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Progress of Theoretical Physics

Mode Coupling Theory of Dynamic Critical Phenomena for Classical Liquids. I: Dynamic Critical Exponents

T. Ohta, Kyozi Kawasaki

Published May 1, 1976• 86 citations
Publisher

Abstract

The dynamic critical exponents of classical liquids are studied on the basis of the mode coupling theory. The shear viscosity for the spatial dimensionality between two and four exhibits the weak power law divergence at a critical point, which was briefly reported in a previous paper. The non-Markoffian effects and the vertex corrections are also investigated. It is shown that both corrections have only small contributions to the order parameter decay rate and do not affect the dynamic critical exponents.

DOI
10.1143/ptp.55.1384

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The dynamic critical exponents of classical liquids are studied on the basis of the mode coupling theory. The shear viscosity for the spatial dimensionality between two and four exhibits the weak power law divergence at a critical point, which was briefly reported in a previous paper. The non-Markoffian effects and the vertex corrections are also investigated. It is shown that both corrections have only small contributions to the order parameter decay rate and do not affect the dynamic critical exponents.
Recursion relations correct to lowest order in $\ensuremath{\epsilon}=4\ensuremath{-}d$ are obtained for simple models representing the critical dynamics of a binary liquid, a Heisenberg antiferromagnet, superfluid helium, and related systems. The exponents for the divergences of the transport coefficients satisfy the "scaling" relations predicted by mode-mode coupling theory. The viscosity of the binary liquid is predicted to diverge as ${k}^{\ensuremath{-}\frac{\ensuremath{\epsilon}}{19}}$ near d=4d=4d=4, which is a new result.
We discuss renormalization-group and mode-coupling theories of critical dynamics for several models. We show that to lowest order in $\ensuremath{\epsilon}={d}_{c}\ensuremath{-}d$, where for d>dcd>{d}_{c}d>dc​ conventional theory is valid, the renormalizationgroup differential equations are related by a simple transformation to those obtained from mode-coupling theory. Furthermore, the values of the dynamical fixed-point parameters essentially coincide with the critical amplitudes of the diverging transport coefficients, as determined by mode-coupling theory. In addition, we present a correct renormalization-group treatment for dynamical systems with more than one time scale, as for the binary liquid. We stress the fact that there are two distinct classes of critical dynamics, as illustrated by the results for the models studied here. We also discuss the instability of the conventional fixed point (time-dependent Ginzburg-Landau like) against mode-coupling perturbations for d<dcd<{d}_{c}d<dc​, with particular emphasis on a model for superfluid helium.
Power-law singularities and critical exponents in n-vector models are considered from different theoretical points of view. It includes a theoretical approach called the GFD (grouping of Feynman diagrams) theory, as well as the perturbative renormalization group (RG) treatment. A non-perturbative proof concerning corrections to scaling in the two-point correlation function of the phi^4 model is provided, showing that predictions of the GFD theory rather than those of the perturbative RG theory can be correct. Critical exponents determined from highly accurate experimental data very close to the lambda-transition point in liquid helium, as well as the Goldstone mode singularities in n-vector spin models, evaluated from Monte Carlo simulation results, are discussed with an aim to test the theoretical predictions. Our analysis shows that in both cases the data can be well interpreted within the GFD theory.
Power-law singularities and critical exponents in n-vector models are considered from different theoretical points of view. It includes a theoretical approach called the GFD (grouping of Feynman diagrams) theory, as well as the perturbative renormal- ization group (RG) treatment. A non-perturbative proof concerning corrections to scaling in the two-point correlation function of the ' 4 model is provided, showing that predictions of the GFD theory rather than those of the perturbative RG theory can be correct. Critical exponents determined from highly accurate experimental data very close to the �-transition point in liquid helium, as well as the Goldstone mode singularities in n-vector spin models, evaluated from Monte Carlo simulation results, are discussed with an aim to test the theoretical predictions. Our analysis shows that in both cases the data can be well interpreted within the GFD theory.
An introductory review to short-time critical dynamics is given. From the scaling relation valid already in the early stage of the evolution of a system at or near the critical point, one derives power law behaviour for various quantities. By a numerical simulation of the system one can measure the critical exponents and, by searching for the best power law behaviour, one can determine the critical point. Critical slowing down as well as finite size corrections are nearly absent, since the correlation length is still small for times far before equilibrium is reached. By measuring the (pseudo) critical points it is also possible to distinguish (weak) first-order from second-order phase transitions.
Equipped with the field theory representation of non-linear Langevin equations, the tools of dynamic perturbation theory, and the dynamic renormalization group introduced in Chapters 4 and 5, we are now in the position to revisit models for dynamic critical behavior that entail reversible mode couplings and other conserved hydrodynamic modes. We have already encountered some of these in Section 3.3. In models C and D, respectively, a non-conserved or conserved n -component order parameter is coupled to a conserved scalar field, the energy density. Through a systematic renormalization group analysis, we may critically assess the earlier predictions from scaling theory, and discuss the stability of fixed points characterized by strong dynamic scaling, wherein the order parameter and conserved non-critical mode fluctuate with equal rates, and weak dynamic scaling regimes, where these characteristic time scales differ. Next we investigate isotropic ferromagnets (model J), with the conserved spin density subject to reversible precession in addition to diffusive relaxation. Exploiting rotational invariance, we can now firmly establish the scaling relation z = ( d + 2 − η )/2. Similar symmetry arguments yield a scaling relation for the dynamic exponents associated with the order parameter and the non-critical fields in the O ( n )-symmetric SSS model that encompasses model E for planar ferromagnets and superfluid helium 4 (for n = 2), and model G for isotropic antiferromagnets ( n = 3). There exist competing strong- and weak-scaling fixed points, with the former stable to one-loop order, and characterized by z = d /2 for all slow modes.