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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Single photons cannot be extracted from the light of multi-atom light sources

Karl Otto Greulich

Published Aug 26, 2007• 2 citations
Publisher

Abstract

Throughout the development and confirmation of the photon concept, "Gedankenexperiments" have been invoked where a light source is attenuated until "only one photon is in the apparatus." Such a statement requires, however, knowledge on details of the light generation process, which were not known until the advent of true single-photon light sources such as isolated single atoms or molecules. Here, starting from a two atom light source, it is shown that probably multi-atom or multi-molecule light sources do not generate, even not in small fractions, antibunching photons and that attenuation down to one photon per time unit is not reliably possible. Thus, one of the strongest arguments in favour of the existence of single "photons" in free space, the accumulation time argument, which discusses the absorption of a single photon by a single atom or molecule, becomes questionable.

DOI
10.1117/12.735798

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Throughout the development and confirmation of the photon concept, "Gedankenexperiments" have been invoked where a light source is attenuated until "only one photon is in the apparatus." Such a statement requires, however, knowledge on details of the light generation process, which were not known until the advent of true single-photon light sources such as isolated single atoms or molecules. Here, starting from a two atom light source, it is shown that probably multi-atom or multi-molecule light sources do not generate, even not in small fractions, antibunching photons and that attenuation down to one photon per time unit is not reliably possible. Thus, one of the strongest arguments in favour of the existence of single "photons" in free space, the accumulation time argument, which discusses the absorption of a single photon by a single atom or molecule, becomes questionable.
Crucial experiments of physics, such as the quantum mechanical version of the double slit experiment, have so far not been performed with true single (antibunching) photons. Instead, attenuated classical light sources such as bulbs or lasers have been suggested to provide the photons in these experiments. Since attenuators do not change photon statistics, i.e. do not convert classical into non - classical light, reliable single photon beams cannot be generated on this way. Antibunching sources, for example single molecules, are required. Due to the lack of such sources in the past, some extrapolations from the many - photon case to the one photon case have remained speculative, for example the long wavetrain model for a single photon. Alternative hypotheses, elaborated by considering details of the emission of single photons by single molecules are equally probable. Arguments are presented which disfavour the wavetrain model and favour the short pulse as a model for a photon.
Single molecule techniques improve our understanding of the photon and light. If the single photon double slit experiment is performed at the "single photon limit" of a multi-atom light source, faint light pulses with more than one photon hamper the interpretation. Single molecules, quantum dots or defect centres in crystals should be used as light source. "Single photon detectors" do not meet their promise-only "photon number resolving single photon detectors" do so. Particularly, the accumulation time argument, the only safe basis for the postulate of a strictly particle like photon, has so far not yet been verified.
Quantum mechanics does neither give information on details of the emission of a photon from a single atom or molecule nor on the physical size of a photon. Experiments to get answers to such questions have, at least in principle, become possible only recently with the advent of single molecule photon sources. If diffraction of light at wavelength sized apertures is already a property of individual photons, some clear statements on emisission can be made: The energy of an individual photon, which at the start of the process is concentrated in an Angstrom sized atom or molecule, is diluted to micrometer dimensions, i.e. by many orders of magnitude. Since single photons can still be detected at least 18 m after their emission, the dilution must be terminated at some point. A photon model presented in an accompanying paper suggests a size for a photon of λ / 2π and explains what does stop and revert the expansion process, thus starting an oscillation.
The concept of the photon , central to Einstein's explanation of the photoelectric effect, is exactly 100 years old. Yet, while photons have been detected individually for more than 50 years, devices producing individual photons on demand have only appeared in the last few years. New concepts for single-photon sources, or 'photon guns', have originated from recent progress in the optical detection, characterization and manipulation of single quantum objects. Single emitters usually deliver photons one at a time. This so-called antibunching of emitted photons can arise from various mechanisms, but ensures that the probability of obtaining two or more photons at the same time remains negligible. We briefly recall basic concepts in quantum optics and discuss potential applications of single-photon states to optical processing of quantum information: cryptography, computing and communication. A photon gun's properties are significantly improved by coupling it to a resonant cavity mode, either in the Purcell or strong-coupling regimes. We briefly recall early production of single photons with atomic beams, and the operation principles of macroscopic parametric sources, which are used in an overwhelming majority of quantum-optical experiments. We then review the photophysical and spectroscopic properties and compare the advantages and weaknesses of various single nanometre-scale objects used as single-photon sources: atoms or ions in the gas phase and, in condensed matter, organic molecules, defect centres, semiconductor nanocrystals and heterostructures. As new generations of sources are developed, coupling to cavities and nano-fabrication techniques lead to improved characteristics, delivery rates and spectral ranges. Judging from the brisk pace of recent progress, we expect single photons to soon proceed from demonstrations to applications and to bring with them the first practical uses of quantum information.