A comparison is reported of the observed spectral narrowing of amplified spontaneous emission from dye amplifiers with predictions from a dynamical model based on rate equations. This is employed to develop a generally applicable method of determining the unsaturated gain within the dye medium. Comparison is made with another technique for determining gain over the restricted pumping range for which it is applicable. The matching of theory to experiment is sufficiently sensitive that good values can also be determined for the wavelength dependence of the excited singlet state absorption cross section.
A comparison is reported of the observed spectral narrowing of amplified spontaneous emission from dye amplifiers with predictions from a dynamical model based on rate equations. This is employed to develop a generally applicable method of determining the unsaturated gain within the dye medium. Comparison is made with another technique for determining gain over the restricted pumping range for which it is applicable. The matching of theory to experiment is sufficiently sensitive that good values can also be determined for the wavelength dependence of the excited singlet state absorption cross section.
A new method for determining the gain in high gain amplifiers is reported. The technique only requires measurements of the relative intensity and the output spectral width of the amplified spontaneous emission from the amplifier as a function of input pumping. The results of an experimental test of this technique using a flashlamp-pumped rhodamine 6G dye amplifier are described. Simple approximate analytical models are used to compare with experiment thereby determining the gain. The results are found to be in good agreement with both more accurate gain measurements and an alternative technique which can be applied over a restricted range of operational parameters.
The major purpose of the work described in this thesis is the experimental and theoretical study of the amplification of the spontaneous emission in dye amplifiers. This work falls into three distinct sections: (a) the study of high-current short-pulse flashtubes operating in (or near) the ablation regime; (b) the study of the amplification process of the spontaneous emission in a homogeneously broadened medium, such as a dye material, in the thin cell case, where there is no variation of the pumping across the cell; and, (c) the study of the amplification of the spontaneous emission in the thick cell case, where gain and index of refraction inhomogeneities exist across the cell thickness. In each case, we have developed theoretical models and compared their predictions with the experimental results. In particular, for the ablation-type flashlamps, it is shown that their behaviour is well represented by an analysis in which the discharge plasma is supposed to radiate as a blackbody at the temperature of the plasma. This model accounts for the fact that the light output from a flashlamp saturates whereas the current does not, provides a more accurate value for the plasma resistivity as a function of temperatures and gives a useful design criterion for determining the physical dimensions of an ablation-type flashlamp. With respect to the amplification of the spontaneous emission in a thin cell, it is mainly shown that (i) the spontaneous emission propagating along the gain medium is subject to narrowing along with shifting of its peak wavelength; (ii) even at moderate pumping the population of the excited singlet state, which determines the gain of the system, is non-uniform along the cell; (iii) it is possible to calculate the unsaturated gain by calculating the intensity of a particular wave-length and its spectral narrowing both as a function of the exciation and compare them with the same quantities measured experimentally; (iv) it is also possible to develop a semianalytic system independent method to measure the gain approximately. The theory developed to account for the propagation of the amplified spontaneous emission (ASE) has been partly extended to cover the case of the propagation and spectral narrowing of the ASE in a thick cell, where non-uniformities of the index of refraction and the gain are important along with the diffraction losses. In this particular case, it is shown that a model, which assumes an index step variation across the cell, and solves the Maxwell's equation for the field propagation along the cell, can account for the spatial distribution of the field across the cell and its manifestation at the far field. Most of the predictions of the model are verified experimentally. In particular, it is shown that (i) in a thick cell, part of the ASE propagates outside the gain medium, because of the lensing effect caused by heating of the lasing material; (ii) the field across the cell can exhibit stable spatial modes, which can produce a far field far from the amplifying cell axis; (iii) it is possible to improve the spectral narrowing of the ASE since saturation can be delayed to higher pumping than before and most of the narrowing occurs below saturation of the gain; (iv) it is also possible to measure the temperature and the index of refraction change due to heating by measuring the far field angle, and estimate the diffraction losses involved in the propagation of the ASE in a thick cell. Finally, a number of suggestions on further research are proposed.
The widely used technique for determining optical gain and absorption from single-pass, amplified spontaneous emission (ASE) is analyzed with particular attention given to active-volume saturation and three-dimensional effects. The results for homogeneously broadened media show that the population inversion and hence the gain in the active region is diminished by high levels of spontaneous and ASE. The externally measured gain is further reduced for large output collection apertures that admit incompletely amplified off-axis rays. Criteria are given for the excitation and detection geometries required to ensure accurate (∼10-percent) gain measurement. The simultaneous measurement of the equilibrium absorption coefficient can be made under less restrictive conditions.
Introduction In this chapter we will present the theory of spectral gain in optical amplifiers and the related optical power distribution. The concepts are general, as they apply to every optical amplifier configuration, independent of the specific architecture and implementation technology. We will configure the optical amplifying medium as a traveling-wave device, where the optical field undergoes optical amplification as it propagates from the input to the output sections. Generally speaking, optical amplification is achieved by a net stimulated emission process. Referring to a generic section z of infinitesimal thickness dz , optical gain is determined by the imbalance between net stimulated emission and cavity losses, including extrinsic absorption, reflection and radiated fields. As we know from the theory of light amplification in the three-level atomic system presented in Chapter 5, stimulated absorption of photons is governed by the same transition rate as stimulated emission, and is included in the net stimulated emission process. With this in mind, we note the identity between stimulated emission and the stimulated absorption rates, Γ 12 = Γ 21 , and the net stimulated photon term Γ[ j 2 ( t ) – j 1 ( t )] p ( t ) in the rate equation. In order to develop the traveling-wave model, the photon density becomes a function of the longitudinal position 0 ≤ z ≤ L along the amplifier medium. Accordingly, we will set p ( t , z ) as the relative density of stimulated photons per unit volume (0 ≤ p ( t , z ) ≤ 1) at time t and section z . When photons with appropriate energy proceed along the amplifying medium, they are amplified by means of net stimulated emission. At some section z = z 0 , the steady-state photon density P ( z ) can approach the saturation density P sat ( z ).
Amplified spontaneous emission of laser media having a spherical or disk shape is numerically analyzed. Some properties are discussed and a comparison with linear systems is made. Analytical approximations, for the case of high pumping rates and high efficiency, are obtained. Energy level schemes of dye systems are used in the analysis and in the numerical calculations. A coupled set of radiative transfer and rate equations is solved under quasi-steady-state conditions. The model takes into account the fluorescence spectrum and gain saturation effects with radially symmetric distributions of the active dye molecular densities. As a comparison, the numerical examples also include an H2O system which is relevant in astrophysics.
An investigation was made of a longitudinally pumped laser-single-pass dye amplifier system with a view to optimizing the total conversion efficiency. It was shown that competition between two processes–amplification of the external signal and of the spontaneous noise–determines the total efficiency of conversion of the pump into useful signal. The superfluorescence restricts the maximum gain and conversion efficiency of small external signals, as does the saturation by the signal being amplified in the case of large external signals. A quantitative analysis was made of the choice of optimal optical density of the amplifier and of the competition between two coupled waves in a nonlinearly amplifying medium.