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Science

Experimental Verification of Decoherence-Free Subspaces

Paul G. Kwiat, Andrew J. Berglund, Joseph B. Altepeter, Andrew G. White

Published Oct 20, 2000• 520 citations
Publisher

Abstract

Using spontaneous parametric down-conversion, we produce polarization-entangled states of two photons and characterize them using two-photon tomography to measure the density matrix. A controllable decoherence is imposed on the states by passing the photons through thick, adjustable birefringent elements. When the system is subject to collective decoherence, one particular entangled state is seen to be decoherence-free, as predicted by theory. Such decoherence-free systems may have an important role for the future of quantum computation and information processing.

DOI
10.1126/science.290.5491.498

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Using spontaneous parametric down-conversion, we produce polarization-entangled states of two photons and characterize them using two-photon tomography to measure the density matrix. A controllable decoherence is imposed on the states by passing the photons through thick, adjustable birefringent elements. When the system is subject to collective decoherence, one particular entangled state is seen to be decoherence-free, as predicted by theory. Such decoherence-free systems may have an important role for the future of quantum computation and information processing.
Decoherence-free states protect quantum information from collective noise, the predominant cause of decoherence in current implementations of quantum communication and computation. Here we demonstrate that spontaneous parametric down conversion can be used to generate four-photon states which enable the encoding of one qubit in a decoherence-free subspace. The immunity against noise is verified by quantum state tomography of the encoded qubit. We show that particular states of the encoded qubit can be distinguished by local measurements on the four photons only.
Multipartite entangled states are key elements for quantum information processing. Here we experimentally investigate the particular properties of a polarization-entangled four-photon state, which can be generated directly by second order parametric down-conversion. The perfect correlations and the invariance under local transformations enable one to encode one qubit of quantum information in a decoherence-free subspace and thus to communicate it safely over noisy quantum channels. Furthermore, we present an experimental method to detect genuine fourpartite entanglement using entanglement witness operators. The implementation of such operators requires only of few local polarization measurements but uniquely proves the genuine multipartite entanglement.
The nascent field of quantum information offers the promise of dramatic speed increases for certain types of computation and logical protocols which are classically impossible. The phenomenon of nonlocality is fundamental to this study, and polarization-entangled photons o er a clean, bright, and stable system for its experimental investigation. This thesis investigates, both experimentally and theoretically, the creation, manipulation, and measurement of polarization-entangled photon pairs. Our entangled photon pairs are created through spontaneous parametric down-conversion within a pair of adjacent, orthogonally oriented nonlinear crystals. The quality and brightness of this source is then dramatically improved through the use of birefringent crystals which compensate for an angle-dependent phase shift. The use of these compensation crystals has allowed measured count rates of two million pairs per second with 97.7% fidelity (with a maximally entangled state) or alternately, ten thousand pairs per second with 99.5% fidelity. By manipulating these entangled states, it is possible to study both how they change and how they can be used. We discuss the theory of state manipulation and the experimental implementation of extremely precise single-qubit operations. To study the operations themselves, we use quantum process tomography to characterize them and have successfully implemented the first experimental realization of ancilla-assisted process tomography. To study decoherence, we implemented the first experimental decoherence-free subspace. By using techniques developed during these investigations, we are able to transform our source of entangled photons into a source of any two-photon polarization state, mixed or pure. Developing new techniques for state creation and manipulation is possible because of simultaneous development in state measurement. In addition to detailing both a theoretical analysis and experimental instructions for state tomography, we experimentally and theoretically compared state tomography with tests of local realism (Bell inequalities) and entanglement witnesses (an entanglement detection technique). In the process, we have measured the largest violations of local realism to date, both statistical (over 2400-sigma) and absolute (S = 2:826 ± 0:005 -- within 0:2% of a maximal violation).
Developing techniques for characterizing quantum mechanical systems has been a major topic of research, especially in recent years, as quantum technologies, such as quantum communication and quantum cryptography, have grown to become an important asset in modern society. Although techniques such as quantum state tomography is an effective method to characterize a system consisting of two-level systems, the characterization of continuous degree of freedom such as space or frequency stills represents a time-consuming task as the state space scales exponentially with the dimension of the system. In this work, we show an indirect approach for measuring properties of high-dimensional degrees of freedom by coupling them to two-dimensional subsystems that can be measured efficiently via quantum state tomography. In our case, the property of interest is the correlation factor of the joint spectral amplitude describing the two-photon frequency states, which are coupled to the polarization degree of freedom using a completely positive trace-preserving map, called a dephasing channel. The action of the map on the polarization state induces a decoherence effect that depends on the initial frequency state, thus allowing to retrieve information about the frequency correlation factor by only measuring the decoherence in the polarization state. In the experimental part, we produced a pair of photons using spontaneous parametric down-conversion and characterized the joint spectral intensity with stimulated emission tomography. The decoherence was controlled with a birefringent material that acts as a dephasing channel. The polarization state was measured after the dephasing channel for two different initial frequency configurations using quantum state tomography. The bounds for the frequency correlation factor were calculated from the fidelity of the two polarization states and the generalized data processing inequality. The results of this work show that the polarization decoherence can be used as a tool to measure the frequency correlation factor of the joint spectral amplitude.
There is interest in using photon entanglement in biomedical applications. In one application, polarization entangled photons pass through brain tissue. The effect of the brain tissue on the photon entanglement is measured via the decoherence that is imparted on the entangled state. Our current method to obtain a measure of the decoherence involves quantum state tomography, where a minimum of 16 measurements are used in conjunction with tomographic optimization to obtain the density matrix representing the state of the photons. In this work we report on a method to avoid tomographic optimization on behalf of a direct measurement of the elements of the density matrix. We make preliminary comparisons between the two methods.
We describe experiments with photon pairs to evaluate, correct for, and avoid sources of error in optical quantum information processing. It is well known that a simple beamsplitter can non-deterministicially prepare or select entangled polarization states. We use quantum process tomography (QPT) to fully characterize this effect, including loss and decoherence. The QPT results identify errors and indicate how well they can be corrected. To evade decoherence in a noisy quantum channel, we identify decoherence-free subspaces using experimental channel characterization, without need for a priori knowledge of the decoherence mechanism or simplifying assumptions. Working with pairs of polarization-encoded photonic qubits, we use tomographic and adaptive techniques to identify 2- and 3-state decoherence-free subspaces for encoding decoherence-free qubits and qutrits within the noisy channel.