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Optics Communications

Direct measurement of light-induced drift velocities in Rb-Ar mixtures

F. Wittgrefe, Alan D. Streater, Maarten D. Hoogerland, E. R. Eliel, J. P. Woerdman

Published Mar 1, 1989• 8 citations
Publisher
DOI
10.1016/0030-4018(89)90326-x

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Journal of Experimental and Theoretical Physics•Nov 1, 1999•5 citations
The spectral features of the light-induced drift (LID) velocity for rubidium atoms ( 85 Rb and 87 Rb) in an argon buffer medium and in binary buffer mixtures of noble gases (Ne + Ar, Ne + Kr, Ne + Xe, He + Ar, He + Kr, and He + Xe) have been investigated theoretically. A strong temperature dependence of the spectral shape of the LID signal for Rb atoms in an Ar atmosphere is predicted in the temperature range 450 K < T < 800 K. It is shown that the anomalous LID of Rb atoms in binary buffer mixtures of noble gases can be observed at almost any temperature (including the room one) depending on the fractions of neon or helium in these mixtures. The results obtained enable a highly accurate testing of the interatomic interaction potentials used to calculate the drift velocity for anomalous LID in LID experiments.
This paper is a theoretical study of the spectral features of the velocity of light-induced drift (LID) of lithium atoms ( 7 Li and 6 Li) in a binary mixture of noble gases: Ne + Ar, Ne + Kr, and Ne + Xe. The spectral shape of the LID signal is predicted to depend strongly on the fraction ξ of neon in the buffer mixture in the range ξ≈0.8–0.9 (ξ= N Ne / N b , where N Ne is the neon concentration, and N b is the total concentration of the buffer particles). When the velocity of anomalous LID is treated as a function of the radiation frequency, it is found to have one, three, five, or seven zeros and to differ substantially from the dispersion-curve-like behavior with one zero predicted by the standard LID theory with velocity-independent transport collision rates. The reason for these additional zeros of the drift velocity is the alternating-sign dependence on the lithium-atom velocity of the relative difference of transport rates of collisions between buffer particles and excited and unexcited atoms. What is also established is that the anomalous LID of lithium atoms can be observed at almost all temperatures, depending on the value of ξ. At a fixed temperature, anomalous LID can be observed only in a narrow range of values of the fraction of neon in the buffer mixture, Δξ≈0.02. The results make possible highly precise testing in the LID experiments of the interatomic potentials used in calculations of the velocity spectrum of anomalous LID.