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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Possibility of two-photon superradiance in microcavities

Mihai Macovei, N. A. Enaki

Published Jul 2, 1998• 0 citations
Publisher

Abstract

We analyze the two-photon cooperative emission of excited atoms in microcavities with dimensions of the order of the emission wavelength. Here the two-photon dipole-forbidden transitions between the upper and the ground states of the three-level system are possible through the intermediate level that is off resonance with microcavity modes. In this situation one obtains the powerful pulse of two-photon highly correlated light. The superbunching phenomenon in radiated field is also discussed.

DOI
10.1117/12.312781

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We analyze the two-photon cooperative emission of excited atoms in microcavities with dimensions of the order of the emission wavelength. Here the two-photon dipole-forbidden transitions between the upper and the ground states of the three-level system are possible through the intermediate level that is off resonance with microcavity modes. In this situation one obtains the powerful pulse of two-photon highly correlated light. The superbunching phenomenon in radiated field is also discussed.
We study the cooperative two-photon spontaneous decay of an excited atomic system in a microcavity whose size is of the order of several wavelengths of atomic radiation. We show that a thermalized electromagnetic field in the microcavity strongly affects the two-photon cooperative spontaneous emission of radiation. The increase in the rate of spontaneous cooperative decay is due to the presence of a small number of thermalized photons in a microcavity mode. At low temperatures, the two-photon absorption probability is found to be a linear function of the two-photon flux, and photon superbunching is observed.
The spontaneous emission from an atomic ensemble localized in a microcavity with the participation of microcavity photons and an external broadband quantized electromagnetic field at the Raman resonance of photons with an optically forbidden (two-photon) atomic transition has been studied. The average spontaneous decay intensity has been calculated for simple cases. It is shown that the dynamics of spontaneous emission from this atomic ensemble differs generally from the conventional superradiance (spontaneous emission of an atomic ensemble at a one-photon optically allowed transition from excited to the ground state. When the atomic ensemble is strongly excited, the delay times and the emission pulse shape differ significantly. The parameter ranges where the spontaneous emission from the atomic ensemble under consideration at a two-photon Raman transition can be described as conventional superradiance with renormalized parameters are found. In the case of single excitation the photon emission probability depends on the number of photons and atoms in the microcavity.
Superradiance, i.e., spontaneous emission of coherent radiation by an ensemble of two-level atoms in collective states introduced by Dicke in 1954, is one of the enigmatic problems of quantum optics. The startling gist is that even though the atoms have no dipole moment they radiate with increased intensity in particular directions. Following the advances in our understanding of superradiant emission by atoms in entangled W-states we examine the quantum statistical properties of superradiance. Such investigations require the system to have at least two excitations in order to explore the photon-photon correlations of the radiation emitted by such states. We present specifically results for the spatially resolved photon-photon correlations of systems prepared in doubly excited W-states and give conditions when the atomic system emits nonclassial light. Equally, we derive the conditions for the occurrence of bunching and even of superbunching, a rare phenomenon otherwise known only from nonclassical states of light like the squeezed vacuum. We finally investigate the photon-photon cross correlations of the spontaneously scattered light and highlight the nonclassicalty of such correlations. The theoretical findings can be implemented with current technology, e.g., using ions in a linear rf-trap, atoms in an optical lattice or quantum dots in a cavity.
The two-photon and scattering resonances between the spontaneous emissions of the two- and single- photon transitions of the three-level inverted radiators in the Ξ, V configurations and the system of two-level radiators D, inverted relatively the dipole forbidden transition are revised. This approach opens the new possibilities in the manipulation of the decay process and generation of the entangled photon pairs. The correlation between the V and Ξ cascade three-level subsystems on the two-photon transitions of dipole forbidden radiators is studied, taking into consideration the cooperative scattering and two photon resonances through the vacuum field. One of them corresponds to the situation when the total energy of emitted photons by three level dipole-active radiator in the cascade configuration enters into the two-photon resonance with the dipole-forbidden transitions of second atom. Another effect corresponds to the scattering situation, when the difference of the excited energies of the two dipole-active transitions of V three level radiator are in the resonance with the dipole-forbidden transitions of the second one. These effects are accompanied with the interferences between single- and two-quantum collective transitions of the inverted radiators from the ensemble. The two particle collective decay rate is defined in the description of the atomic correlation functions.
The ignition of two-quantum collective emission of inverted sub-ensemble of radiators due to mutual interaction of this sub-ensemble with other two dipole active atomic subsystems in process of two-photon exchanges between the atoms through the vacuum field is proposed. The three particle resonances between two-photon and single quantum transitions of inverted radiators from the ensemble are proposed for acceleration of collective decay rate of bi-photons, obtained relatively dipole-forbidden transitions of excited atomic sub-ensemble. This mutual interaction between three super-fluorescent processes in subatomic ensembles take place relatively dipole-forbidden transitions in one of radiator subsystem. The collective resonance emission and absorption of two-quanta have nontraditional behavior, accompanied with acceleration and inhibition of collective emission processes of photons.
We consider the possible physical processes that may arise in a three-level atom when only two of its levels interact with a strong electromagnetic field and when the atomic transition frequency is nearly equal to once and twice the frequency of the laser field, respectively. There have been found pronounced cooperative effects in the spectrum of the two-level system, which is in resonance with the laser field, arising from the presence of the third level. The excitation spectra describing the transitions from the first excited state into the second excited state and from that to the ground state consist, apart from the two central peaks, of two pairs of sidebands which are induced by the laser field of the neighbouring system. Detailed expressions of the spectral functions for the physical processes of one- and two-photon resonance fluorescence have been derived and discussed in the limit of high photon densities. The excitation spectrum of the low frequency modes has been considered and discussed in detail. It is found that quantum beats in spontaneous emission may appear in the spectra of the one- and two-photon resonance fluorescence arising from the interference between the two atomic transition frequencies and the frequency of the laser field. The importance of the low frequency modes that occur in the processes in question has been pointed out.