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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Manipulation of Rydberg atoms by terahertz pulses

Guang-Rui Jia, Y. F. Liu, Kun Yu, Yizhuang Zhao

Published Nov 18, 2011• 0 citations
Publisher

Abstract

In this paper, ultrashort, unipolar electric-field (terahertz) pulses have been used to coherently control population transfer between Rydberg states in lithium atom. Our numerical results show that populations of lithium atoms can be driven to lower or higher n levels with a train of half-cycle pulses, and the the transition rate is sensitive to the static-electric-field strength, the main laser frequency, the optical pulse profile, and the chirp of the laser pulse. If the paramerters of the half-cycle pulses is optimized appropriately, the population can be transferred to the target state completely.

DOI
10.1117/12.907563

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In this paper, ultrashort, unipolar electric-field (terahertz) pulses have been used to coherently control population transfer between Rydberg states in lithium atom. Our numerical results show that populations of lithium atoms can be driven to lower or higher n levels with a train of half-cycle pulses, and the the transition rate is sensitive to the static-electric-field strength, the main laser frequency, the optical pulse profile, and the chirp of the laser pulse. If the paramerters of the half-cycle pulses is optimized appropriately, the population can be transferred to the target state completely.
Using the time-dependent multilevel approach (TDML), this paper studies the dynamics of coherent control of Rydberg lithium atoms and demonstrates that Rydberg lithium atoms can be transferred to states of higher principal quantum number by exposing them to specially designed frequency-chirped laser pulses. The population transfer from n = 70 to n = 75 states of lithium atoms with efficiency of more than 90% is achieved by means of the sequential adiabatic rapid passages. The results agree well with the experimental ones and show that the coherent control of the population transfer from the lower n to the higher n states can be accomplished by the optimization of the chirping parameters and the intensity of laser field.
Ultrashort, unipolar electric-field pulses have been used to coherently redistribute population between Rydberg states in sodium. The population in several Rydberg states is recorded simultaneously as a function of peak field. In addition, two temporally separated pulses have been used to interferometrically characterize the redistribution process. In the lowest fields, the experimental results are in agreement with the predictions of lowest-order perturbation theory. At slightly higher fields, still well below the ionization threshold, the redistribution process becomes nonperturbative, and a numerical integration of the time-dependent Schr\"odinger equation must be used to achieve partial agreement between theory and experiment.
We discuss a protocol for efficient and quick transfer of population between nearly one-dimensional Rydberg states by a chirped train of half-cycle pulses. The chirp refers both to the time interval and relative strength between subsequent pulses. The most spectacular result obtained by the use of this protocol is the transfer of over 10% of the initial population from the high-Rydberg state of n=50,80n=50,80n=50,80 to much lower ones of ${n}^{\ensuremath{'}}\ensuremath{\approx}10$ in a short time of the order of 1 ns.
Using a time-dependent multilevel approach, we demonstrate that lithium atoms can be transferred to states of lower principle quantum number by exposing them to a frequency chirped microwave pulse. The population transfer from n = 79 to n = 70 states of lithium atoms with more than 80% efficiency is achieved by means of the sequential two-photon Δn = −1 transitions. It is shown that the coherent control of the population transfer can be accomplished by the optimization of the chirping parameters and microwave field strength. The calculation results agree well with the experimental ones and novel explanations have been given to understand the experimental results.