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Physical Review A

Laser second threshold: Its exact analytical dependence on detuning and relaxation rates

A. A. Bakasov, N. B. Abraham

Published Aug 1, 1993• 15 citations
Publisher

Abstract

An exact analysis has been carried out for general analytical expressions for the second threshold of a single-mode homogeneously broadened laser and for the initial pulsation frequency at the second threshold, for arbitary physical values of the relaxation rates, and at an arbitrary detuning between the cavity frequency and the atomic resonance frequency. These expressions also give correspondingly exact forms for asymptotic cases that have been previously studied with some approximations. Earlier approximate results are partly confirmed and partly improved by these more general expressions. The physical status of various expressions and approximations is reconsidered and specified more clearly, including an analysis of what reasonably can be attained in lasers or masers. A general analytical proof is given of the fact that, for a larger detuning of the laser cavity from resonance, a higher value of the laser excitation is required to destabilize the steady-state solution (the second threshold). We also present results for the minimum value of the second threshold at fixed detuning as a function of the other parameters of the system and for the dependence of the ratio of the second threshold to the first threshold as a function of detuning. Minima of the second threshold and of the threshold ratio occur only if the population relaxation rate is equal to zero. The minima of the threshold ratio are shown to be bounded from above as well as from below (as functions of the relaxation rates, so long as the second threshold exists). The upper bound on the minima ratio is equal to 17. The variation of the second threshold in the semi-infinite parameter space of the decay rates is shown at various detunings in plots with a finite domain by normalizing the material relaxation rates to the cavity decay rate.

DOI
10.1103/physreva.48.1633

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An exact analysis has been carried out for general analytical expressions for the second threshold of a single-mode homogeneously broadened laser and for the initial pulsation frequency at the second threshold, for arbitary physical values of the relaxation rates, and at an arbitrary detuning between the cavity frequency and the atomic resonance frequency. These expressions also give correspondingly exact forms for asymptotic cases that have been previously studied with some approximations. Earlier approximate results are partly confirmed and partly improved by these more general expressions. The physical status of various expressions and approximations is reconsidered and specified more clearly, including an analysis of what reasonably can be attained in lasers or masers. A general analytical proof is given of the fact that, for a larger detuning of the laser cavity from resonance, a higher value of the laser excitation is required to destabilize the steady-state solution (the second threshold). We also present results for the minimum value of the second threshold at fixed detuning as a function of the other parameters of the system and for the dependence of the ratio of the second threshold to the first threshold as a function of detuning. Minima of the second threshold and of the threshold ratio occur only if the population relaxation rate is equal to zero. The minima of the threshold ratio are shown to be bounded from above as well as from below (as functions of the relaxation rates, so long as the second threshold exists). The upper bound on the minima ratio is equal to 17. The variation of the second threshold in the semi-infinite parameter space of the decay rates is shown at various detunings in plots with a finite domain by normalizing the material relaxation rates to the cavity decay rate.
We study the five semiclassical laser equations in the mean-field limit for the simple model of two-level atoms with homogeneous broadening in a single-mode unidirectional ring cavity, taking into account detuning between atomic and cavity frequencies. Our analysis concentrates on the properties of the laser at and beyond the second thresh-old in the bad-cavity case. We first show that the position of the second threshold depends on the excitation mechanism: When the pump parameter is increased either adiabatically or abruptly, two different thresholds occur. The sequence of periodic and chaotic solutions beyond the second threshold is then discussed as a function of the detuning and the pump parameter.
A high-intensity single-mode gas laser is analyzed by several mathematical methods. Exact numerical results are best obtained by solving for the coefficients of a Fourier series solution by using a backward recurrence scheme or a successive convergents method for evaluating a continued fraction. Numerical integration techniques can also be used to convert the periodic boundary conditions to initial conditions and then solve the resulting initial-value problem. Direct analytic integration leads to exact solutions in terms of Bessel functions for the special case of zero detuning, equal decay rates, and neglecting of collision broadening. For general single-mode operation, an improved analytic approximation [the second recursion relation approximation (2RCRA)] is obtained by taking an additional term in the recursion relations for the Fourier coefficients. This approximation predicts the existence of one of the secondary resonances in graphs of the spatially averaged population inversion and quadrature polarization coefficient densities and matches the exact solution from the position of the first resonance and outward independent of the intensity. The 2RCRA also matches the exact detuning curve except at small detunings. The first-order ("rate equation") approximation, by comparison, does not predict any secondary resonances and does not match the exact solution at higher intensities. A physical interpretation for the appearance of the secondary resonances is presented in terms of multiphoton interactions and a prediction for the positions of the resonances for the special case discussed above is obtained. As predicted by Greenstein the exact detuning curves show quantitatively that the Lamb dip decreases and disappears as the intensity increases for high excitations.
The results of the quantum theory of a laser given by Riska and Stenholm (see ibid., vol.3, p.536 (1970)) for the case of inhomogeneous broadening and detuning are re-derived by avoiding the Doppler limit approximation to show the exact influence of relaxation parameters on the theory. The threshold condition is seen to be dependent on gamma ab /ku where gamma ab is the relaxation parameter and ku the Doppler parameter. Its value is found to be higher than earlier results. It is noted that the photon distribution function at resonance is much closer to the corresponding distribution obtained from exact calculations for the tuned case. The photon number at the peak of the distribution curve is much lower than earlier values for comparable situations.
This paper presents new results for the steady states of a detuned ring laser with a saturable absorber. We employ a semiclassical model which assumes homogeneously broadened two-level atoms. We proceed by solving the Maxwell-Bloch equations for the longitudinal dependence of the steady states of this system, and then simplify our solution by use of the uniform-field approximation. We present uniform-field results for squared electric field versus operating frequency, and for each of these versus cavity tuning and laser excitation. Various cavity linewidths and both resonant and nonresonant amplifier and absorber line-center frequencies are considered. The most notable finding is that cavity detuning breaks the degeneracies found in the steady-state solutions of the fully tuned case. This leads to the prediction that an actual system will bifurcate from the zero-intensity solution to a steady-state solution as laser excitation increases from zero, rather than to the small-amplitude pulsations found for the model with exactly resonant tuning of the cavity and the media line centers. Other phenomena suggested by the steady-state results include tuning-dependent hysteresis and bistability, and instability in both intensity and frequency due to the appearance of one or more new steady-state solutions as tuning is varied. These effects of detuning are being tested by a linearized stability analysis whose results will be reported separately.
We provide a comprehensive analysis of the standard model of the bidirectional ring laser in which only one mode can be supported in each direction and in the limit that the polarization can be eliminated adiabatically. The interaction between the two counterpropagating modes can be derived and it is most naturally viewed as a coupling between them via scattering from a spatial grating formed in the population inversion. If the grating is a sufficiently small modulation of the spatial average of the population inversion, it can be approximated by a sinusoidal function. A systematic derivation of the model with only a sinusoidal grating for the homogeneously broadened case is presented that reveals and corrects errors in several previously published analyses. The stability of the steady-state solution is analyzed. The bidirectional steady-state solution is unstable and the unidirectional steady-state solutions may be stable or unstable depending on the parameters. The well-established result of bistability between the two modes when the cavity is tuned to resonance is recovered, a result that persists, in part, even when the losses between the two modes are different.With detuning, the unidirectional steady-state solutions can be destabilized, creating regions in the parameter space where only time-dependent solutions are found. For parameters characteristic of solid-state or molecular gas lasers, the instability can occur for very small detunings and even very close to the lasing threshold. Asymptotic limits of the instability boundaries for these parameters are presented. Additional results are derived formally for inhomogeneous broadening with a Lorentzian line shape and for arbitrary inhomogeneous linewidths. Explicit analytic results are presented in the limits of very small and very large inhomogeneous linewidths compared with the homogeneous linewidth. Time-dependent solutions in the homogeneously broadened case for relaxation rates appropriate to CO2{\mathrm{CO}}_{2}CO2​ lasers show that there are broad regions in the parameter space of gain and detuning for which the behavior is dynamically chaotic in the form of nearly ``square-wave'' alternation between the counterpropagating modes of the laser with irregular switching times. In other regions of that parameter space we find more irregular pulsations and pulse alternations. Regions of periodic pulsations also have been found.
We use the semiclassical strong-signal theory of the laser to predict and explain the onset of side-mode buildup in lasers with one oscillating mode. Two general categories are considered: one for which the side modes and the oscillating mode all have the same wavelength and the other for which they have different wavelengths. The treatments include an arbitrary amount of inhomogeneous broadening. Our approach unifies the treatments of the side-mode instabilities presented earlier and extends them to handle standing waves in addition to the previously treated running waves. We write the field and the population matrix elements as Fourier series in the adjacent-mode beat frequency. This approach has been used extensively in both multimode laser theory and saturation spectroscopy. This technique coincides with linear stability analyses used by others, provided that our beat frequency includes a contribution that is proportional to the complex side-mode gain. We give a solution that allows for detuned operation along with its simpler, centrally tuned special case. The connection with saturation spectroscopy clearly reveals that the side-mode instabilities require side-mode gain. For the single-wavelength case, nonlinear anomalous dispersion is also required. The side-mode gain and dispersion result from both inhomogeneous broadening and population pulsations. The lowest instability thresholds occur when both of these mechanisms play a role. The approach can also be used to treat instabilities in optical bistability by substituting the appropriate equation of state for the strong-mode intensity and by changing the sign of the absorption coefficient. In homogeneously broadened, standing-wave lasers, we show that multiwavelength instabilities depend strongly on the position of the medium in the cavity. We illustrate the theory by giving numerical results for the output pulsation frequency and for the instability threshold by using parameters that are appropriate for the He–Xe laser. These results correlate well with experimental observations.