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Quantum Electronics

Anisotropy of nonlinear absorption in a V3+: YAG crystal

Nikolai N Il'ichev, А. V. Kiryanov, Pavel P Pashinin, V. A. Sandulenko, Alexander V. Sandulenko, S M Shpuga

Published Dec 31, 1995• 11 citations
Publisher

Abstract

An investigation was made of the polarisation characteristics of the nonlinear absorption of λ = 1.055 μm radiation in a V 3+ : YAG crystal at the saturation stage. The duration of a pulse propagating in the crystal was considerably less than the lifetime of an excited state of the V 3+ impurity centres. A comparison of the experimental results with those of a theoretical calculation showed that the best description was provided by a phenomenological model in which resonant absorption in a crystal is attributed to three linear dipoles oriented along the main crystallographic axes of YAG.

DOI
10.1070/qe1995v025n12abeh000554

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An investigation was made of the polarisation characteristics of the nonlinear absorption of λ = 1.055 μm radiation in a V 3+ : YAG crystal at the saturation stage. The duration of a pulse propagating in the crystal was considerably less than the lifetime of an excited state of the V 3+ impurity centres. A comparison of the experimental results with those of a theoretical calculation showed that the best description was provided by a phenomenological model in which resonant absorption in a crystal is attributed to three linear dipoles oriented along the main crystallographic axes of YAG.
An investigation was made of changes in the profile and state of polarisation of a short (25 ns) resonant light pulse (λ ~ 1.06 μm) during its propagation in a YAG : Cr4+ crystal. The experimental results were in good agreement with a theory in which the absorption of light by the Cr4+ impurity centres in a YAG crystal is described phenomenologically as a consequence of the interaction of light with three orthogonal groups of resonant linear dipoles. The result demonstrated the fleasibility of controlling the profile of a light pulse propagating through polariser — YAG : Cr4+ crystal — polariser system. The application of a single-frequency pulse to this system generated output pulses with two or three intensity maxima. This was a direct result of a self-induced change in the state of the polarisation of the light in the YAG : Cr4+ crystal at the saturation absorption stage.
Saturation absorption experiments are conducted on the title compound at 1.064 μm with laser light propagating along both the [001] and [111] crystallographic axes. Rotation of the crystals about these axes during the experiments reveals that the transmission of the polarized 1.064 μm radiation is highly anisotropic in the saturation regime. The details of the anisotropy and saturation curves are explained using a simple model of subsets of optical centers along with a relevant set of rate equations. The ground and excited-state absorption cross sections at 1.064 μm are calculated to be σgs=5.7(±2)×10−18 cm2 and σes=8(±2)×10−19 cm2, respectively, and the optimum crystallographic orientation for utilization in optical devices is discussed.
We studied both experimentally and theoretically the transmission and polarization characteristics of a Cr4+ : YAG saturable absorber crystal as a function of the intensity and polarization state of an incident laser beam. We found that a birefringent absorption behaviour is induced and we show that the experimental results are well described by a full numerical model which includes excited-state absorption as well as a ground-state cross-absorption term. By using pump-probe measurements we show that a finite cross-saturation of the absorption is achieved along the crystal axes orthogonal to the polarization of the optical radiation. No induced refractive index birefringence is observed.
A model of degenerate four-wave mixing (DFWM) in Cr4+:YAG saturable absorbers is given in the transient regime. Because of the presence of absorbing dipoles oriented along specific directions, the DFWM process exhibits an anisotropic behavior. The effects of pump beam fluences, relative polarization of the beams, crystal orientation, absorbance, excited-state absorption, and nonresonant losses are analyzed. The theoretical results are supported by DFWM experiments in Cr4+:YAG performed at 1.06 µm with nanosecond pulses.
A mathematical model describing the dynamic emission of intracavity polarized isotropic Cr 4+ :YAG solid--state saturable absorber was developed.This model considers double pumping laser pulses to simulate the actions of Cr 4+ :YAG as a dual Q-switched crystal (1.06 µm) and lasing medium (1.4 µm).The model describes the time evolution of interaction between the pumping laser pulse, partial polarizer and the polarized saturable absorber.The analysis of the polarization process is based on the assumption that at each moment of lasing evolution, the state of polarization represented by an eigenstate corresponds to the lowest radiation losses state.The model offers a simple mechanism for studying the kinetics of the pulsed lasers and the influence of the variations of the pumping laser power and nonlinear anisotropy parameter on the characteristics of the output laser pulses 1.06 µm and 1.4 µm.The angular rotation of the passive switch Cr 4+ :YAG reveals that the transmission of the polarized 1.06 µm laser radiation is strongly anisotropic in the saturation regime.The suggested model estimates the transmission of pumping laser density of the polarized light 1.06 µm radiation as a function of nonlinear anisotropy parameter, temporal behavior of the relative population inversion of Nd-laser, population inversion of the different polarized levels of Cr 4+ :YAG pulsed laser and the output laser pulse densities under impact of different values of the nonlinear anisotropy which is due to the self-induced anisotropy of its saturated absorption.
We describe a theory of four-wave mixing in the saturable absorber Cr4+:YAG{\mathrm{Cr}}^{4+}:\mathrm{Y}\mathrm{A}\mathrm{G}Cr4+:YAG and compare with experiments performed at 1.064 \ensuremath{\mu}m wavelength. We show that the strong polarization dependence of the saturable absorption along orthogonal crystallographic axes leads to unique polarization properties for wave mixing in Cr4+:YAG{\mathrm{Cr}}^{4+}:\mathrm{Y}\mathrm{A}\mathrm{G}Cr4+:YAG. Also there are a range of conditions that lead to vector phase conjugation of the polarization state of a signal beam. Optimum reflectivity for vector phase conjugation occurs when the pump beams have either orthogonal circular polarizations or parallel linear polarizations at 45\ifmmode^\circ\else\textdegree\fi{} to the crystallographic axes. The latter case is unique to this type of nonlinearity.