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Comptes Rendus Physique

Dynamics of fluctuations in non-Markovian systems

Daniel Alonso, Inés de Vega, E. Hernández-Concepción

Published Jun 1, 2007• 2 citations
Publisher

Abstract

The dynamics of multiple time correlation functions (MTCFs) of a system in contact with a non-Markovian environment is relevant in many different contexts. In this article we study the dynamical equations that satisfy MTCFs of a system and how they are used to characterize its fluctuations. The non-Markovian character of the interaction between the system and its environment leads to dynamical equations different from those derived from the Quantum Regression Theorem. We further discuss an stochastic method to compute MTCFs. To illustrate the theory we apply it to the evaluation of the emission spectrum of an atom in contact with a non-Markovian environment. The emission spectrum strongly depends on the way the environment reacts to the absorption of a photon emitted by the atom.

DOI
10.1016/j.crhy.2007.05.019

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AIP conference proceedings•Jan 1, 2010•0 citations
The dynamics of multiple time correlation functions (MTCFs) of a system in contact with a non-Markovian environment is relevant in many different contexts. In this article we study the dynamical equations that satisfy MTCFs of a system and how they are used to characterize its fluctuations. The non-Markovian character of the interaction between the system and its environment leads to dynamical equations different from those derived from the Quantum Regression Theorem. We further discuss an stochastic method to compute MTCFs. To illustrate the theory we apply it to the evaluation of the emission spectrum of an atom in contact with a non-Markovian environment. The emission spectrum strongly depends on the way the environment reacts to the absorption of a photon emitted by the atom.
We derive the dynamical equation of the reduced propagator, an object that evolves state vectors of the system conditioned to the dynamics of its environment, which is not necessarily in the vacuum state at the initial time. Such a reduced propagator is essential to obtain multiple-time correlation functions (MTCFs). We also study the evolution of MTCFs within the weak-coupling limit and show that the quantum regression theorem is, in general, not satisfied. We illustrate the theory in two different cases: first, solving an exact model, and, second, presenting the results of the numerical integration for a system coupled with a thermal environment through a nondiagonal interaction.
Beyond the conventional quantum regression theorem, a general formula for non-Markovian correlation functions of arbitrary system operators both in the time- and frequency-domain is given. Weapproach the problem by transforming the conventional time-non-local master equation into dispersed time-local equations-of-motion. The validity of our approximations is discussed and we find that the non-Markovian terms have to be included for short times. While calculations of the density matrix at short times suffer from the initial value problem, a correlation function has a well defined initial state. The resulting formula for the non-Markovian correlation function has a simple structure and is as convenient in its application as the conventional quantum regression theorem for the Markovian case. For illustrations, we apply our method to investigate the spectrum of the current fluctuations of interacting quantum dots contacted with two electrodes. The corresponding non- Markovian characteristics are demonstrated.
Beyond the conventional quantum regression theorem, a general formula for non-Markovian correlation functions of arbitrary system operators both in the time- and frequency-domain is given. We approach the problem by transforming the conventional time-non-local master equation into dispersed time-local equations-of-motion. The validity of our approximations is discussed and we find that the non-Markovian terms have to be included for short times. While calculations of the density matrix at short times suffer from the initial value problem, a correlation function has a well defined initial state. The resulting formula for the non-Markovian correlation function has a simple structure and is as convenient in its application as the conventional quantum regression theorem for the Markovian case. For illustrations, we apply our method to investigate the spectrum of the current fluctuations of interacting quantum dots contacted with two electrodes. The corresponding non-Markovian characteristics are demonstrated.
We investigate non-Markovianity measure using two-time correlation functions for open quantum systems. We define non-Markovianity measure as the difference between the exact two-time correlation function and the one obtained from quantum regression theorem in the Born-Markov approximation. Such non-Markovianity can easily be measured in experiments. We found that the non-Markovianity dynamics in different time scale crucially depends on the system-environment coupling strength and other physical parameters such as the initial temperature of the environment and the initial state of the system. In particular, we obtain the short-time and long-time behaviors of non-Markovianity for different spectral densities. We find that the thermal fluctuation always reduce the non-Markovian memory effect. Also, the non-Markovianity measure shows nontrivial initial state dependence in different time scales.
In the present Thesis we study the behavior of multi-time correlation functions and of thermodynamical quantities such as heat in open quantum systems undergoing an evolution generally affected by the presence of memory effects, i.e. non-Markovian. In the last decade, a large part of the scientific community in this field has dedicated its efforts to the understanding, precise definition and quantification of non-Markovianity in the quantum realm and now we have at our disposal several benchmark results and a plethora of different estimators that allow to determine the degree of non-Markovianity of a given dynamics. It comes therefore natural to investigate how other different dynamical quantities relate to such estimators also in order to understand the physical implications of memory effects on the statistics of observable quantities. In the first part of this work, a quantitative test of the violation of the so-called quantum regression theorem in presence of a non-Markovian dynamical regime is investigated. The quantum regression theorem represents a procedure that, whenever valid, allows to reconstruct two-time correlation functions of system's operators from the sole knowledge of the dynamics of mean values. It is worth stressing that two-time correlation functions are necessary in order to fully characterize the statistical properties of a quantum system, since they are able to catch aspects of the dynamics, such as fluorescence spectrum, in general not accessible looking at mean values. Despite their relevance however, obtaining two-time correlation functions often represents a formidable task, since the knowledge of the full "system+environment" dynamics is required, a generally too demanding request in the context of open quantum systems theory. The quantum regression theorem represents in this regard the easiest route to determine two-time correlation functions, this highlighting its importance. In this work we show that, in a pure-dephasing spin-boson model, the quantum regression theorem represents a stronger condition than non-Markovianity, in the sense that any presence of memory effects in the reduced dynamics inevitably results in violations to the former. These results have been published in [G.Guarnieri, A. Smirne, B. Vacchini, Phys. Rev. A 90, 022110 (2014)]. The second part of the Thesis is devoted to the characterization of heat ow at the microscopic level in open quantum systems, both finite and infinite dimensional. In particular we begin by studying the time behavior of its mean value in a non-Markovian dynamical regime, showing that, at variance with what happens in the Born-Markov semigroup limiting case, heat can backflow from the environment to the system. After providing a condition for the occurrence of such phenomenon and a measure for its amount for a given dynamics, the relationship with suitable non-Markovianity estimators is sought in two paradigmatic models, namely the spin-boson and the quantum brownian motion. The results, collected in [ G. Guarnieri, C. Uchiyama, B. Vacchini, Phys. Rev. A 93, 012118 (2016); G. Guarnieri, J. Nokkala, R. Schmidt, S. Maniscalco, B. Vacchini, Phys. Rev. A 94, 062101 (2016)], on the one hand allow for the identification of parameter-regions where the heat backflow is absent or maximum. On the other hand they show that the occurrence of heat backflow represents a stricter condition than non-Markovianity, in the sense that non-Markovianity allows for the observation of heat flowing back from the environment to the system and, vice versa, a Markovian dynamics prevents its occurrence. This Thesis concludes with the formulation of a new family of lower bounds to the mean dissipated heat in an environmental-assisted erasure-protocol scenario where Landauer's principle applies. As originally conceived for classical systems, this principle states that every irreversible erasure of information stored in a system inevitably carries along an amount of heat dissipated into the environment which is expended to perform the action. Within the framework recently put forward in [D. Reeb, M. M. Wolf, New J. Phys. 16, 103011 (2014)], which guarantees the validity of Landauer's principle in an open quantum systems scenario, we provide an asymptotically tight family of lower bounds to the dissipated heat which are also valid in the non-equilibrium setting. This construction is applied to an open system consisting of a three-level V-system, in which one transition is externally pumped by a laser field while the other is coupled through an XX-interaction to an environment consisting of a spin chain. Beside calculating all these quantities, an exact solution for the dynamics of such system is also provided. These results are collected in [G. Guarnieri, S. Campbell, J. Goold, S. Pigeon, M. Paternostro, B. Vacchini, in preparation].
Open quantum systems are often encountered in many different physical situations. From quantum optics to statistical mechanics, they are fundamental in the understanding of a great variety of different phenomena. Some of the most common examples are the relaxation to equilibrium, the existence of nonequilibrium stationary states, and the dynamics of atoms in interaction with electromagnetic fields. A crucial step in the analysis is to consider the quantum open system and its environment as the two mutually interacting components of a larger isolated system. Thereafter, the so‐called Markov approximation is often considered, which consists on assuming that the time scales associated to the dynamics of the quantum open system are larger than those of the environment. It is the interplay of the different time scales associated with the system and the environment what determines the validity of the different approximations made. In this paper we will discuss the dynamics of a open quantum system in contact with a reservoir when the Markov approximation is not valid, and we have to include some non‐Markovian or memory effects.