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Reviews of Modern Physics

Experiments and theory in cold and ultracold collisions

J. Weiner, Vanderlei Salvador Bagnato, Sérgio Carlos Zílio, Paul S. Julienne

Published Jan 1, 1999• 976 citations
Publisher

Abstract

The authors review progress in understanding the nature of atomic collisions occurring at temperatures ranging from the millidegrees Kelvin to the nanodegrees Kelvin regime. The review includes advances in experiments with atom beams, light traps, and purely magnetic traps. Semiclassical and fully quantal theories are described and their appropriate applicability assessed. The review divides the subject into two principal categories: collisions in the presence of one or more light fields and ground-state collisions in the dark.

DOI
10.1103/revmodphys.71.1

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The authors review progress in understanding the nature of atomic collisions occurring at temperatures ranging from the millidegrees Kelvin to the nanodegrees Kelvin regime. The review includes advances in experiments with atom beams, light traps, and purely magnetic traps. Semiclassical and fully quantal theories are described and their appropriate applicability assessed. The review divides the subject into two principal categories: collisions in the presence of one or more light fields and ground-state collisions in the dark.
In the past two decades, the revolutionary technologies of creating cold and ultracold molecules have provided cutting-edge experiments for studying the fundamental phenomena of collision physics. To a large degree, the recent explosion of interest in the molecular collisions has been sparked by dramatic progress of experimental capabilities and theoretical methods, which permit molecular collisions to be explored deep in the quantum mechanical limit. Tremendous experimental advances in the field have already been achieved, and the authors, from an experimental perspective, provide a review of these studies for exploring the nature of molecular collisions occurring at temperatures ranging from the Kelvin to the nanoKelvin regime, as well as for applications of producing ultracold molecules.
Cold and ultracold collisions occupy a strategic position at the intersection of several powerful themes of current research in chemical physics, in atomic, molecular and optical physics, and even in condensed matter. The nature of these collisions has important consequences for optical manipulation of inelastic and reactive processes, precision measurement of molecular and atomic properties, matter-wave coherences and quantum-statistical condensates of dilute, weakly interacting atoms. This crucial position explains the wide interest and explosive growth of the field since its inception in 1987. The author reviews elements of the quantum theory of scattering theory, collisions taking place in the presence of one or more light fields, and collisions in the dark, below the photon recoil limit imposed by the presence of any light field. Finally, it reviews the essential properties of these mesoscopic quantum systems and describes the key importance of the scattering length to condensate stability.
Cold and ultracold collisions occupy a strategic position at the intersection of several powerful themes of current research in chemical physics, in atomic, molecular and optical physics, and even in condensed matter. The nature of these collisions has important consequences for optical manipulation of inelastic and reactive processes, precision measurement of molecular and atomic properties, matter–wave coherences and quantum-statistical condensates of dilute, weakly interacting atoms. This crucial position explains the wide interest and explosive growth of the field since its inception in 1987. The author reviews elements of the quantum theory of scattering theory, collisions taking place in the presence of one or more light fields, and collisions in the dark, below the photon recoil limit imposed by the presence of any light field. Finally, it reviews the essential properties of these mesoscopic quantum systems and describes the key importance of the scattering length to condensate stability.
The recent development of a range of new methods for producing samples of gas-phase molecules that are translationally cold ( K) or ultracold ( mK) is driving efforts to study reactive and inelastic collisional processes in these temperature regimes. In this review article the new methods for cold/ultracold molecule production are reviewed in the context of their potential or current use in collisional studies and progress in the application of these methods is highlighted. In these sub-Kelvin temperature ranges, where the de Broglie wavelength is long compared with molecular dimensions, quantum effects may play a crucial role in the collision dynamics. Reactions with no potential energy barrier are of greatest importance, and this review article summarizes some of the principal theoretical approaches to understanding quantum effects in these barrierless processes.
Abstract : This research program seeks to understand and control atomic collisions at ultracold temperatures where quantum and light-filed effects lead to new interactions between atoms. We have pursued experimental and theoretical investigations of optical shielding and suppression, and the nature of ground-state collisions in and near a Bose-Einstein condensate. This research shows how inelastic collisions can be turned on and turned off by light fields, how the scattering length of ultracold ground-state collisions might be altered by light fields.