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Bulletin of the American Physical Society

Effects of Multi-pulse Dynamical Decoupling Schemes on Dephasing in a GaAs Spin Qubit

James Medford, Christian Barthel, Charles M. Marcus, Micah P. Hanson, Arthur C. Gossard

Published Mar 24, 2011• 0 citations
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Decoherence and Dynamical Decoupling in Solid-State Spin Qubits

Wayne M. Witzel

This dissertation is a study of the decoherence of a solid-state spin qubit, either that of a localized electron spin or a donor nucleus, caused by a nuclear spin bath relevant to semiconductor quantum computer architectures. In the presence of an external magnetic field and at low temperatures, the dominant decoherence mechanism is the spectral diffusion of the qubit spin resonance frequency due to the temporally fluctuating random magnetic field associated with the dipolar interaction induced flip-flops of nuclear spin pairs. The qubit spin dephasing due to this random magnetic field depends intricately on the quantum dynamics of the nuclear spin bath, making the coupled decoherence problem difficult to solve. We provide a formally exact solution of this non-Markovian quantum decoherence problem which numerically calculates accurate spin decoherence at short times, of particular relevance in solid-state spin quantum computer architectures. A quantum cluster expansion method is motivated, developed, and tested for the spectral diffusion problem. The method is applicable to any ideal pulse sequence applied to the qubit. Dynamical decoupling sequences, which aim to prolong qubit coherence, are analyzed. In particular, concatenated dynamical decoupling sequences are shown to prolong not only the coherence time over the entire sequence but also the length of time between pulses necessary to maintain coherence. This is shown to result from successive low-order cancellations in applicable perturbative expansions with each level of concatenation. Each cancellation, however, will require the inclusion, in the cluster expansion, of increasingly large clusters to obtain the lowest-order results. These larger clusters in the lowest order often dominate decoherence and therefore invalidate, as being overly optimistic, the pair approximation as a means to study the effect of concatenated dynamical decoupling. We present numerical results from our cluster expansion technique for echoes of single (Hahn), concatenated, and periodic pulse sequences using realistic models of a localized electron in phosphorus doped Si and in a GaAs quantum dot and of a P donor nucleus in Si or GaAs. In the Si:P electron spin decoherence problem, we consider, along with spectral diffusion, the effects of anisotropic hyperfine (AHF) interactions and suggest a technique to suppress electron spin echo envelope modulations (ESEEM), an additional source of decoherence resulting from the AHF interactions. Our calculations for the Si:P Hahn echoes, including the effects of both anisotropic hyperfine interactions and spectral diffusion, are in excellent agreement with experimental results. Our calculations of concatenated pulse sequence echoes offer important predictions for the effectiveness of a promising strategy to preserve qubit coherence in semiconductor quantum computer architectures.

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Dynamical decoupling (DD) and bath engineering are two parallel techniques employed to mitigate qubit decoherence resulting from their unavoidable coupling to the environment. Here, we present a hybrid DD approach that integrates pulsed DD with bath spin polarization to enhance qubit coherence within the central spin model. This model, which can be realized using GaAs semiconductor quantum dots or analogous quantum simulators, demonstrates a significant extension of the central spin's coherence time by approximately 2 to 3 orders of magnitude that compared with the free-induced decay time, where the dominant contribution from DD and a moderate improvement from spin-bath polarization. This study, which integrates uniaxial dynamical decoupling and auxiliary bath-spin engineering, paves the way for prolonging coherence times in various practical quantum systems, including GaAs/AlGaAs, silicon and Si/SiGe. And this advancement holds substantial promise for applications in quantum information processing.

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Comparison of Dynamical Decoupling Schemes in Double Quantum Dot Spin Qubits

Christian Barthel, James Medford, Hendrik Bluhm +3 more

Bulletin of the American Physical Society•Mar 15, 2010•0 citations
In order to achieve the high-fidelity quantum control needed for a broad range of quantum information technologies, reducing the effects of noise and system inhomogeneities is an essential task. It is well known that a system can be decoupled from noise or made insensitive to inhomogeneous dephasing dynamically by using carefully designed pulse sequences based on square or delta-function waveforms such as Hahn spin echo or CPMG. However, such ideal pulses are often challenging to implement experimentally with high fidelity. Here, we uncover a new geometrical framework for visualizing all possible driving fields, which enables one to generate an unlimited number of smooth, experimentally feasible pulses that perform dynamical decoupling or dynamically corrected gates to arbitrarily high order. We demonstrate that this scheme can significantly enhance the fidelity of single-qubit operations in the presence of noise and when realistic limitations on pulse rise times and amplitudes are taken into account.
This dissertation is a study of the decoherence of a solid-state spin qubit, either that of a localized electron spin or a donor nucleus, caused by a nuclear spin bath relevant to semiconductor quantum computer architectures. In the presence of an external magnetic field and at low temperatures, the dominant decoherence mechanism is the spectral diffusion of the qubit spin resonance frequency due to the temporally fluctuating random magnetic field associated with the dipolar interaction induced flip-flops of nuclear spin pairs. The qubit spin dephasing due to this random magnetic field depends intricately on the quantum dynamics of the nuclear spin bath, making the coupled decoherence problem difficult to solve. We provide a formally exact solution of this non-Markovian quantum decoherence problem which numerically calculates accurate spin decoherence at short times, of particular relevance in solid-state spin quantum computer architectures. A quantum cluster expansion method is motivated, developed, and tested for the spectral diffusion problem. The method is applicable to any ideal pulse sequence applied to the qubit. Dynamical decoupling sequences, which aim to prolong qubit coherence, are analyzed. In particular, concatenated dynamical decoupling sequences are shown to prolong not only the coherence time over the entire sequence but also the length of time between pulses necessary to maintain coherence. This is shown to result from successive low-order cancellations in applicable perturbative expansions with each level of concatenation. Each cancellation, however, will require the inclusion, in the cluster expansion, of increasingly large clusters to obtain the lowest-order results. These larger clusters in the lowest order often dominate decoherence and therefore invalidate, as being overly optimistic, the pair approximation as a means to study the effect of concatenated dynamical decoupling. We present numerical results from our cluster expansion technique for echoes of single (Hahn), concatenated, and periodic pulse sequences using realistic models of a localized electron in phosphorus doped Si and in a GaAs quantum dot and of a P donor nucleus in Si or GaAs. In the Si:P electron spin decoherence problem, we consider, along with spectral diffusion, the effects of anisotropic hyperfine (AHF) interactions and suggest a technique to suppress electron spin echo envelope modulations (ESEEM), an additional source of decoherence resulting from the AHF interactions. Our calculations for the Si:P Hahn echoes, including the effects of both anisotropic hyperfine interactions and spectral diffusion, are in excellent agreement with experimental results. Our calculations of concatenated pulse sequence echoes offer important predictions for the effectiveness of a promising strategy to preserve qubit coherence in semiconductor quantum computer architectures.
Dynamical decoupling (DD) and bath engineering are two parallel techniques employed to mitigate qubit decoherence resulting from their unavoidable coupling to the environment. Here, we present a hybrid DD approach that integrates pulsed DD with bath spin polarization to enhance qubit coherence within the central spin model. This model, which can be realized using GaAs semiconductor quantum dots or analogous quantum simulators, demonstrates a significant extension of the central spin's coherence time by approximately 2 to 3 orders of magnitude that compared with the free-induced decay time, where the dominant contribution from DD and a moderate improvement from spin-bath polarization. This study, which integrates uniaxial dynamical decoupling and auxiliary bath-spin engineering, paves the way for prolonging coherence times in various practical quantum systems, including GaAs/AlGaAs, silicon and Si/SiGe. And this advancement holds substantial promise for applications in quantum information processing.