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Europhysics Letters (EPL)

Observation of polarized neutron interference in spin space

Fokko M. Mulder, Сергей Валентинович Григорьев, Wicher H. Kraan, M.Th. Rekveldt

Published Jul 1, 2000• 7 citations
Publisher

Abstract

The coherent superposition of particle quantum states resulting from different spatial paths shows well-known interference effects. Another type of interference is Larmor precession, which can be described as neutron wave interference in spin space, i.e. interference on the same spatial path. Here we show several new manifestations of interference phenomena of the latter type. The interference is produced by coherent population of different I z = ±½ spin states in a polarized neutron beam between two resonant radio-frequency (RF) spin flippers. Their spin flip probability, and thus the occupation numbers of the spin states, can be tuned between 0 and 1 by changing the RF amplitude. This leads to interference effects in the polarization since the energy exchanged between the RF field and spin yields different phase evolution in the spatial parts of the neutron states. Depending on the preparation of the initial neutron states, five values for the time-independent phase difference between the final neutron states can be observed.

DOI
10.1209/epl/i2000-00332-7

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The coherent superposition of particle quantum states resulting from different spatial paths shows well-known interference effects. Another type of interference is Larmor precession, which can be described as neutron wave interference in spin space, i.e. interference on the same spatial path. Here we show several new manifestations of interference phenomena of the latter type. The interference is produced by coherent population of different I z = ±½ spin states in a polarized neutron beam between two resonant radio-frequency (RF) spin flippers. Their spin flip probability, and thus the occupation numbers of the spin states, can be tuned between 0 and 1 by changing the RF amplitude. This leads to interference effects in the polarization since the energy exchanged between the RF field and spin yields different phase evolution in the spatial parts of the neutron states. Depending on the preparation of the initial neutron states, five values for the time-independent phase difference between the final neutron states can be observed.
Neutron resonance spin-echo (NRSE) phenomena are investigated experimentally and theoretically. In our experiments, spin precession produced in a classical manner and by neutron resonance is combined as two arms of a spin-echo machine. A magnetic-field scan in the classical SE coil reveals a spin-echo signal of the precession produced by the NRSE arm. The neutron spin-flip probability $\ensuremath{\rho}$ in the resonance coils turns out to be a key parameter of the NRSE arm. The limiting cases $\ensuremath{\rho}=0$ and $\ensuremath{\rho}=1$ lead, respectively, to Larmor precession with phase ${\ensuremath{\varphi}}_{1}$ in the static magnetic fields of the NR flippers or to NRSE precession with ${\ensuremath{\varphi}}_{2}.$ The case $0<\ensuremath{\rho}<1$ produces quantum interference resulting in additional echoes with phases ${\ensuremath{\varphi}}_{3}=({\ensuremath{\varphi}}_{1}+{\ensuremath{\varphi}}_{2})/2$ and ${\ensuremath{\varphi}}_{4}=\ifmmode\pm\else\textpm\fi{}({\ensuremath{\varphi}}_{1}\ensuremath{-}{\ensuremath{\varphi}}_{2})/2.$ The amplitude of each pattern depends on the spin-flip probability $\ensuremath{\rho}$ and the initial polarization. These experiments demonstrate explicitly the quantum-mechanical principle of linear spin state superposition of neutron particle waves, and the interference as a result of that.
The observation of the 4π symmetry of spinor wave functions was one of the first and highly debated neutron interference experiments. Polarized neutrons have been used to verify the spin-superposition principle on a macroscopic level when the spin in one beam path is inverted with respect to the other one. This results in a spin polarization perpendicular to both initial spins. When a Rabi flipper is used the final spin polarization rotates in this perpendicular plane with the Larmor frequency of the flipper field. Thus, it produces a “frozen” Larmor spin rotation in free space. In this case the spin-flip is associated with an energy (photon) transfer which causes this effect. A magnetic Josephson effect-like situation exists when spin-flippers with slightly different resonance frequencies are used in both beam paths. When such a spin reversal is done in both beam paths a magnetic Josephson effect analog has been realized which shows a remarkably high energy resolution. Multiphoton exchange can be achieved when off-resonance fields are used.
Neutron resonance spin echo phenomena, produced by resonance coils with adiabatic passage of the neutron spin, are investigated experimentally and theoretically. The adiabatic passage of the neutron spin through a resonance coil requires a specific configuration of the magnetic field. The solution of the Schr\"odinger equation, obtained for the required configuration, shows the probability of a spin-flip process; it also shows the phase shift, which the neutron experienced, when it flies through it. The precession phase inside the coil consists of three contributions in the rotating frame approach. The first, biggest contribution is the phase of the rotating frame ${\ensuremath{\omega}}_{0}\ensuremath{\tau}.$ The second is the precession phase of the neutron spin in the rotating frame since it follows adiabatically the effective field as seen in this frame. The third, smallest contribution is Berry's phase since the magnetic field rotates over an angle approaching $\ensuremath{\pi}$ in this rotating frame. This rotation is followed adiabatically by the neutron spin. Finally, the amplitude of the interference pattern and the phase shift between the neutron-spin states are derived for a system consisting of two such flippers. The theoretical consideration is experimentally confirmed.
Neutron-multiwave-interference phenomena based on Ramsey's resonance method of ``separated oscillating fields'' are studied. A neutron passes through N successive resonant coils $(\ensuremath{\Elzxh}{\ensuremath{\omega}}_{0}=2{\ensuremath{\mu}}_{n}{B}_{0}),$ which flip the neutron spin with a probability $\ensuremath{\rho}$ smaller than 1. These coils are separated by path lengths L over which a homogeneous field B1{B}_{1}B1​ is present. Because the spin-flip probability $\ensuremath{\rho}$ is smaller than 1, the number of waves for a neutron is doubled after each flipper, so as to produce 2N{2}^{N}2N neutron waves at the end of the setup. The phase difference between any pair of waves is a multiple of a ``phase quantum'' determined by the line integral of the field difference ${B}_{1}\ensuremath{-}{B}_{0}$ over the length L. Highly regular patterns of the quantum-mechanical probability R in ${(B}_{1},\ensuremath{\rho})$ space appear due to pair interference between individual waves. Possible applications of this phenomenon, such as a direct measurement of n-particle correlation function, are pointed out.
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We consider the neutron-optical phenomena that emerge during the coherent interaction of a neutron with a sample when the neutron spin precesses in a magnetic field. As follows from general considerations, such an interaction gives rise to an extra precession phase, which is added to the Larmor precession phase. This phenomenon can be interpreted as a manifestation of the time delay due to a finite time of the neutron-sample interaction. The Larmor neutron spin precession with a constant frequency serves as a clock for measuring this time delay. We used such a clock to directly measure the difference between the neutron velocity in matter and its vacuum value. We also present the results of the first experiments in which Larmor clocks were used to measure the neutron tunneling time in the resonance of a quasi-bound state and the Bragg diffraction time. Prospects for further applications of the method are discussed.