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Physical Review Letters

Resonance Fluorescence from Semiconductor Quantum Dots: Beyond the Mollow Triplet

Anders Moelbjerg, Per Kaer, Michael Lorke, Jesper Mørk

Published Jan 3, 2012• 56 citations
Publisher

Abstract

We show that the resonance fluorescence spectrum of a quantum dot excited by a strong optical pulse contains multiple peaks beyond those of the Mollow triplet. We show that as the area of the optical pulse is increased, new side peaks split off the central peak and shift in frequency. A simple analytical theory has been derived, which quantitatively accounts for the appearance and position of the peaks. This theory explains the physics responsible for the multiple peaks. By considering the time-dependent spectrum we demonstrate a time ordering of the side peaks, which is further evidence for the suggested physical explanation.

DOI
10.1103/physrevlett.108.017401

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We show that the resonance fluorescence spectrum of a quantum dot excited by a strong optical pulse contains multiple peaks beyond those of the Mollow triplet. We show that as the area of the optical pulse is increased, new side peaks split off the central peak and shift in frequency. A simple analytical theory has been derived, which quantitatively accounts for the appearance and position of the peaks. This theory explains the physics responsible for the multiple peaks. By considering the time-dependent spectrum we demonstrate a time ordering of the side peaks, which is further evidence for the suggested physical explanation.
The coherent interaction between a two-level system and electromagnetic fields serves as a foundation for fundamental quantum physics and modern photonic quantum technology. A profound example is resonance fluorescence, where the non-classical photon emission appears in the form of a Mollow-triplet when a two-level system is continuously driven by a resonant laser. Pushing resonance fluorescence from a static to dynamic regime by using short optical pulses generates on-demand emissions of highly coherent single photons. Further increasing the driving strength in the dynamical regime enables the pursuit of exotic non-classical light emission in photon number superposition, photon number entanglement, and photon bundle states. However, the long-sought-after spectrum beyond the Mollow-triplet, a characteristic of dynamic resonance fluorescence under strong driving strength, has not been observed yet. Here we report the direct observation and systematic investigations of dynamic resonance fluorescence spectra beyond the Mollow-triplet in a solid-state cavity quantum electrodynamic system. The dynamic resonance fluorescence spectra with up to five pairs of side peaks, excitation detuning induced spectral asymmetry, and cavity filtering effect are observed and quantitatively modeled by a full quantum model with phonon scattering included. Time-resolved measurements further reveal that the multiple side peaks originate from interference of the emission associated with different temporal positions of the excitation pulses. Our work facilitates the generation of a variety of exotic quantum states of light with dynamic driving of two-level systems.
We study the two-time correlation function and the resonance fluorescence spectrum of a semiconductor quantum dot excited by a strong off-resonant laser pulse. The obtained analytical expressions exhibit a specific detuning-dependent damping of Rabi oscillations of the dressed quantum dot as well as a detuning-dependent width of Mollow-triplet lines. In the absence of pure dephasing, the central peak of the triplet is broadened, upon increasing detuning, but the blue and red side peaks are narrowed. We demonstrate that pure dephasing processes can invert these dependences. A crossover between the regimes of detuning-dependent narrowing and broadening of the side and central peaks is identified. The predicted effects are consistent with resent experimental results and numerical calculations.
Abstract The coherent interaction between a two-level system and electromagnetic fields serves as a foundation for fundamental quantum physics and modern photonic quantum technology. A profound example is resonance fluorescence, where the non-classical photon emission appears in the form of a Mollow-triplet when a two-level system is continuously driven by a resonant laser. Pushing resonance fluorescence from a static to dynamic regime by using short optical pulses generates on-demand emissions of highly coherent single photons. Further increasing the driving strength in the dynamical regime enables the pursuit of exotic non-classical light emission in photon number superposition, photon number entanglement, and photon bundle states. However, the long-sought-after spectrum beyond the Mollow-triplet, a characteristic of dynamic resonance fluorescence under strong driving strength, has not been observed yet. Here we report the direct observation and systematic investigations of dynamic resonance fluorescence spectra beyond the Mollow-triplet in a solid-state cavity quantum electrodynamic system. The dynamic resonance fluorescence spectra with up to five pairs of side peaks, excitation detuning induced spectral asymmetry, and cavity filtering effect are observed and quantitatively modeled by a full quantum model with phonon scattering included. Time-resolved measurements further reveal that the multiple side peaks originate from interference of the emission associated with different temporal positions of the excitation pulses. Our work facilitates the generation of a variety of exotic quantum states of light with dynamic driving of two-level systems.
The fluorescence spectrum of a strongly pumped two-level system is characterized by the Mollow triplet that has been observed in a variety of systems, ranging from atoms to quantum dots and superconducting qubits. We theoretically studied the fluorescence of a strongly pumped intersubband transition in a quantum well. Our results show that the many-electron nature of such a system leads to a modification of the usual Mollow theory. In particular, the intensity of the central peak in the fluorescence spectrum becomes a function of the electron coherence, allowing access to the coherence time of a two-dimensional electron gas through a fluorescence intensity measurement.
The thesis presents the investigations of the emission properties of the Mollow triplet (resonance fluorescence above emitter saturation) and dephasing effects in semiconductor quantum dots. The investigations of the Mollow triplet emission properties focus on the detuning dependent Mollow triplet emission especially the relative areas and width of the individual Mollow peaks. If both fine-structure components of the exciton are excited a Mollow quintuplet is experimentally observed, which is found to be in agreement with a theoretical model. In addition the indistinguishable photon emission from the individual Mollow sidebands is verified. The investigations on dephasing effects focus on the phonon-assisted incoherent excitation of a quantum dot and a comprehensive study of the emission properties under these excitation conditions. A second study focuses on the non-resonant emitter mode coupling of a quantum dot coupeld to two modes of the micro pillar cavity together with the corresponding emission properties.