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Scientific Reports

Efficient Single-Mode Photon-Coupling Device Utilizing a Nanofiber Tip

Sho Chonan, Shinya Kato, Takao Aoki

Published Apr 24, 2014• 31 citations
Publisher

Abstract

Single-photon sources are important elements in quantum optics and quantum information science. It is crucial that such sources be able to couple photons emitted from a single quantum emitter to a single propagating mode, preferably to the guided mode of a single-mode optical fiber, with high efficiency. Various photonic devices have been successfully demonstrated to efficiently couple photons from an emitter to a single mode of a cavity or a waveguide. However, efficient coupling of these devices to optical fibers is sometimes challenging. Here we show that up to 38% of photons from an emitter can be directly coupled to a single-mode optical fiber by utilizing the flat tip of a silica nanofiber. With the aid of a metallic mirror, the efficiency can be increased to 76%. The use of a silicon waveguide further increases the efficiency to 87%. This simple device can be applied to various quantum emitters.

DOI
10.1038/srep04785

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This thesis presents single photon generation and spectroscopy using quantum dots (q-dots) on optical nanofibers. Optical nanofibers are essentially vacuum-clad silica fibers with sub-wavelength diameter, which can support only the propagation of the fundamental mode through the guided mode. Optical nanofibers are realized using adiabatically tapered single mode optical fibers. Experiments were performed by depositing colloidal core-shell type CdSeTe (ZnS) q-dots on the optical nanofiber surface. A method is developed to deposit single q-dots systematically and reproducibly along the optical nanofiber. In the view point of investigation of fluorescence photon emission characteristics for single q-dots on optical nanofibers, the absolute fluorescence photon-count rates channeled into the nanofiber guided modes and the normalized photon correlations at various excitation laser intensities are measured. The results are able to obtain the product between the fluorescence photon channeling efficiency and the quantum efficiency of the single q-dots. However, the channeling efficiency cannot be determined without accurate information on the quantum efficiency of the single q-dots. Therefore, a method is devised to determine the channeling of fluorescence photons from single q-dots into the guided modes by measuring the fluorescence photon-count rates through the guided and radiation modes simultaneously. By measuring for various nanofiber diameters, a maximum channeling efficiency obtained to be 22.0 (±4.8)% at a fiber diameter of 350 nm for an emission wavelength of 780 nm. The measured results completely reproduce the theoretical predictions within the experimental error. We demonstrate in situ measurements of fluorescence quantum efficiency of single q-dots using the present nanofiber technique. We determine fluorescence quantum efficiency of single q-dots accurately by assuming the theoretical values for the channeling efficiency from the product of the channeling efficiency and the quantum efficiency. We demonstrate that one can pick up one q-dot on the nanofiber with fluorescence quantum efficiency higher than the average value measured for an ensemble. Thus, the optical nanofiber method offers a promising way for generating and manipulating single photons. This work should provide a basis for extending the optical nanofiber method to a general technique in quantum optics, which may open new possibilities in quantum information technologies.

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Single-photon sources are important elements in quantum optics and quantum information science. It is crucial that such sources be able to couple photons emitted from a single quantum emitter to a single propagating mode, preferably to the guided mode of a single-mode optical fiber, with high efficiency. Various photonic devices have been successfully demonstrated to efficiently couple photons from an emitter to a single mode of a cavity or a waveguide. However, efficient coupling of these devices to optical fibers is sometimes challenging. Here we show that up to 38% of photons from an emitter can be directly coupled to a single-mode optical fiber by utilizing the flat tip of a silica nanofiber. With the aid of a metallic mirror, the efficiency can be increased to 76%. The use of a silicon waveguide further increases the efficiency to 87%. This simple device can be applied to various quantum emitters.
Optical nanofiber-based single-photon source has attracted considerable interest due to its property of seamless integration with a single-mode fiber. With nanostructure engraved in the nanofiber, the single-photon collection efficiency can be greatly boosted with enhanced interaction between the single quantum emitter and the guided light. However, the prerequisite nanofabrication processes introduce complexities and extra loss. Here, we demonstrate that by simply placing a quantum emitter in the gap of two parallel nanofibers, single-photon coupling efficiency may reach 54.2%. Our numerical simulation results indicate that photon coupling efficiency of such simple structure is insensitive to the discrepancy in nanofiber radii, which further reduces the difficulties in device fabrication.
Nitrogen-Vacancy (NV) centers in diamond are promising solid-state quantum emitters that can be utilized for photonic quantum applications. Various diamond nanophotonic devices have been fabricated for efficient extraction of single photons emitted from NV centers to a single guided mode. However, for constructing scalable quantum networks, further efficient coupling of single photons to a guided mode of a single-mode fiber (SMF) is indispensable and a difficult challenge. Here, we propose a novel efficient hybrid system between an optical nanofiber and a cylindrical-structured diamond nanowire. The maximum coupling efficiency as high as 75% for the sum of both fiber ends is obtained by numerical simulations. The proposed hybrid system will provide a simple and efficient interface between solid-state quantum emitters and a SMF suitable for constructing scalable quantum networks.
In this talk, our recent activities for nanofiber-integrated single light emitters for photonic quantum network. First, we report the coupling of various single light emitters, including diamond nanocrystals with color centers and hexagonal Boron Nitride flakes, to ultra-thin tapered optical fibers (nano optical fiber) with a diameter as small as 300 nm, keeping the transmittance of the fiber more than 90%. Second, for further improvement of the coupling efficiency, we introduce our development of nanofiber Bragg cavity (NFBC) with the mode volume of under 1 mu m^3 and repeatable tuning capability over more than 20 nm at visible wavelengths. The improvement of Q factor using He-ion beam milling will also be reported.
We present a novel approach to enhance the spontaneous emission rate of single quantum emitters in an optical nanofiber-based cavity by introducing a narrow air-filled groove into the cavity. Our results show that the Purcell factor for single quantum emitters inside the groove of the nanofiber-based cavity can be at least six times greater than for such an emitter on the fiber surface when using an optimized cavity mode and groove width. Moreover, the coupling efficiency of single quantum emitters into the guided mode of this nanofiber-based cavity can reach up to ∼80% with only 35 cavity-grating periods. This new system has the potential to act as an all-fiber platform to realize efficient coupling of photons from single emitters into an optical fiber for quantum information applications.
This thesis presents single photon generation and spectroscopy using quantum dots (q-dots) on optical nanofibers. Optical nanofibers are essentially vacuum-clad silica fibers with sub-wavelength diameter, which can support only the propagation of the fundamental mode through the guided mode. Optical nanofibers are realized using adiabatically tapered single mode optical fibers. Experiments were performed by depositing colloidal core-shell type CdSeTe (ZnS) q-dots on the optical nanofiber surface. A method is developed to deposit single q-dots systematically and reproducibly along the optical nanofiber. In the view point of investigation of fluorescence photon emission characteristics for single q-dots on optical nanofibers, the absolute fluorescence photon-count rates channeled into the nanofiber guided modes and the normalized photon correlations at various excitation laser intensities are measured. The results are able to obtain the product between the fluorescence photon channeling efficiency and the quantum efficiency of the single q-dots. However, the channeling efficiency cannot be determined without accurate information on the quantum efficiency of the single q-dots. Therefore, a method is devised to determine the channeling of fluorescence photons from single q-dots into the guided modes by measuring the fluorescence photon-count rates through the guided and radiation modes simultaneously. By measuring for various nanofiber diameters, a maximum channeling efficiency obtained to be 22.0 (±4.8)% at a fiber diameter of 350 nm for an emission wavelength of 780 nm. The measured results completely reproduce the theoretical predictions within the experimental error. We demonstrate in situ measurements of fluorescence quantum efficiency of single q-dots using the present nanofiber technique. We determine fluorescence quantum efficiency of single q-dots accurately by assuming the theoretical values for the channeling efficiency from the product of the channeling efficiency and the quantum efficiency. We demonstrate that one can pick up one q-dot on the nanofiber with fluorescence quantum efficiency higher than the average value measured for an ensemble. Thus, the optical nanofiber method offers a promising way for generating and manipulating single photons. This work should provide a basis for extending the optical nanofiber method to a general technique in quantum optics, which may open new possibilities in quantum information technologies.
The interaction of photons with individual quantum systems is a very fundamental process in physics. Thereby, the emission rate as well as the angular emission pattern of a quantum emitter are not only a function of intrinsic properties of the emitter itself, but are also strongly modified by its surrounding. For instance, by restricting the optical modes which are allowed at the position of the dipole, the emission rate can be strongly modified and the emitted photons can be directed into specific optical modes. This effect can be demonstrated by the interaction of a single optically active quantum emitter with the strongly confined optical mode of a single-mode dielectric waveguide. Efficient coupling of the emitter to the dielectric structure can be achieved by placing the quantum emitter inside the evanescent field of the guided mode. This evanescent field coupling mechanism is discussed and demonstrated experimentally. A single nitrogen-vacancy center (NV-center), hosted in a nanodiamond is deterministically coupled to a tapered optical fiber (TOF) via the evanescent field of its guided mode (coupling efficiencies exceeding 30% are predicted). By employing an AFM-based nanomanipulation technique, the diamond nanocrystal is placed on the nanofiber waist of the TOF. Beforehand, the diamond nanocrystal has been characterized to guarantee that it hosts only one fluorescing NV-center. While the diamond nanocrystal is optically exited, single photon fluorescence of the NV-center is detected at both outputs of the tapered optical fiber. This verifies the evanescent coupling of the emitter to the guided mode. In order to quantify the coupling, the comparison of the emission rate into free space with the rate into the fiber yields that 10.0(5) of the emitted photons are coupled into the tapered optical fiber. In the determination of this value, the orientation of the emitting dipoles and the emission pattern, which are modified by the TOF, have been considered. The NV-center features a broad emission spectrum which can be used to investigate the wavelength-dependence of the coupling. Comparing the spectra of the emission into the fiber mode with the emission into free space modes roughly resembles the expected wavelength dependency of the coupling efficiency. The evanescent coupling and the deterministic positioning of preselected fluorescing diamond nanocrystals, which has been demonstrated with the TOF, can be applied to other waveguide structures as well. Dielectric single-mode waveguides made of Ta2O5 on a SiO2 substrate promise similar coupling efficiencies to tapered optical fibers (above 30%). With the design of the on-chip wave-guiding structure being flexible, the combination with other optical on-chip elements is feasible, rendering it a promising platform for on-chip photonic experiments. Test structures of this waveguide design are realized using lithographic processes and are characterized. These waveguides are equipped with inverted taper structures to allow efficient off-chip coupling with butt-coupling to standard single-mode fibers. The evanescent coupling of a single quantum emitter to a singe optical mode can be used to efficiently collect emission of the quantum emitter. This can help building a compact single photon source and is beneficial for the optical read-out of the quantum emitter's internal degree of freedom, which can be either used as probe (sensing) or as information-storage. Utilizing the high coupling efficiency, for instance, the non-linearities of the quantum system can be exploited to build a single photon transistor. The evanescent coupling is very broadband (about hundred nanometers), allowing to efficiently collect emission from broadband emitters like the NV-center, but it can also be used for multi-wavelength manipulation schemes.