describe these phenomena. The connection between strongly and weakly interacting paramagnetic systems is made obvious by considering two special cases: (1) a weakly interacting spin-polarized quantum gas and (2) a parametrization of strongly correlated degenerate Fermi liquids in terms a weakly interacting gas of ``quasiparticles.'' Transport coefficients are calculated with a novel method which may be generalizable to systems with no translational invariance.
The identical spin rotation effect is the quantum mechanical collisional effect underlying the transverse nuclear spin waves recently seen in dilute non degenerate gases in Paris [3He] and at Cornell University [H↓]. This mechanism could in principle give rise, at low enough temperatures, to hydrodynamic oscillatory modes associated with any non diagonal elements of the atomic internal density matrix (generalized spin waves or coherences waves). Starting from a quantum Boltzmann equation recently derived for the study of 4-component atomic hydrogen, we show that the current of any transverse quantity (hyperfine or Zeeman coherence) does indeed precess around molecular exchange fields. Unhappily, in most cases, the oscillatory modes associated with these transverse quantities are heavily damped. The first intrinsic cause of damping of these waves is spin exchange. We study the conditions under which this damping is minimized in both zero field and in high magnetic field. Numerical values of all relevant parameters for the description of spin transport properties in atomic hydrogen are given in the appendices.
Spin-polarized, atomic hydrogen at temperatures below 1K shows promise of becoming the first physically realizable example of a degenerate, weakly interacting Bose gas. Because of the hyperfine structure of the hydrogen atom the Bose condensed state is expected to exhibit novel magnetic properties such as spin wave excitations of the superfluid and possibly a coherent precessing, spontaneous magnetization. This paper discusses a variety of theoretical problems which arise in the study of atomic hydrogen gas. Theories are presented for spin relaxation of the hyperfine levels and for the recombination of H-atoms into H2 molecules. The problem of the binding of H atoms to a surface of superfluid 4He is reviewed together with the theory of surface superfluidity in the hydrogen film proposed by Edwards and Mantz. Finally we consider the problem of superfluidity in the bulk atomic hydrogen gas. We describe the theory of Siggia and Ruckenstein of double Bose condensation into the two lowest hyperfine states and speculate about the possible observable consequences of this phenomenon.
Abstract : With the production of polar molecules in the quantum regime, long-range dipolar interactions are expected to facilitate understanding of strongly interacting many-body quantum systems and to realize lattice spin models for exploring quantum magnetism. In ordinary atomic systems, where contact interactions require wavefunction overlap, effective spin interactions on a lattice can be mediated by tunnelling, through a process referred to as superexchange; however, the coupling is relatively weak and is limited to nearest-neighbour interactions. In contrast, dipolar interactions exist even in the absence of tunnelling and extend beyond nearest neighbours. This allows coherent spin dynamics to persist even for gases with relatively high entropy and low lattice filling. Measured effects of dipolar interactions in ultracold molecular gases have been limited to the modification of inelastic collisions and chemical reactions. Here we use dipolar interactions of polar molecules pinned in a three-dimensional optical lattice to realize a lattice spin model. Spin is encoded in rotational states of molecules that are prepared and probed by microwaves. Resonant exchange of rotational angular momentum between two molecules realizes a spin-exchange interaction. The dipolar interactions are apparent in the evolution of the spin coherence, which shows oscillations in addition to an overall decay of the coherence. The frequency of these oscillations, the strong dependence of the spin coherence time on the lattice filling factor and the effect of a multipulse sequence designed to reverse dynamics due to two-body exchange interactions all provide evidence of dipolar interactions. Furthermore, we demonstrate the suppression of loss in weak lattices due to a continuous quantum Zeno mechanism. Measurements of these tunnelling-induced losses allow us to determine the lattice filling factor independently.