The principle of remote-resonance spectroscopy

Wei Qin, Guilu Long

We develop a novel method for multiphoton controllable transport between remote resonators. Specifically, an auxiliary resonator is used to control the coherent long-range coupling of two spatially separated resonators, mediated by a coupled-resonator chain of arbitrary length. In this manner, an arbitrary multiphoton quantum state can be either transmitted through or reflected off the intermediate chain on demand, with very high fidelity. We find, on using a time-independent perturbative treatment, that quantum information leakage of an arbitrary Fock state is limited by two upper bounds, one for the transmitted case and the other for the reflected case. In principle, the two upper bounds can be made arbitrarily small, which is confirmed by numerical simulations.

J. I. Steinfeld, Paul L. Houston

U. Fano

Agata Cygan, Adam J. Fleisher, R. Ciuryło +3 more

Abstract Measurements of ultrahigh-fidelity absorption spectra can help validate quantum theory, engineer ultracold chemistry, and remotely sense atmospheres. Recent achievements in cavity-enhanced spectroscopy using either frequency-based dispersion or time-based absorption approaches have set new records for accuracy with uncertainties at the sub-per-mil level. However, laser scanning or susceptibility to nonlinearities limits their ultimate performance. Here we present cavity buildup dispersion spectroscopy (CBDS), probing the CO molecule as an example, in which the dispersive frequency shift of a cavity resonance is encoded in the cavity’s transient response to a phase-locked non-resonant laser excitation. Beating between optical frequencies during buildup exactly localizes detuning from mode center, and thus enables single-shot dispersion measurements. CBDS can yield an accuracy limited by the chosen frequency standard and measurement duration and is currently 50 times less susceptible to detection nonlinearity compared to intensity-based methods. Moreover, CBDS is significantly faster than previous frequency-based cavity-enhanced methods. The generality of CBDS shows promise for improving fundamental research into a variety of light–matter interactions.

Sune R. Svanberg

Jabir Chathanathil, Gengyuan Liu, Svetlana Malinovskaya

A theoretical framework for the remote detection of molecules is presented in which a quantum control technique, determined to maximize the vibrational coherence in coherent anti-Stokes Raman spectroscopy, is used to optimize the backscattered signal from a cloud of molecules.